Corrosion Science, volume 211, pages 110829
Point Defect Model for the kinetics of oxide film growth on the surface of T91 steel in contact with lead–bismuth eutectic
Publication type: Journal Article
Publication date: 2023-02-01
General Chemistry
General Chemical Engineering
General Materials Science
Abstract
Point Defect Model (PDM) has been successfully employed for aqueous solutions to describe the rate of surface corrosion of structural materials. In this work, the adaptation of PDM for the case of lead-bismuth coolant is developed. The necessary modifications in the set of electrochemical reactions and in the model of electrostatic potential distribution in the oxide film are made. Parameters of the proposed model, PDM_PB, are optimized using the experimental data for T91 grade steel. The obtained adaptation of PDM shows applicability to the case of lead and lead-bismuth coolants which is of critical importance for the next-generation fast-neutron reactors. • A Point Defect Model for steel oxidation by a liquid metal coolant – lead/LBE. • A set of interfacial reactions specific to the case of liquid metal coolant. • Model of electrostatic potential distribution in the oxide layer. • Optimization of PDM parameters for T91 grade steel in contact with LBE. • Model verification via temperature dependence of oxidation kinetics.
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Kolotinskii D. A. et al. Point Defect Model for the kinetics of oxide film growth on the surface of T91 steel in contact with lead–bismuth eutectic // Corrosion Science. 2023. Vol. 211. p. 110829.
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Kolotinskii D. A., Nikolaev V. S., Stegailov V., Timofeev A. V. Point Defect Model for the kinetics of oxide film growth on the surface of T91 steel in contact with lead–bismuth eutectic // Corrosion Science. 2023. Vol. 211. p. 110829.
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TY - JOUR
DO - 10.1016/j.corsci.2022.110829
UR - https://doi.org/10.1016%2Fj.corsci.2022.110829
TI - Point Defect Model for the kinetics of oxide film growth on the surface of T91 steel in contact with lead–bismuth eutectic
T2 - Corrosion Science
AU - Kolotinskii, D A
AU - Nikolaev, V S
AU - Stegailov, Vladimir V.
AU - Timofeev, A. V.
PY - 2023
DA - 2023/02/01 00:00:00
PB - Elsevier
SP - 110829
VL - 211
SN - 0010-938X
ER -
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@article{2023_Kolotinskii,
author = {D A Kolotinskii and V S Nikolaev and Vladimir V. Stegailov and A. V. Timofeev},
title = {Point Defect Model for the kinetics of oxide film growth on the surface of T91 steel in contact with lead–bismuth eutectic},
journal = {Corrosion Science},
year = {2023},
volume = {211},
publisher = {Elsevier},
month = {feb},
url = {https://doi.org/10.1016%2Fj.corsci.2022.110829},
pages = {110829},
doi = {10.1016/j.corsci.2022.110829}
}