Energy Storage Materials, volume 38, pages 157-189

Design of safe, long-cycling and high-energy lithium metal anodes in all working conditions: Progress, challenges and perspectives

Chuanliang Wei
Yuchan Zhang
Yuan Tian
Liwen Tan
Yongling An
Yi Qian
Baojuan Xi
Shenglin Xiong
Jinkui Feng
Yitai Qian
Publication typeJournal Article
Publication date2021-06-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor20.4
ISSN24058297, 24058297
General Materials Science
Energy Engineering and Power Technology
Renewable Energy, Sustainability and the Environment
Abstract
Lithium (Li) metal is a “superstar” among all the anode materials for lithium-ion batteries (LIBs) owing to its low electrochemical potential, high theoretical specific capacity, low density, etc. The inherent issues of Li-metal anodes including high chemical activity, uncontrollable growth of Li dendrites, large volume changes, and unstable solid electrolyte interphase (SEI) have been gradually improved in the past several years. However, most of the previous study on Li-metal anodes is performed at room temperature under inert atmosphere. The stability and behavior of Li-metal anode in extreme conditions such as air, water, and high/low temperatures are easy to be ignored. Improving the stability of Li-metal anodes in extreme conditions is meaningful for constructing safe, long-cycling, low-cost, and high-energy Li-metal batteries in all working conditions. Tremendous work has been conducted to enable stable Li-metal anodes in extreme conditions recently. Here we carefully present a review for stable Li-metal anodes in extreme conditions. The backgrounds of Li-metal anodes and strategies for achieving stable Li-metal anodes in extreme conditions are carefully summarized. Meanwhile, we proposed some outlooks and perspectives. We hope this review can make more researchers pay attention to Li-metal anodes in extreme conditions.

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Wei C. et al. Design of safe, long-cycling and high-energy lithium metal anodes in all working conditions: Progress, challenges and perspectives // Energy Storage Materials. 2021. Vol. 38. pp. 157-189.
GOST all authors (up to 50) Copy
Wei C., Zhang Y., Tian Y., Tan L., An Y., Qian Y., Xi B., Xiong S., Feng J., Qian Y. Design of safe, long-cycling and high-energy lithium metal anodes in all working conditions: Progress, challenges and perspectives // Energy Storage Materials. 2021. Vol. 38. pp. 157-189.
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RIS Copy
TY - JOUR
DO - 10.1016/j.ensm.2021.03.006
UR - https://doi.org/10.1016/j.ensm.2021.03.006
TI - Design of safe, long-cycling and high-energy lithium metal anodes in all working conditions: Progress, challenges and perspectives
T2 - Energy Storage Materials
AU - Wei, Chuanliang
AU - Zhang, Yuchan
AU - Tian, Yuan
AU - Tan, Liwen
AU - An, Yongling
AU - Qian, Yi
AU - Xi, Baojuan
AU - Xiong, Shenglin
AU - Feng, Jinkui
AU - Qian, Yitai
PY - 2021
DA - 2021/06/01 00:00:00
PB - Elsevier
SP - 157-189
VL - 38
SN - 2405-8297
SN - 2405-8297
ER -
BibTex
Cite this
BibTex Copy
@article{2021_Wei,
author = {Chuanliang Wei and Yuchan Zhang and Yuan Tian and Liwen Tan and Yongling An and Yi Qian and Baojuan Xi and Shenglin Xiong and Jinkui Feng and Yitai Qian},
title = {Design of safe, long-cycling and high-energy lithium metal anodes in all working conditions: Progress, challenges and perspectives},
journal = {Energy Storage Materials},
year = {2021},
volume = {38},
publisher = {Elsevier},
month = {jun},
url = {https://doi.org/10.1016/j.ensm.2021.03.006},
pages = {157--189},
doi = {10.1016/j.ensm.2021.03.006}
}
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