Electrochimica Acta, volume 253, pages 430-438

Electrochemical performance of all-solid-state lithium batteries using inorganic lithium garnets particulate reinforced PEO/LiClO4 electrolyte

Samson Ho Sum Cheng ^{1, 2, 3, 4}

Kang‐Qiang He ^{5, 6}

Ying Liu ⁵

Md. Kamruzzaman ^{1, 2, 3, 4}

Robin L W Ma ⁷

Zhi-min Dang ⁸

R. Li ^{1, 2, 3, 4}

C K Chung ^{1, 2, 3, 4}

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CHINA |

Hong Kong |

CITY UNIVERSITY OF HONG KONG |

⁴

Department of Physics and Materials Science

⁵

Department of Physics and Materials Science, City University of Hong Kong, Hong Kong, China |

⁶

School of Chemistry and Biological Engineering, University of Science and Technology Beijing, Beijing 100083, PR China |

⁷

§Department of Mechanical and Aerospace Engineering, The Hong Kong University of Science and Technology, Hong Kong, China. |

⁸

State Key Laboratory of Power System, Department of Electrical Engineering, Tsinghua University, Beijing, 100084, PR China. |

Publication type: Journal Article

Publication date: 2017-11-01

Elsevier

Journal: Electrochimica Acta

Quartile SCImago

Quartile WOS

Impact factor: 6.6

ISSN: 00134686

DOI: 10.1016/j.electacta.2017.08.162

Copy DOI

General Chemical Engineering

Electrochemistry

Abstract

All-solid-state batteries are proposed to have ultimate safety and higher power and energy densities over conventional lithium ion batteries with liquid electrolytes. The Li ion conductivity and interfacial resistance between electrolyte and electrodes are the major bottleneck of the development of all-solid-state batteries for practical uses. Here, we reported a novel composite electrolyte which is composed of uniform distributed Li ion conducting Li6.4La3Zr1.4Ta0.6O12 (LLZTO) fillers in PEO/LiClO4 matrix. The EO:Li+ ratio of 15:1 is being used to achieve lower interfacial resistance between electrolyte and electrodes through the melting process. The composite electrolyte is fabricated by simple solution casting method, which is more advantageous comparing with high temperature sintering or sol-gel method used in the fabrication of ceramic electrolytes. The composite electrolyte exhibits good Li ion conductivity of 4.8 × 10−4 Scm−1 at 60 °C and excellent interfacial stability against Li metal. The all-solid-state lithium battery using this composite electrolyte shows a specific capacity of 140mAhg−1 and an unprecedentedly high capacity retention of 83% after 500 cycles at 60 °C and the rate of 1C. It is concluded that good electrode/electrolyte interfacial stability and contact as well as fast Li ion conductivity obtained by the addition of active garnet particulates to PEO/LiClO4 matrix are essential criteria for good charge/discharge performance of all-solid-state lithium batteries.

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Citations by journals

	1 2 3 4 5 6 7
ACS Applied Energy Materials	ACS Applied Energy Materials, 7, 5.19% ACS Applied Energy Materials 7 publications, 5.19%
Energy Storage Materials	Energy Storage Materials, 6, 4.44% Energy Storage Materials 6 publications, 4.44%
Electrochimica Acta	Electrochimica Acta, 6, 4.44% Electrochimica Acta 6 publications, 4.44%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 6, 4.44% Journal of Materials Chemistry A 6 publications, 4.44%
ACS applied materials & interfaces	ACS applied materials & interfaces, 5, 3.7% ACS applied materials & interfaces 5 publications, 3.7%
Journal of Energy Chemistry	Journal of Energy Chemistry, 4, 2.96% Journal of Energy Chemistry 4 publications, 2.96%
Journal of Power Sources	Journal of Power Sources, 4, 2.96% Journal of Power Sources 4 publications, 2.96%
Solid State Ionics	Solid State Ionics, 4, 2.96% Solid State Ionics 4 publications, 2.96%
Nano Energy	Nano Energy, 4, 2.96% Nano Energy 4 publications, 2.96%
Batteries	Batteries, 3, 2.22% Batteries 3 publications, 2.22%
Ionics	Ionics, 3, 2.22% Ionics 3 publications, 2.22%
Batteries & Supercaps	Batteries & Supercaps, 2, 1.48% Batteries & Supercaps 2 publications, 1.48%
Materials	Materials, 2, 1.48% Materials 2 publications, 1.48%
Science China Materials	Science China Materials, 2, 1.48% Science China Materials 2 publications, 1.48%
Composites Science and Technology	Composites Science and Technology, 2, 1.48% Composites Science and Technology 2 publications, 1.48%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 1.48% Chemical Engineering Journal 2 publications, 1.48%
Journal of Membrane Science	Journal of Membrane Science, 2, 1.48% Journal of Membrane Science 2 publications, 1.48%
ChemSusChem	ChemSusChem, 2, 1.48% ChemSusChem 2 publications, 1.48%
Advanced Materials	Advanced Materials, 2, 1.48% Advanced Materials 2 publications, 1.48%
Advanced Science	Advanced Science, 2, 1.48% Advanced Science 2 publications, 1.48%
International Journal of Energy Research	International Journal of Energy Research, 2, 1.48% International Journal of Energy Research 2 publications, 1.48%
Angewandte Chemie	Angewandte Chemie, 2, 1.48% Angewandte Chemie 2 publications, 1.48%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 2, 1.48% Angewandte Chemie - International Edition 2 publications, 1.48%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 2, 1.48% Journal of Physical Chemistry C 2 publications, 1.48%
Chemistry of Materials	Chemistry of Materials, 2, 1.48% Chemistry of Materials 2 publications, 1.48%
Small	Small, 2, 1.48% Small 2 publications, 1.48%
Functional Materials Letters	Functional Materials Letters, 1, 0.74% Functional Materials Letters 1 publication, 0.74%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 1, 0.74% Journal of the Electrochemical Society 1 publication, 0.74%
Membranes	Membranes, 1, 0.74% Membranes 1 publication, 0.74%
	1 2 3 4 5 6 7

