Chemical Engineering Journal, volume 382, pages 122935

In-situ crosslinked single ion gel polymer electrolyte with superior performances for lithium metal batteries

Xiang Guan ¹

Qingping Wu ^{2, 3}

Xiaowan Zhang ¹

Xuhong Guo ¹

Chilin Li

Chilin Li ⁴

Jun Xu ¹

Jun Xu

Hide authors affiliations Show authors affiliations: 4 affiliations

State-Key Laboratory of Chemical Engineering,East China University of Science and Technology,Shanghai 200237,China) |

State Key Laboratory of Chemical Engineering East China University of Science and Technology Shanghai 200237 China |

State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 585 He Shuo Road, Shanghai, 201899, China |

⁴

State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 585 He Shuo Road, Shanghai 201899, China |

Publication type: Journal Article

Publication date: 2020-02-01

Elsevier

Journal: Chemical Engineering Journal

Quartile SCImago

Quartile WOS

Impact factor: 15.1

ISSN: 13858947, 03009467

DOI: 10.1016/j.cej.2019.122935

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General Chemistry

General Chemical Engineering

Industrial and Manufacturing Engineering

Environmental Chemistry

Abstract

Conventional dual-ion conductive gel polymer electrolytes (GPEs) attracted tremendous interest for their combined advantages of liquid and solid electrolytes. However, their cycling performance usually degrades due to the concentration polarization of anions. Single lithium ion gel polymer electrolytes (SLIGPEs), which have anions covalently bonded to the polymer or inorganic backbone, can suppress the motion of anions by the interactions between the pedant anions and mobile ions. Especially, Li+ deposition in SLIGPEs can be regulated uniformly to avoid lithium dendrite growth. Herein, novel 3D-structured SLIGPEs were prepared by in-situ crosslinking of lithium (4-styrenesulfonyl) (trifluoromethanesulfonyl) imide (LiSTFSI) with polyethylene glycol dimethacrylate (PEGDMA), soaked with liquid electrolyte. The obtained SLIGPEs not only promote the absorption of liquid electrolyte and accelerate the transport of Li+, but also show a high limitation for the migration of anions, proved by high ionic conductivity (2.74 × 10−5 S cm−1 at room temperature) and high lithium ion transference number (0.622) of SLIGPE-3.5, respectively. The long cycle life (cycling for over 600 h under 0.05 mA cm−2 and 0.1 mA cm−2) of symmetric lithium batteries with SLIGPEs as both separator and electrolyte exhibits good interfacial stability between SLIGPEs and electrodes. Meanwhile, LiFePO4/SLIGPE-2/Li shows a specific discharge capacity of 132.1 mAh g−1 at 0.1 C, 80.0% of the capacity retention ratio and 99.0% of the coulombic efficiency after 150 cycles at room temperature. Moreover, confirmed by SEM, lithium dendrite growth is significantly suppressed during repeated Li plating/stripping cycles. Density functional theory calculations (DFT) confirm the mutual interactions between STFSI− pendants and ions in electrolytes and that between PEO segments and ions. We believe that these in-situ SLIGPEs with superior performances have great potential for the application in lithium metal batteries.

