Significant enhancement of light-harvesting efficiency through the formation of [2]pseudorotaxane with γ-cyclodextrin based on a bolaamphiphile of salicylaldehyde azine moiety
Zhe-Xiong Lian
1
,
Man Jiang
2
,
Fei Qiao
1
,
Zhao Yuan
1
,
Meng Ning Chen
1
,
Rong-Zhou Wang
1
,
Tian Zhang
1
,
Liping Xu
1
,
Yan Hui
3
,
Shuping Zhuo
1
,
Publication type: Journal Article
Publication date: 2019-03-01
scimago Q2
wos Q1
SJR: 0.680
CiteScore: 8.5
Impact factor: 4.2
ISSN: 01437208, 18733743
General Chemical Engineering
Process Chemistry and Technology
Abstract
In this work, we have designed and synthesized a bolaamphiphile of salicylaldehyde azine (BSA), which can form [2]pseudorotaxane with γ-cyclodextrin (BSA@γ-CD) in aqueous solution and exhibit remarkable enhancement of the fluorescence emission. Both BSA and BSA@γ-CD assembly can spontaneously form spherical aggregates in aqueous solution with diameter at about 30 nm and 20 nm, respectively. By using BSA and BSA@γ-CD as energy donor and sulforhodamine 101 (SR101) as energy acceptor, we fabricated two artificial light-harvesting systems in aqueous solution. Significantly, an efficient energy transfer process was revealed to occur between the BSA or BSA@γ-CD assembly and the loaded SR101 to obtain high energy transfer efficiency and antenna effect. More importantly, energy transfer efficiency and antenna effect can be greatly improved in these two systems only just by addition of γ-CD.
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Total citations:
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Citations from 2024:
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(17.65%)
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GOST
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Lian Z. et al. Significant enhancement of light-harvesting efficiency through the formation of [2]pseudorotaxane with γ-cyclodextrin based on a bolaamphiphile of salicylaldehyde azine moiety // Dyes and Pigments. 2019. Vol. 162. pp. 475-480.
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Lian Z., Jiang M., Qiao F., Yuan Z., Chen M. N., Wang R., Zhang T., Xu L., Hui Y., Zhuo S., Xing L. Significant enhancement of light-harvesting efficiency through the formation of [2]pseudorotaxane with γ-cyclodextrin based on a bolaamphiphile of salicylaldehyde azine moiety // Dyes and Pigments. 2019. Vol. 162. pp. 475-480.
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TY - JOUR
DO - 10.1016/j.dyepig.2018.10.062
UR - https://doi.org/10.1016/j.dyepig.2018.10.062
TI - Significant enhancement of light-harvesting efficiency through the formation of [2]pseudorotaxane with γ-cyclodextrin based on a bolaamphiphile of salicylaldehyde azine moiety
T2 - Dyes and Pigments
AU - Lian, Zhe-Xiong
AU - Jiang, Man
AU - Qiao, Fei
AU - Yuan, Zhao
AU - Chen, Meng Ning
AU - Wang, Rong-Zhou
AU - Zhang, Tian
AU - Xu, Liping
AU - Hui, Yan
AU - Zhuo, Shuping
AU - Xing, Ling-Bao
PY - 2019
DA - 2019/03/01
PB - Elsevier
SP - 475-480
VL - 162
SN - 0143-7208
SN - 1873-3743
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2019_Lian,
author = {Zhe-Xiong Lian and Man Jiang and Fei Qiao and Zhao Yuan and Meng Ning Chen and Rong-Zhou Wang and Tian Zhang and Liping Xu and Yan Hui and Shuping Zhuo and Ling-Bao Xing},
title = {Significant enhancement of light-harvesting efficiency through the formation of [2]pseudorotaxane with γ-cyclodextrin based on a bolaamphiphile of salicylaldehyde azine moiety},
journal = {Dyes and Pigments},
year = {2019},
volume = {162},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016/j.dyepig.2018.10.062},
pages = {475--480},
doi = {10.1016/j.dyepig.2018.10.062}
}