Energy Storage Materials, volume 47, pages 262-270

A 3D interconnected metal-organic framework-derived solid-state electrolyte for dendrite-free lithium metal battery

Zhongliang Li

Zhong-Liang Li ¹

Shuxian Wang ¹

Junkai Shi Junkai

Junkai Shi ¹

Yang Liu ¹

Yang Liu

Siyan Zheng ¹

Hanqin Zou ¹

Yilin Chen ¹

Wenxi Kuang ¹

Kui Ding ¹

Luyi Chen ¹

Ya-Qian Lan ¹

Yue-Peng Cai ¹

Qifeng Zheng ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

School of Chemistry, South China Normal University, 55 West Zhongsan Rd., Guangzhou 510006, Guangdong, China |

Publication type: Journal Article

Publication date: 2022-05-01

Elsevier

Journal: Energy Storage Materials

Quartile SCImago

Quartile WOS

Impact factor: 20.4

ISSN: 24058297, 24058297

DOI: 10.1016/j.ensm.2022.02.014

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General Materials Science

Energy Engineering and Power Technology

Renewable Energy, Sustainability and the Environment

Abstract

• A 3D interconnected metal-organic framework (MOF)-derived solid-state electrolyte (SSE) without any liquid was rationally designed. • The SSE exhibited high ionic conductivity, high Li + transference number, wide potential window, excellent interfacial compatibility, and outstanding ability to inhibit the growth of lithium dendrites. • The Li||Li symmetric cell using 3D interconnected MOF-derived SSE can be stably operated for more than 700 h. • The all-solid-state lithium-metal full cell fabricated with 3D interconnected MOF-derived SSE exhibited superior cycling performance even with a 20 µm thin Li anode. The urgent need for high-energy and high-safety batteries is leading research to all-solid-state lithium-metal batteries. However, achieving high ionic conductivities, homogenous Li + flux, excellent interfacial compatibility, as well as enhanced mechanical strength simultaneously still remain a serious challenge for solid-state electrolyte (SSE). Herein, we rationally develop a three-dimensional (3D) interconnected metal-organic framework (MOF) network-based SSE without any liquid, where the MOF with optimized pore size and strong cationic site is able to restrict anions transport to afford a homogeneous Li + flux and a high Li + transference number (0.52). Furthermore, the 3D interconnected MOF-based networks not only build continuous ion conductive pathways for fast Li + transport (ionic conductivity of 2.89 × 10 −4 S cm −1 ), but also provide structural reinforcement to enhance the mechanical strength (Young's modulus of 819.4 MPa). Consequently, the Li||Li symmetric cell using 3D interconnected MOF-derived SSE can be stably operated for more than 700 h. The all-solid-state lithium-metal full cells fabricated with 3D interconnected MOF-derived SSE exhibit excellent cycling performance even with a 20 µm thin Li anode or high-voltage cathode. A 3D interconnected metal-organic framework (MOF)-derived solid-state electrolyte without any liquid was developed to enable the stable operation of Li||Li, 20 µm thin Li||LiFePO 4 , and high voltage Li||LiNi 1/3 Mn 1/3 Co 1/3 O 2 cells. Rationally, the optimized MOF affords a homogeneous Li + flux, the interconnected MOF-based nanofiber builds continuous pathways for fast Li + transport, and 3D nanofiber network provides structural reinforcement to enhance the mechanical strength.

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Chemical Engineering Journal	Chemical Engineering Journal, 5, 5.38% Chemical Engineering Journal 5 publications, 5.38%
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Electrochimica Acta	Electrochimica Acta, 3, 3.23% Electrochimica Acta 3 publications, 3.23%
ACS applied materials & interfaces	ACS applied materials & interfaces, 3, 3.23% ACS applied materials & interfaces 3 publications, 3.23%
Advanced Science	Advanced Science, 2, 2.15% Advanced Science 2 publications, 2.15%
Nano-Micro Letters	Nano-Micro Letters, 2, 2.15% Nano-Micro Letters 2 publications, 2.15%
Batteries & Supercaps	Batteries & Supercaps, 2, 2.15% Batteries & Supercaps 2 publications, 2.15%
Energy & Environmental Materials	Energy & Environmental Materials, 2, 2.15% Energy & Environmental Materials 2 publications, 2.15%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 2, 2.15% Journal of Materials Chemistry A 2 publications, 2.15%
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Angewandte Chemie	Angewandte Chemie, 2, 2.15% Angewandte Chemie 2 publications, 2.15%
ACS Nano	ACS Nano, 2, 2.15% ACS Nano 2 publications, 2.15%
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Chemical Reviews	Chemical Reviews, 1, 1.08% Chemical Reviews 1 publication, 1.08%
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ACS Materials Letters	ACS Materials Letters, 1, 1.08% ACS Materials Letters 1 publication, 1.08%
EnergyChem	EnergyChem, 1, 1.08% EnergyChem 1 publication, 1.08%
Materials Today Energy	Materials Today Energy, 1, 1.08% Materials Today Energy 1 publication, 1.08%
Chinese Journal of Chemical Engineering	Chinese Journal of Chemical Engineering, 1, 1.08% Chinese Journal of Chemical Engineering 1 publication, 1.08%
International Journal of Mechanical Sciences	International Journal of Mechanical Sciences, 1, 1.08% International Journal of Mechanical Sciences 1 publication, 1.08%
	1 2 3 4 5

