Energy Storage Materials, volume 31, pages 267-273

Interfacial redox behaviors of sulfide electrolytes in fast-charging all-solid-state lithium metal batteries

Gao-Long Zhu ^{1, 2}

Chen-Zi Zhao ³

Hong Yuan ⁴

Bo Chen Zhao ³

Boquan Li ³

Xin-Bing Cheng ³

Hao Xiong Nan ^{1, 5}

Yang Lu ³

Jian Zhang ⁶

Jia-Qi Huang ⁴

Quan Bing Liu ⁷

Chuan Xin He ²

Qiang Zhang ³

Hide authors affiliations Show authors affiliations: 7 affiliations

Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing, 100084, China |

Shenzhen Key Laboratory of Functional Polymer, College of Chemistry and Chemical Engineering, Shenzhen University, Shenzhen, 518000, China |

Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical Engineering, Tsinghua University, Beijing, 100084, China. |

⁴

Advanced Research Institute of Multidisciplinary Science Beijing Institute of Technology Beijing 100081 China |

⁵

School of Chemical Engineering and Light Industry Guangdong University of Technology Guangzhou 510006 China |

⁶

AAC Technologies Holdings Inc., Nanjing, 10093, China |

⁷

School of Chemical Engineering and Light Industry Guangdong University of Technology Guangzhou 510006 China |

Publication type: Journal Article

Publication date: 2020-10-01

Elsevier

Journal: Energy Storage Materials

Quartile SCImago

Quartile WOS

Impact factor: 20.4

ISSN: 24058297, 24058297

DOI: 10.1016/j.ensm.2020.05.017

Copy DOI

General Materials Science

Energy Engineering and Power Technology

Renewable Energy, Sustainability and the Environment

Abstract

Sulfide solid electrolytes offer great opportunities to construct solid-state Li metal batteries with high energy density. The high ionic conductivity of well-developed sulfide electrolytes enables solid-state battery to operate at high current rates. However, sulfide electrolytes exhibit severe decomposition in working cells, constituting a significant obstacle for the practical applications of sulfide solid-state electrolytes. The decomposition behaviors of sulfides are complicated and strongly depend on the electrochemical windows, some of which are even regarded reversible during battery cycling. Herein, we investigate the redox behaviors of Li7P3S11 sulfide solid electrolyte under different voltage windows, and their effects on interfacial transport and battery cycle lifetime. Moreover, Li metal | Li4Ti5O12 (LTO) batteries are introduced to further probe the role of multiphase redox reactions on interfacial ion conduction. By regulating the redox behaviors of electrolytes through varying working voltage window, Li | LTO metal batteries enable a rapid charge/discharge process in 10 min (6 C) and lifespan of 600 cycles at 1 C with 85% capacity retention. An all-solid-state Li | LTO metal pouch cell is also assembled and exhibits a stable cycling performance with a capacity of 120 mAh g−1. This work provides understandings about interfacial redox behaviors of sulfide electrolyte, presenting novel insights in the rational design of future solid-state lithium batteries with high-energy/power-density.

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Solid State Ionics	Solid State Ionics, 1, 1.85% Solid State Ionics 1 publication, 1.85%
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Elsevier	Elsevier, 26, 48.15% Elsevier 26 publications, 48.15%
Wiley	Wiley, 15, 27.78% Wiley 15 publications, 27.78%
American Chemical Society (ACS)	American Chemical Society (ACS), 5, 9.26% American Chemical Society (ACS) 5 publications, 9.26%
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IOP Publishing	IOP Publishing, 1, 1.85% IOP Publishing 1 publication, 1.85%
Chemical Industry Press	Chemical Industry Press, 1, 1.85% Chemical Industry Press 1 publication, 1.85%
Springer Nature	Springer Nature, 1, 1.85% Springer Nature 1 publication, 1.85%
Chinese Academy of Sciences	Chinese Academy of Sciences, 1, 1.85% Chinese Academy of Sciences 1 publication, 1.85%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.85% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.85%
	5 10 15 20 25 30

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Zhu G. et al. Interfacial redox behaviors of sulfide electrolytes in fast-charging all-solid-state lithium metal batteries // Energy Storage Materials. 2020. Vol. 31. pp. 267-273.

GOST all authors (up to 50) Copy

Zhu G., Zhao C., Yuan H., Zhao B. C., Li B., Cheng X., Nan H. X., Lu Y., Zhang J., Huang J., Liu Q. B., He C. X., Zhang Q. Interfacial redox behaviors of sulfide electrolytes in fast-charging all-solid-state lithium metal batteries // Energy Storage Materials. 2020. Vol. 31. pp. 267-273.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.ensm.2020.05.017

UR - https://doi.org/10.1016/j.ensm.2020.05.017

TI - Interfacial redox behaviors of sulfide electrolytes in fast-charging all-solid-state lithium metal batteries

T2 - Energy Storage Materials

AU - Zhu, Gao-Long

AU - Zhao, Chen-Zi

AU - Yuan, Hong

AU - Zhao, Bo Chen

AU - Li, Boquan

AU - Cheng, Xin-Bing

AU - Nan, Hao Xiong

AU - Lu, Yang

AU - Zhang, Jian

AU - Huang, Jia-Qi

AU - Liu, Quan Bing

AU - He, Chuan Xin

AU - Zhang, Qiang

PY - 2020

DA - 2020/10/01 00:00:00

PB - Elsevier

SP - 267-273

VL - 31

SN - 2405-8297

ER -

BibTex

Cite this

BibTex Copy

@article{2020_Zhu,

author = {Gao-Long Zhu and Chen-Zi Zhao and Hong Yuan and Bo Chen Zhao and Boquan Li and Xin-Bing Cheng and Hao Xiong Nan and Yang Lu and Jian Zhang and Jia-Qi Huang and Quan Bing Liu and Chuan Xin He and Qiang Zhang},

title = {Interfacial redox behaviors of sulfide electrolytes in fast-charging all-solid-state lithium metal batteries},

journal = {Energy Storage Materials},

year = {2020},

volume = {31},

publisher = {Elsevier},

month = {oct},

url = {https://doi.org/10.1016/j.ensm.2020.05.017},

pages = {267--273},

doi = {10.1016/j.ensm.2020.05.017}

}

Found error?

Publisher

Elsevier

Journal

Energy Storage Materials

Quartile SCImago

Quartile WOS

Impact factor

20.4

ISSN

24058297 (Electronic)
24058297 (Print)