Open Access
Chem, volume 4, issue 1, pages 174-185
Highly Fluorinated Interphases Enable High-Voltage Li-Metal Batteries
Xiulin Fan
1
,
Long Chen
1
,
Xiao Ji
1
,
Tao Deng
1
,
Singyuk Hou
1
,
Ji Jhong Chen
1
,
Jing Zheng
1
,
Fei Wang
1
,
Jianjun Jiang
2
,
Kang Xu
3
,
ChunSheng Wang
1
1
3
Electrochemistry Branch, Power and Energy Division Sensor and Electron Devices Directorate US Army Research Laboratory Adelphi MD 20783 USA
|
Publication type: Journal Article
Publication date: 2018-01-01
Materials Chemistry
General Chemistry
Biochemistry
General Chemical Engineering
Environmental Chemistry
Biochemistry (medical)
Abstract
Summary We were able to demonstrate excellent cycling performance of Li-metal anodes in carbonate electrolytes by increasing the Li bis(fluorosulfonyl)imide (LiFSI) concentration to ∼10 M. The high concentration (10 M) of FSI anion enabled interphases of high F content on both Li-metal anode and Ni-rich NMC (nickel-manganese-cobalt) cathode surfaces. Such F-rich interphases effectively suppressed Li dendrite formation, as demonstrated by a high Li plating/stripping Coulombic efficiency of ∼99.3%, and stabilized the carbonate molecules against oxidation at high cutoff voltages of 4.6 V on the surface of LiNi 0.6 Mn 0.2 Co 0.2 O 2 (NMC622). The combination of unique stabilization on both Li-metal anode and NMC622 cathodes enabled high-energy Li-metal batteries constructed on the aggressive chemistry. Under the harsh conditions of a high charge voltage of 4.6 V and high loading of 2.5 mAh/cm 2 , the NMC622||Li cells retained ∼86% of their original capacity after 100 cycles. The electrolyte strategy presented here offers unique guidelines for further optimizing beyond Li-ion chemistries.
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Citations by publishers
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Fan X. et al. Highly Fluorinated Interphases Enable High-Voltage Li-Metal Batteries // Chem. 2018. Vol. 4. No. 1. pp. 174-185.
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Fan X., Chen L., Ji X., Deng T., Hou S., Chen J. J., Zheng J., Wang F., Jiang J., Xu K., Wang C. Highly Fluorinated Interphases Enable High-Voltage Li-Metal Batteries // Chem. 2018. Vol. 4. No. 1. pp. 174-185.
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TY - JOUR
DO - 10.1016/j.chempr.2017.10.017
UR - https://doi.org/10.1016/j.chempr.2017.10.017
TI - Highly Fluorinated Interphases Enable High-Voltage Li-Metal Batteries
T2 - Chem
AU - Fan, Xiulin
AU - Chen, Long
AU - Ji, Xiao
AU - Deng, Tao
AU - Hou, Singyuk
AU - Chen, Ji Jhong
AU - Zheng, Jing
AU - Wang, Fei
AU - Jiang, Jianjun
AU - Xu, Kang
AU - Wang, ChunSheng
PY - 2018
DA - 2018/01/01 00:00:00
PB - Elsevier
SP - 174-185
IS - 1
VL - 4
SN - 2451-9294
SN - 1925-6981
SN - 1925-699X
ER -
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@article{2018_Fan,
author = {Xiulin Fan and Long Chen and Xiao Ji and Tao Deng and Singyuk Hou and Ji Jhong Chen and Jing Zheng and Fei Wang and Jianjun Jiang and Kang Xu and ChunSheng Wang},
title = {Highly Fluorinated Interphases Enable High-Voltage Li-Metal Batteries},
journal = {Chem},
year = {2018},
volume = {4},
publisher = {Elsevier},
month = {jan},
url = {https://doi.org/10.1016/j.chempr.2017.10.017},
number = {1},
pages = {174--185},
doi = {10.1016/j.chempr.2017.10.017}
}
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Fan, Xiulin, et al. “Highly Fluorinated Interphases Enable High-Voltage Li-Metal Batteries.” Chem, vol. 4, no. 1, Jan. 2018, pp. 174-185. https://doi.org/10.1016/j.chempr.2017.10.017.