Citations by publishers

	5 10 15 20 25 30 35
Elsevier	Elsevier, 35, 37.63% Elsevier 35 publications, 37.63%
Wiley	Wiley, 25, 26.88% Wiley 25 publications, 26.88%
American Chemical Society (ACS)	American Chemical Society (ACS), 12, 12.9% American Chemical Society (ACS) 12 publications, 12.9%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 8, 8.6% Royal Society of Chemistry (RSC) 8 publications, 8.6%
Springer Nature	Springer Nature, 6, 6.45% Springer Nature 6 publications, 6.45%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 3.23% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 3.23%
Chemical Industry Press	Chemical Industry Press, 1, 1.08% Chemical Industry Press 1 publication, 1.08%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 1.08% American Association for the Advancement of Science (AAAS) 1 publication, 1.08%
IOP Publishing	IOP Publishing, 1, 1.08% IOP Publishing 1 publication, 1.08%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.08% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.08%
	5 10 15 20 25 30 35

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Li Z. et al. A 3D interconnected metal-organic framework-derived solid-state electrolyte for dendrite-free lithium metal battery // Energy Storage Materials. 2022. Vol. 47. pp. 262-270.

GOST all authors (up to 50) Copy

Li Z., Li Z., Wang S., Shi Junkai J., Shi J., Liu Y., Liu Y., Zheng S., Zou H., Chen Y., Kuang W., Ding K., Chen L., Lan Y., Cai Y., Zheng Q. A 3D interconnected metal-organic framework-derived solid-state electrolyte for dendrite-free lithium metal battery // Energy Storage Materials. 2022. Vol. 47. pp. 262-270.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1016/j.ensm.2022.02.014

UR - https://doi.org/10.1016/j.ensm.2022.02.014

TI - A 3D interconnected metal-organic framework-derived solid-state electrolyte for dendrite-free lithium metal battery

T2 - Energy Storage Materials

AU - Li, Zhongliang

AU - Shi Junkai, Junkai

AU - Liu, Yang

AU - Zheng, Siyan

AU - Zou, Hanqin

AU - Kuang, Wenxi

AU - Ding, Kui

AU - Chen, Luyi

AU - Zheng, Qifeng

AU - Li, Zhong-Liang

AU - Wang, Shuxian

AU - Shi, Junkai

AU - Liu, Yang

AU - Chen, Yilin

AU - Lan, Ya-Qian

AU - Cai, Yue-Peng

PY - 2022

DA - 2022/05/01 00:00:00

PB - Elsevier

SP - 262-270

VL - 47

SN - 2405-8297

ER -

BibTex

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BibTex Copy

@article{2022_Li,

author = {Zhongliang Li and Junkai Shi Junkai and Yang Liu and Siyan Zheng and Hanqin Zou and Wenxi Kuang and Kui Ding and Luyi Chen and Qifeng Zheng and Zhong-Liang Li and Shuxian Wang and Junkai Shi and Yang Liu and Yilin Chen and Ya-Qian Lan and Yue-Peng Cai},

title = {A 3D interconnected metal-organic framework-derived solid-state electrolyte for dendrite-free lithium metal battery},

journal = {Energy Storage Materials},

year = {2022},

volume = {47},

publisher = {Elsevier},

month = {may},

url = {https://doi.org/10.1016/j.ensm.2022.02.014},

pages = {262--270},

doi = {10.1016/j.ensm.2022.02.014}

}

Found error?

Publisher

Elsevier

Journal

Energy Storage Materials

Quartile SCImago

Quartile WOS

Impact factor

20.4

ISSN

24058297 (Electronic)
24058297 (Print)

Profiles

Lan, Ya-Qian P