Synthesis, characterization and application of meso-substituted fluorinated boron dipyrromethenes (BODIPYs) with different styryl groups in organic photovoltaic cells
Publication type: Journal Article
Publication date: 2019-09-01
scimago Q2
wos Q1
SJR: 0.680
CiteScore: 8.5
Impact factor: 4.2
ISSN: 01437208, 18733743
General Chemical Engineering
Process Chemistry and Technology
Abstract
A series of highly fluorinated BODIPY dyes with different styryl aromatic donor groups such as phenyl, naphthyl and anthracyl were designed, synthesized, characterized and applied as electron-donor materials in organic photovoltaic cells (OPV). The introduction of the styryl moieties leads to a large bathochromic shift and to a significant decrease in the HOMO-LUMO energy-gaps. All the BODIPY dyes showed relatively low HOMO energies ranging from −5.21 to −5.54 eV as determined from cyclic voltammetry measurements. Furthermore, they all show good solubility in organic solvents, thermal stability, excellent film-forming abilities which added with the great optoelectronics characteristics makes them excellent candidates as electron-donor materials for OPV cells. The power conversion efficiency (PCE) of the OPV based on the best BODIPY blend (BDP3/PC70BM (1:2, w/w) was 2.8% with a high open circuit voltage (VOC) of 1.00 V, which is a very promising PCE result for BODIPY based OPV and a top VOC value for this kind of systems.
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Total citations:
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Citations from 2024:
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Aguiar A. et al. Synthesis, characterization and application of meso-substituted fluorinated boron dipyrromethenes (BODIPYs) with different styryl groups in organic photovoltaic cells // Dyes and Pigments. 2019. Vol. 168. pp. 103-110.
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Aguiar A., Farinhas J., da Silva W. O., Ghica M., Brett C., Morgado J., SOBRAL A. J. F. N. Synthesis, characterization and application of meso-substituted fluorinated boron dipyrromethenes (BODIPYs) with different styryl groups in organic photovoltaic cells // Dyes and Pigments. 2019. Vol. 168. pp. 103-110.
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TY - JOUR
DO - 10.1016/j.dyepig.2019.04.031
UR - https://doi.org/10.1016/j.dyepig.2019.04.031
TI - Synthesis, characterization and application of meso-substituted fluorinated boron dipyrromethenes (BODIPYs) with different styryl groups in organic photovoltaic cells
T2 - Dyes and Pigments
AU - Aguiar, António
AU - Farinhas, Joana
AU - da Silva, Wanderson Oliveira
AU - Ghica, Mariana
AU - Brett, Christopher
AU - Morgado, J.M.
AU - SOBRAL, ABÍLIO J. F. N.
PY - 2019
DA - 2019/09/01
PB - Elsevier
SP - 103-110
VL - 168
SN - 0143-7208
SN - 1873-3743
ER -
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@article{2019_Aguiar,
author = {António Aguiar and Joana Farinhas and Wanderson Oliveira da Silva and Mariana Ghica and Christopher Brett and J.M. Morgado and ABÍLIO J. F. N. SOBRAL},
title = {Synthesis, characterization and application of meso-substituted fluorinated boron dipyrromethenes (BODIPYs) with different styryl groups in organic photovoltaic cells},
journal = {Dyes and Pigments},
year = {2019},
volume = {168},
publisher = {Elsevier},
month = {sep},
url = {https://doi.org/10.1016/j.dyepig.2019.04.031},
pages = {103--110},
doi = {10.1016/j.dyepig.2019.04.031}
}