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Citations by journals

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Chemical Engineering Journal	Chemical Engineering Journal, 11, 11.34% Chemical Engineering Journal 11 publications, 11.34%
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ACS Applied Energy Materials	ACS Applied Energy Materials, 4, 4.12% ACS Applied Energy Materials 4 publications, 4.12%
Energy Storage Materials	Energy Storage Materials, 3, 3.09% Energy Storage Materials 3 publications, 3.09%
Applied Surface Science	Applied Surface Science, 3, 3.09% Applied Surface Science 3 publications, 3.09%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 3, 3.09% Journal of Materials Chemistry A 3 publications, 3.09%
ACS Energy Letters	ACS Energy Letters, 2, 2.06% ACS Energy Letters 2 publications, 2.06%
Journal of Solid State Electrochemistry	Journal of Solid State Electrochemistry, 2, 2.06% Journal of Solid State Electrochemistry 2 publications, 2.06%
Journal of Energy Chemistry	Journal of Energy Chemistry, 2, 2.06% Journal of Energy Chemistry 2 publications, 2.06%
eScience	eScience, 2, 2.06% eScience 2 publications, 2.06%
Chinese Chemical Letters	Chinese Chemical Letters, 2, 2.06% Chinese Chemical Letters 2 publications, 2.06%
Electrochimica Acta	Electrochimica Acta, 2, 2.06% Electrochimica Acta 2 publications, 2.06%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 2, 2.06% Journal of Colloid and Interface Science 2 publications, 2.06%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 2, 2.06% Physical Chemistry Chemical Physics 2 publications, 2.06%
Journal of Energy Storage	Journal of Energy Storage, 2, 2.06% Journal of Energy Storage 2 publications, 2.06%
Royal Society Open Science	Royal Society Open Science, 1, 1.03% Royal Society Open Science 1 publication, 1.03%
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Cellulose	Cellulose, 1, 1.03% Cellulose 1 publication, 1.03%
Ionics	Ionics, 1, 1.03% Ionics 1 publication, 1.03%
Macromolecular Research	Macromolecular Research, 1, 1.03% Macromolecular Research 1 publication, 1.03%
Inorganica Chimica Acta	Inorganica Chimica Acta, 1, 1.03% Inorganica Chimica Acta 1 publication, 1.03%
Nano Energy	Nano Energy, 1, 1.03% Nano Energy 1 publication, 1.03%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 1, 1.03% Journal of Alloys and Compounds 1 publication, 1.03%
Batteries & Supercaps	Batteries & Supercaps, 1, 1.03% Batteries & Supercaps 1 publication, 1.03%
Advanced Energy Materials	Advanced Energy Materials, 1, 1.03% Advanced Energy Materials 1 publication, 1.03%
Advanced Materials Interfaces	Advanced Materials Interfaces, 1, 1.03% Advanced Materials Interfaces 1 publication, 1.03%
Macromolecular Materials and Engineering	Macromolecular Materials and Engineering, 1, 1.03% Macromolecular Materials and Engineering 1 publication, 1.03%
	2 4 6 8 10 12

Citations by publishers

	5 10 15 20 25 30 35 40 45
Elsevier	Elsevier, 45, 46.39% Elsevier 45 publications, 46.39%
American Chemical Society (ACS)	American Chemical Society (ACS), 19, 19.59% American Chemical Society (ACS) 19 publications, 19.59%
Wiley	Wiley, 11, 11.34% Wiley 11 publications, 11.34%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 10, 10.31% Royal Society of Chemistry (RSC) 10 publications, 10.31%
Springer Nature	Springer Nature, 6, 6.19% Springer Nature 6 publications, 6.19%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 2.06% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 2.06%
The Royal Society	The Royal Society, 1, 1.03% The Royal Society 1 publication, 1.03%
Polymer Society of Korea	Polymer Society of Korea, 1, 1.03% Polymer Society of Korea 1 publication, 1.03%
The Electrochemical Society	The Electrochemical Society, 1, 1.03% The Electrochemical Society 1 publication, 1.03%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.03% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.03%
	5 10 15 20 25 30 35 40 45

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Guan X. et al. In-situ crosslinked single ion gel polymer electrolyte with superior performances for lithium metal batteries // Chemical Engineering Journal. 2020. Vol. 382. p. 122935.

GOST all authors (up to 50) Copy

Guan X., Wu Q., Zhang X., Guo X., Li C., Li C., Xu J., Xu J. In-situ crosslinked single ion gel polymer electrolyte with superior performances for lithium metal batteries // Chemical Engineering Journal. 2020. Vol. 382. p. 122935.

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RIS Copy

TY - JOUR

DO - 10.1016/j.cej.2019.122935

UR - https://doi.org/10.1016/j.cej.2019.122935

TI - In-situ crosslinked single ion gel polymer electrolyte with superior performances for lithium metal batteries

T2 - Chemical Engineering Journal

AU - Guan, Xiang

AU - Wu, Qingping

AU - Zhang, Xiaowan

AU - Guo, Xuhong

AU - Li, Chilin

AU - Xu, Jun

AU - Li, Chilin

AU - Xu, Jun

PY - 2020

DA - 2020/02/01 00:00:00

PB - Elsevier

SP - 122935

VL - 382

SN - 1385-8947

SN - 0300-9467

ER -

BibTex

Cite this

BibTex Copy

@article{2020_Guan,

author = {Xiang Guan and Qingping Wu and Xiaowan Zhang and Xuhong Guo and Chilin Li and Jun Xu and Chilin Li and Jun Xu},

title = {In-situ crosslinked single ion gel polymer electrolyte with superior performances for lithium metal batteries},

journal = {Chemical Engineering Journal},

year = {2020},

volume = {382},

publisher = {Elsevier},

month = {feb},

url = {https://doi.org/10.1016/j.cej.2019.122935},

pages = {122935},

doi = {10.1016/j.cej.2019.122935}

}

Found error?

Publisher

Elsevier

Journal

Chemical Engineering Journal

Quartile SCImago

Quartile WOS

Impact factor

15.1

ISSN

13858947 (Print)
03009467 (Print)