Chemical Engineering Journal, volume 375, pages 121922

A highly ionic conductive poly(methyl methacrylate) composite electrolyte with garnet-typed Li6.75La3Zr1.75Nb0.25O12 nanowires

孙建宁 Sun Jianning ¹

Yaogang Li ²

Qinghong Zhang ²

Chengyi Hou ¹

Qiuwei Shi ^{3, 4}

Hongzhi Wang ¹

Hide authors affiliations Show authors affiliations: 4 affiliations

State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and Engineering Donghua University Shanghai 201620 PR China |

Engineering Research Center of Advanced Glasses Manufacturing Technology, Ministry of Education, Donghua University, Shanghai 201620, PR China |

School of Materials Science and Engineering, Nanyang Technological University, 639798, Singapore |

⁴

State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua University, Shanghai 201620, PR China |

Publication type: Journal Article

Publication date: 2019-11-01

Elsevier

Journal: Chemical Engineering Journal

Quartile SCImago

Quartile WOS

Impact factor: 15.1

ISSN: 13858947, 03009467

DOI: 10.1016/j.cej.2019.121922

Copy DOI

General Chemistry

General Chemical Engineering

Industrial and Manufacturing Engineering

Environmental Chemistry

Abstract

Composite solid polymer electrolytes, integrating advantages (inflammability and electrochemical stability) of inorganic parts and virtues (lower interfacial resistance, flexibility and handy preparation) of polymer matrix, present a promising prospect for safe high-energy solid-state lithium energy storage systems. Herein, one-dimensional garnet-typed Li6.75La3Zr1.75Nb0.25O12 nanowires are successfully synthesized, and the nanowires are complexed with poly(methyl methacrylate), lithium perchlorate to fabricate composite solid polymer electrolyte membranes via a facile solution-casting method. The ionic conductivity is sharply increased from 5.98 × 10−7 of filler-free solid electrolyte to 2.20 × 10−5 S cm−1 of composite solid polymer electrolyte at room temperature, because the interaction between nanowires and polymer chains provide more free volume and special ionic conductive channels. In the meantime, the composite solid polymer electrolytes exhibit the wide electrochemical window and good stability against lithium anode. The feasibility of composite solid polymer electrolyte is examined in LiCoO2/Li configuration at 0.2 C under 60 and 70 °C, the cells deliver discharge capacity of 134.6 and 143.6 mAh g−1 at first cycle and kept 92.3%, 71.8% retention after 80 and 65 cycles respectively. The results indicate that the as-prepared composite solid polymer electrolytes will be a promising candidate for solid-state lithium batteries in the future.

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Citations by publishers

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Elsevier	Elsevier, 27, 42.86% Elsevier 27 publications, 42.86%
Springer Nature	Springer Nature, 9, 14.29% Springer Nature 9 publications, 14.29%
Wiley	Wiley, 9, 14.29% Wiley 9 publications, 14.29%
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Sun Jianning 孙. et al. A highly ionic conductive poly(methyl methacrylate) composite electrolyte with garnet-typed Li6.75La3Zr1.75Nb0.25O12 nanowires // Chemical Engineering Journal. 2019. Vol. 375. p. 121922.

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Sun Jianning 孙., Li Y., Zhang Q., Hou C., Shi Q., Wang H. A highly ionic conductive poly(methyl methacrylate) composite electrolyte with garnet-typed Li6.75La3Zr1.75Nb0.25O12 nanowires // Chemical Engineering Journal. 2019. Vol. 375. p. 121922.

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RIS Copy

TY - JOUR

DO - 10.1016/j.cej.2019.121922

UR - https://doi.org/10.1016/j.cej.2019.121922

TI - A highly ionic conductive poly(methyl methacrylate) composite electrolyte with garnet-typed Li6.75La3Zr1.75Nb0.25O12 nanowires

T2 - Chemical Engineering Journal

AU - Sun Jianning, 孙建宁

AU - Li, Yaogang

AU - Zhang, Qinghong

AU - Hou, Chengyi

AU - Shi, Qiuwei

AU - Wang, Hongzhi

PY - 2019

DA - 2019/11/01 00:00:00

PB - Elsevier

SP - 121922

VL - 375

SN - 1385-8947

SN - 0300-9467

ER -

BibTex

Cite this

BibTex Copy

@article{2019_Sun Jianning,

author = {孙建宁 Sun Jianning and Yaogang Li and Qinghong Zhang and Chengyi Hou and Qiuwei Shi and Hongzhi Wang},

title = {A highly ionic conductive poly(methyl methacrylate) composite electrolyte with garnet-typed Li6.75La3Zr1.75Nb0.25O12 nanowires},

journal = {Chemical Engineering Journal},

year = {2019},

volume = {375},

publisher = {Elsevier},

month = {nov},

url = {https://doi.org/10.1016/j.cej.2019.121922},

pages = {121922},

doi = {10.1016/j.cej.2019.121922}

}

Found error?

Publisher

Elsevier

Journal

Chemical Engineering Journal

Quartile SCImago

Quartile WOS

Impact factor

15.1

ISSN

13858947 (Print)
03009467 (Print)