Energy Storage Materials, volume 23, pages 306-313

Elastic and well-aligned ceramic LLZO nanofiber based electrolytes for solid-state lithium batteries

Yun Zhao ¹

Jianhua Yan ²

Weiping Cai ³

YIMEI LAI ³

Jun Song ⁴

Jianyong Yu ⁵

Yang Si ⁵

Hide authors affiliations Show authors affiliations: 5 affiliations

Key Laboratory of Textile Science and Technology of Ministry of Education, College of Textiles, Donghua University, Shanghai, 201620, China |

Key Laboratory of Textile Science & Technology of Ministry of Education, College of Textiles, Donghua University, Shanghai 201620, China. |

School of Textile Materials and Engineering, Wuyi University, Guangdong, 529020, China |

⁴

College of Materials Science and Engineering, Donghua University, Shanghai 201620 (China) |

⁵

Innovation Center for Textile Science and Technology Donghua University Shanghai 200051 China. |

Publication type: Journal Article

Publication date: 2019-12-01

Elsevier

Journal: Energy Storage Materials

Quartile SCImago

Quartile WOS

Impact factor: 20.4

ISSN: 24058297, 24058297

DOI: 10.1016/j.ensm.2019.04.043

Copy DOI

General Materials Science

Energy Engineering and Power Technology

Renewable Energy, Sustainability and the Environment

Abstract

Ceramic Li7La3Zr2O12 is one of the most attractive electrolyte materials for solid-state batteries due to its high ionic conductivity and chemical/thermal stability, but the battery performance is always limited by the high electrolyte-electrode interfacial resistances. Here, we have fabricated elastic solid electrolytes by filling ionic-conductive polymers into well-aligned Li6.4La3Zr2Al0.2O12 (LLZO) nanofiber films. Such electrolytes can provide fast and continuous ionic-transportation channels and thus exhibit a high ionic conductivity of 1.16 × 10−4 S cm−1 at 30 °C. Moreover, the elastic surfaces of the electrolytes can well conform to electrodes without separations to adapt volume changes of the electrodes during the repeated cycles, enabling a stable Li plating/stripping cycling over 700 h. Fabricated solid-state NCA//Li cells exhibit ultra-low internal resistances of 87 Ω and deliver large discharge capacities with high Coulombic efficiencies that are comparable with the liquid type batteries. The reported approach allows low-cost fabrication of solid electrolytes that possess high ionic conductivity for solid state batteries.

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Citations by journals

	1 2 3 4 5 6 7 8 9
Energy Storage Materials	Energy Storage Materials, 9, 5.84% Energy Storage Materials 9 publications, 5.84%
Chemical Engineering Journal	Chemical Engineering Journal, 8, 5.19% Chemical Engineering Journal 8 publications, 5.19%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 8, 5.19% Journal of Materials Chemistry A 8 publications, 5.19%
ACS applied materials & interfaces	ACS applied materials & interfaces, 7, 4.55% ACS applied materials & interfaces 7 publications, 4.55%
ACS Applied Energy Materials	ACS Applied Energy Materials, 6, 3.9% ACS Applied Energy Materials 6 publications, 3.9%
Small	Small, 4, 2.6% Small 4 publications, 2.6%
Journal of Energy Chemistry	Journal of Energy Chemistry, 4, 2.6% Journal of Energy Chemistry 4 publications, 2.6%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 4, 2.6% Journal of Alloys and Compounds 4 publications, 2.6%
Electrochimica Acta	Electrochimica Acta, 4, 2.6% Electrochimica Acta 4 publications, 2.6%
Journal of Power Sources	Journal of Power Sources, 4, 2.6% Journal of Power Sources 4 publications, 2.6%
Journal of Advanced Ceramics	Journal of Advanced Ceramics, 3, 1.95% Journal of Advanced Ceramics 3 publications, 1.95%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 3, 1.95% Journal of Colloid and Interface Science 3 publications, 1.95%
Advanced Science	Advanced Science, 3, 1.95% Advanced Science 3 publications, 1.95%
ACS Nano	ACS Nano, 3, 1.95% ACS Nano 3 publications, 1.95%
Nano-Micro Letters	Nano-Micro Letters, 2, 1.3% Nano-Micro Letters 2 publications, 1.3%
Journal of Electronic Materials	Journal of Electronic Materials, 2, 1.3% Journal of Electronic Materials 2 publications, 1.3%
Electrochemical Energy Reviews	Electrochemical Energy Reviews, 2, 1.3% Electrochemical Energy Reviews 2 publications, 1.3%
Applied Materials Today	Applied Materials Today, 2, 1.3% Applied Materials Today 2 publications, 1.3%
ChemNanoMat	ChemNanoMat, 2, 1.3% ChemNanoMat 2 publications, 1.3%
Advanced Functional Materials	Advanced Functional Materials, 2, 1.3% Advanced Functional Materials 2 publications, 1.3%
Nano Letters	Nano Letters, 2, 1.3% Nano Letters 2 publications, 1.3%
Materials Chemistry Frontiers	Materials Chemistry Frontiers, 2, 1.3% Materials Chemistry Frontiers 2 publications, 1.3%
Colloids and Surfaces A: Physicochemical and Engineering Aspects	Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2, 1.3% Colloids and Surfaces A: Physicochemical and Engineering Aspects 2 publications, 1.3%
Advanced Materials	Advanced Materials, 2, 1.3% Advanced Materials 2 publications, 1.3%
Chemical Reviews	Chemical Reviews, 1, 0.65% Chemical Reviews 1 publication, 0.65%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 1, 0.65% Journal of the Electrochemical Society 1 publication, 0.65%
Gels	Gels, 1, 0.65% Gels 1 publication, 0.65%
Fibers and Polymers	Fibers and Polymers, 1, 0.65% Fibers and Polymers 1 publication, 0.65%
Tungsten	Tungsten, 1, 0.65% Tungsten 1 publication, 0.65%
	1 2 3 4 5 6 7 8 9

