Elsevier
Chemical Engineering and Processing: Process Intensification
,  том 150 ,  страницы 107876

Simulation of diesel autothermal reforming over Rh/Ce0.75Zr0.25O2-δ-η-Al2O3/FeCrAl wire mesh honeycomb catalytic module

Тип публикации: Journal Article
Дата публикации: 2020-04-01
Elsevier
scimago Q1
wos Q2
БС1
SJR: 0.794
CiteScore: 7.9
Impact factor: 3.9
ISSN: 02552701, 18733204
General Chemistry
General Chemical Engineering
Process Chemistry and Technology
Industrial and Manufacturing Engineering
Energy Engineering and Power Technology
Краткое описание
The study was dedicated to the mathematical modeling of the catalytic autothermal reforming (ATR) of diesel fuel – effective method for hydrogen production. The structured wire mesh Rh/Ce0.75Zr0.25O2-δ-η-Al2O3/FeCrAl catalyst was tested in pilot scale reactor and showed high efficiency in studied diesel autothermal reaction conditions. The process simulation was carried out by commercial software COMSOL Multiphysics in 2D axisymmetric geometry. The catalyst module was simulated as homogeneous porous medium. Reaction model included diesel oxidation, diesel steam reforming, water-gas shift reaction, CO methanation, CO oxidation and hydrogen oxidation. Fitting the experimental results including product distribution and temperature profile allowed to define the kinetic parameters corresponding to the best fit. The suggested simple quasi-homogeneous model describes experimental results (module temperature and outlet gas composition) with a good accuracy and could be used for process optimization and up-scaling.
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Zazhigalov S. V. et al. Simulation of diesel autothermal reforming over Rh/Ce0.75Zr0.25O2-δ-η-Al2O3/FeCrAl wire mesh honeycomb catalytic module // Chemical Engineering and Processing: Process Intensification. 2020. Vol. 150. p. 107876.
ГОСТ со всеми авторами (до 50) Скопировать
Zazhigalov S. V., Shilov V. A., RUBAN N., KULIKOV A., Zagoruiko A. N., Sobyanin V. A., Rogozhnikov V. N., Snytnikov P., Potemkin D., Simonov R. A. Simulation of diesel autothermal reforming over Rh/Ce0.75Zr0.25O2-δ-η-Al2O3/FeCrAl wire mesh honeycomb catalytic module // Chemical Engineering and Processing: Process Intensification. 2020. Vol. 150. p. 107876.
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TY - JOUR
DO - 10.1016/j.cep.2020.107876
UR - https://doi.org/10.1016/j.cep.2020.107876
TI - Simulation of diesel autothermal reforming over Rh/Ce0.75Zr0.25O2-δ-η-Al2O3/FeCrAl wire mesh honeycomb catalytic module
T2 - Chemical Engineering and Processing: Process Intensification
AU - Zazhigalov, S V
AU - Shilov, V. A.
AU - RUBAN, N.V.
AU - KULIKOV, A.V.
AU - Zagoruiko, A N
AU - Sobyanin, V. A.
AU - Rogozhnikov, V N
AU - Snytnikov, Pavel
AU - Potemkin, Dmitry
AU - Simonov, Ruslan A
PY - 2020
DA - 2020/04/01
PB - Elsevier
SP - 107876
VL - 150
SN - 0255-2701
SN - 1873-3204
ER -
BibTex
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@article{2020_Zazhigalov,
author = {S V Zazhigalov and V. A. Shilov and N.V. RUBAN and A.V. KULIKOV and A N Zagoruiko and V. A. Sobyanin and V N Rogozhnikov and Pavel Snytnikov and Dmitry Potemkin and Ruslan A Simonov},
title = {Simulation of diesel autothermal reforming over Rh/Ce0.75Zr0.25O2-δ-η-Al2O3/FeCrAl wire mesh honeycomb catalytic module},
journal = {Chemical Engineering and Processing: Process Intensification},
year = {2020},
volume = {150},
publisher = {Elsevier},
month = {apr},
url = {https://doi.org/10.1016/j.cep.2020.107876},
pages = {107876},
doi = {10.1016/j.cep.2020.107876}
}