Citations by publishers

	5 10 15 20 25 30 35 40 45
Elsevier	Elsevier, 43, 31.85% Elsevier 43 publications, 31.85%
Wiley	Wiley, 25, 18.52% Wiley 25 publications, 18.52%
American Chemical Society (ACS)	American Chemical Society (ACS), 21, 15.56% American Chemical Society (ACS) 21 publications, 15.56%
Springer Nature	Springer Nature, 12, 8.89% Springer Nature 12 publications, 8.89%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 10, 7.41% Multidisciplinary Digital Publishing Institute (MDPI) 10 publications, 7.41%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 10, 7.41% Royal Society of Chemistry (RSC) 10 publications, 7.41%
Frontiers Media S.A.	Frontiers Media S.A., 2, 1.48% Frontiers Media S.A. 2 publications, 1.48%
Tsinghua University Press	Tsinghua University Press, 2, 1.48% Tsinghua University Press 2 publications, 1.48%
World Scientific	World Scientific, 1, 0.74% World Scientific 1 publication, 0.74%
The Electrochemical Society	The Electrochemical Society, 1, 0.74% The Electrochemical Society 1 publication, 0.74%
Materials Research Society	Materials Research Society, 1, 0.74% Materials Research Society 1 publication, 0.74%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 0.74% Korean Society of Industrial Engineering Chemistry 1 publication, 0.74%
Taylor & Francis	Taylor & Francis, 1, 0.74% Taylor & Francis 1 publication, 0.74%
Hindawi Limited	Hindawi Limited, 1, 0.74% Hindawi Limited 1 publication, 0.74%
Korean Ceramic Society	Korean Ceramic Society, 1, 0.74% Korean Ceramic Society 1 publication, 0.74%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.74% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.74%
	5 10 15 20 25 30 35 40 45

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Ho Sum Cheng S. et al. Electrochemical performance of all-solid-state lithium batteries using inorganic lithium garnets particulate reinforced PEO/LiClO4 electrolyte // Electrochimica Acta. 2017. Vol. 253. pp. 430-438.

GOST all authors (up to 50) Copy

Ho Sum Cheng S., He K., Liu Y., Kamruzzaman M., Ma R. L. W., Dang Z., Li R., Chung C. K. Electrochemical performance of all-solid-state lithium batteries using inorganic lithium garnets particulate reinforced PEO/LiClO4 electrolyte // Electrochimica Acta. 2017. Vol. 253. pp. 430-438.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1016/j.electacta.2017.08.162

UR - https://doi.org/10.1016/j.electacta.2017.08.162

TI - Electrochemical performance of all-solid-state lithium batteries using inorganic lithium garnets particulate reinforced PEO/LiClO4 electrolyte

T2 - Electrochimica Acta

AU - Ho Sum Cheng, Samson

AU - He, Kang‐Qiang

AU - Liu, Ying

AU - Dang, Zhi-min

AU - Kamruzzaman, Md.

AU - Ma, Robin L W

AU - Li, R.

AU - Chung, C K

PY - 2017

DA - 2017/11/01 00:00:00

PB - Elsevier

SP - 430-438

VL - 253

SN - 0013-4686

ER -

BibTex

Cite this

BibTex Copy

@article{2017_Ho Sum Cheng,

author = {Samson Ho Sum Cheng and Kang‐Qiang He and Ying Liu and Zhi-min Dang and Md. Kamruzzaman and Robin L W Ma and R. Li and C K Chung},

title = {Electrochemical performance of all-solid-state lithium batteries using inorganic lithium garnets particulate reinforced PEO/LiClO4 electrolyte},

journal = {Electrochimica Acta},

year = {2017},

volume = {253},

publisher = {Elsevier},

month = {nov},

url = {https://doi.org/10.1016/j.electacta.2017.08.162},

pages = {430--438},

doi = {10.1016/j.electacta.2017.08.162}

}

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Publisher

Elsevier

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Electrochimica Acta

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Quartile WOS

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6.6

ISSN

00134686 (Print)