Ceramics International, volume 45, issue 14, pages 17874-17883
Effect of dual doping on the structure and performance of garnet-type Li7La3Zr2O12 ceramic electrolytes for solid-state lithium-ion batteries
Publication type: Journal Article
Publication date: 2019-10-01
Journal:
Ceramics International
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 5.2
ISSN: 02728842
Materials Chemistry
Surfaces, Coatings and Films
Ceramics and Composites
Electronic, Optical and Magnetic Materials
Process Chemistry and Technology
Abstract
Nb–Gd co-doping Li7La3Zr2O12 electrolytes with compositions of Li7-x+yLa3Zr2-x-yNbxGdyO12 (x = 0.6; y = 0, 0.05, 0.10 and 0.20) were prepared via solid-state reaction. The X-ray diffraction (XRD) and Raman spectra demonstrated that all compositions exhibited a single cubic structure. Among these prepared samples, Li6.5La3Zr1.3Nb0.6Gd0.1O12 sample presented the lithium-ion conductivity of 9.86 × 10−4 S cm−1 when sintered at 1150 °C for 12 h. Meanwhile, bending strength and compressive strength reached 131 and 280.8 MPa, respectively. Further investigations were performed on the chemical and electrochemical properties of Li6.5La3Zr1.3Nb0.6Gd0.1O12. The XRD and cyclic voltammetry (CV) results showed that the ceramic sheet had excellent stability against metallic lithium and liquid electrolyte. A decrease in the interfacial resistance of Li/Li6.5La3Zr1.3Nb0.6Gd0.1O12, from 940 Ω cm2 to 178 Ω cm2, was observed. The full cells exhibited an initial discharge capacity of 138.5mAh g−1, and the capacity remained at 130.8mAh g−1 after 100 cycles.
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Luo Y. et al. Effect of dual doping on the structure and performance of garnet-type Li7La3Zr2O12 ceramic electrolytes for solid-state lithium-ion batteries // Ceramics International. 2019. Vol. 45. No. 14. pp. 17874-17883.
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Luo Y., Zhang Y., Zhang Q., Zheng Y., Chen H., Guo L. Effect of dual doping on the structure and performance of garnet-type Li7La3Zr2O12 ceramic electrolytes for solid-state lithium-ion batteries // Ceramics International. 2019. Vol. 45. No. 14. pp. 17874-17883.
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TY - JOUR
DO - 10.1016/j.ceramint.2019.06.002
UR - https://doi.org/10.1016/j.ceramint.2019.06.002
TI - Effect of dual doping on the structure and performance of garnet-type Li7La3Zr2O12 ceramic electrolytes for solid-state lithium-ion batteries
T2 - Ceramics International
AU - Luo, Yali
AU - Zhang, Yanli
AU - Zhang, Qixi
AU - Zheng, Yi-Feng
AU - Chen, Han
AU - Guo, Lucun
PY - 2019
DA - 2019/10/01 00:00:00
PB - Elsevier
SP - 17874-17883
IS - 14
VL - 45
SN - 0272-8842
ER -
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@article{2019_Luo,
author = {Yali Luo and Yanli Zhang and Qixi Zhang and Yi-Feng Zheng and Han Chen and Lucun Guo},
title = {Effect of dual doping on the structure and performance of garnet-type Li7La3Zr2O12 ceramic electrolytes for solid-state lithium-ion batteries},
journal = {Ceramics International},
year = {2019},
volume = {45},
publisher = {Elsevier},
month = {oct},
url = {https://doi.org/10.1016/j.ceramint.2019.06.002},
number = {14},
pages = {17874--17883},
doi = {10.1016/j.ceramint.2019.06.002}
}
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Luo, Yali, et al. “Effect of dual doping on the structure and performance of garnet-type Li7La3Zr2O12 ceramic electrolytes for solid-state lithium-ion batteries.” Ceramics International, vol. 45, no. 14, Oct. 2019, pp. 17874-17883. https://doi.org/10.1016/j.ceramint.2019.06.002.