Citations by publishers

	10 20 30 40 50 60
Elsevier	Elsevier, 60, 38.96% Elsevier 60 publications, 38.96%
Wiley	Wiley, 26, 16.88% Wiley 26 publications, 16.88%
American Chemical Society (ACS)	American Chemical Society (ACS), 24, 15.58% American Chemical Society (ACS) 24 publications, 15.58%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 13, 8.44% Royal Society of Chemistry (RSC) 13 publications, 8.44%
Springer Nature	Springer Nature, 11, 7.14% Springer Nature 11 publications, 7.14%
Tsinghua University Press	Tsinghua University Press, 3, 1.95% Tsinghua University Press 3 publications, 1.95%
The Electrochemical Society	The Electrochemical Society, 1, 0.65% The Electrochemical Society 1 publication, 0.65%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 0.65% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 0.65%
The Korean Fiber Society	The Korean Fiber Society, 1, 0.65% The Korean Fiber Society 1 publication, 0.65%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 0.65% Korean Society of Industrial Engineering Chemistry 1 publication, 0.65%
IOP Publishing	IOP Publishing, 1, 0.65% IOP Publishing 1 publication, 0.65%
Chinese Ceramic Society	Chinese Ceramic Society, 1, 0.65% Chinese Ceramic Society 1 publication, 0.65%
Taylor & Francis	Taylor & Francis, 1, 0.65% Taylor & Francis 1 publication, 0.65%
Electrochemical Science Group, University of Belgrade	Electrochemical Science Group, University of Belgrade, 1, 0.65% Electrochemical Science Group, University of Belgrade 1 publication, 0.65%
OAE Publishing Inc.	OAE Publishing Inc., 1, 0.65% OAE Publishing Inc. 1 publication, 0.65%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.65% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.65%
	10 20 30 40 50 60

We do not take into account publications without a DOI.
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Zhao Y. et al. Elastic and well-aligned ceramic LLZO nanofiber based electrolytes for solid-state lithium batteries // Energy Storage Materials. 2019. Vol. 23. pp. 306-313.

GOST all authors (up to 50) Copy

Zhao Y., Yan J., Cai W., LAI Y., Song J., Yu J., Si Y. Elastic and well-aligned ceramic LLZO nanofiber based electrolytes for solid-state lithium batteries // Energy Storage Materials. 2019. Vol. 23. pp. 306-313.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1016/j.ensm.2019.04.043

UR - https://doi.org/10.1016/j.ensm.2019.04.043

TI - Elastic and well-aligned ceramic LLZO nanofiber based electrolytes for solid-state lithium batteries

T2 - Energy Storage Materials

AU - Zhao, Yun

AU - Yan, Jianhua

AU - Cai, Weiping

AU - LAI, YIMEI

AU - Song, Jun

AU - Yu, Jianyong

AU - Si, Yang

PY - 2019

DA - 2019/12/01 00:00:00

PB - Elsevier

SP - 306-313

VL - 23

SN - 2405-8297

ER -

BibTex

Cite this

BibTex Copy

@article{2019_Zhao,

author = {Yun Zhao and Jianhua Yan and Weiping Cai and YIMEI LAI and Jun Song and Jianyong Yu and Yang Si},

title = {Elastic and well-aligned ceramic LLZO nanofiber based electrolytes for solid-state lithium batteries},

journal = {Energy Storage Materials},

year = {2019},

volume = {23},

publisher = {Elsevier},

month = {dec},

url = {https://doi.org/10.1016/j.ensm.2019.04.043},

pages = {306--313},

doi = {10.1016/j.ensm.2019.04.043}

}

Found error?

Publisher

Elsevier

Journal

Energy Storage Materials

Quartile SCImago

Quartile WOS

Impact factor

20.4

ISSN

24058297 (Electronic)
24058297 (Print)