Current Opinion in Solid State and Materials Science, volume 24, issue 6, pages 100875
Toward design of cation transport in solid-state battery electrolytes: Structure-dynamics relationships
Publication type: Journal Article
Publication date: 2020-12-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 11
ISSN: 13590286
General Materials Science
Abstract
• Close experiment-computation coupling is needed to understand cation transport. • A combination of multiple descriptors is needed to predict ionic conductivity. • Tensile strain may slightly help transport; compressive strain usually hinders it. • Grain boundaries processing-structure tailoring strongly impacts cation transport. • Kinetic stabilization is the next step to widen the electrochemical stability window. Cation-conducting, solid-state electrolytes represent a burgeoning focus of battery research, offering the potential for enhanced safety profiles, durability, and wide electrochemical stability windows for high energy density. In this review, we focus primarily on the Li/Na ion conductivity as one of the requirements and limiting factors in development of solid-state electrolytes and secondarily on stability. We highlight experimental and computational methods leading to the current state of understanding of solid-state cation transport, with the goal of drawing out structure-property relationships that lead to design strategies. Topics covered include: descriptors and high-throughput search methodologies including machine learning for identification of fast cation conductors; defect chemistry and its relationship to conduction mechanisms including emerging understanding of frustration, disorder, and concerted ion migration; the impact of strain on transport; factors determining stability; and the role of microstructure and extended defects. We conclude certain sections and the overall review with an outlook for the field, offering ideas for necessary research directions to address knowledge and property gaps.
Top-30
Citations by journals
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1 publication, 3.03%
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1 publication, 3.03%
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1 publication, 3.03%
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1 publication, 3.03%
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1 publication, 3.03%
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1 publication, 3.03%
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1 publication, 3.03%
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1 publication, 3.03%
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eScience
1 publication, 3.03%
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1 publication, 3.03%
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1 publication, 3.03%
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1 publication, 3.03%
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Citations by publishers
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Elsevier
11 publications, 33.33%
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American Chemical Society (ACS)
5 publications, 15.15%
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Royal Society of Chemistry (RSC)
5 publications, 15.15%
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Springer Nature
3 publications, 9.09%
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The Royal Society
2 publications, 6.06%
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Wiley
2 publications, 6.06%
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Frontiers Media S.A.
1 publication, 3.03%
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American Physical Society (APS)
1 publication, 3.03%
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 3.03%
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University of Novi Sad
1 publication, 3.03%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 3.03%
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12
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Lin Yu. et al. Toward design of cation transport in solid-state battery electrolytes: Structure-dynamics relationships // Current Opinion in Solid State and Materials Science. 2020. Vol. 24. No. 6. p. 100875.
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Lin Yu., Yong A. X. B., Gustafson W. I., Reedy C. N., Ertekin E., Krogstad J. A., Perry N. H. Toward design of cation transport in solid-state battery electrolytes: Structure-dynamics relationships // Current Opinion in Solid State and Materials Science. 2020. Vol. 24. No. 6. p. 100875.
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TY - JOUR
DO - 10.1016/j.cossms.2020.100875
UR - https://doi.org/10.1016/j.cossms.2020.100875
TI - Toward design of cation transport in solid-state battery electrolytes: Structure-dynamics relationships
T2 - Current Opinion in Solid State and Materials Science
AU - Lin, Yu
AU - Yong, Adrian Xiao Bin
AU - Gustafson, William I.
AU - Reedy, Colin N
AU - Ertekin, Elif
AU - Krogstad, Jessica A
AU - Perry, Nicola H.
PY - 2020
DA - 2020/12/01 00:00:00
PB - Elsevier
SP - 100875
IS - 6
VL - 24
SN - 1359-0286
ER -
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@article{2020_Lin,
author = {Yu Lin and Adrian Xiao Bin Yong and William I. Gustafson and Colin N Reedy and Elif Ertekin and Jessica A Krogstad and Nicola H. Perry},
title = {Toward design of cation transport in solid-state battery electrolytes: Structure-dynamics relationships},
journal = {Current Opinion in Solid State and Materials Science},
year = {2020},
volume = {24},
publisher = {Elsevier},
month = {dec},
url = {https://doi.org/10.1016/j.cossms.2020.100875},
number = {6},
pages = {100875},
doi = {10.1016/j.cossms.2020.100875}
}
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MLA
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Lin, Yu., et al. “Toward design of cation transport in solid-state battery electrolytes: Structure-dynamics relationships.” Current Opinion in Solid State and Materials Science, vol. 24, no. 6, Dec. 2020, p. 100875. https://doi.org/10.1016/j.cossms.2020.100875.