Energy Storage Materials, volume 63, pages 103038

Challenges and strategies towards the interface between lithium anode and Li10GeP2S12 electrolyte in all-solid-state lithium metal batteries

Quan Zheng 1
Yi Song 1
Weixing Huang 1
Jie Yang 2
Tao Li 1
Ying Xu 1, 3
Publication typeJournal Article
Publication date2023-11-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor20.4
ISSN24058297, 24058297
General Materials Science
Energy Engineering and Power Technology
Renewable Energy, Sustainability and the Environment
Abstract
All-solid-state lithium (Li) metal batteries (ASLMBs) have attracted enormous attention due to the safety of solid-state electrolytes (SSEs) and the high energy density of Li metal. Among various SSEs, sulfide SSEs, especially the Li10GeP2S12 (LGPS), shows liquid electrolytes comparable conductivity at room temperature, thus being considered as one of the most promising candidates. However, the interfacial issues with Li have severely hindered the further development of the LGPS-based ASLMBs. Herein, we present the distinctive crystal structure and ion transport mechanism of LGPS at first. The origin of the interfacial issues with Li and the corresponding modification strategies are summarized then. Finally, combined with the present opportunities and challenges, perspectives are presented in the end for designing practically accessible LGPS-based ASLMBs in the future.

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Zheng Q. et al. Challenges and strategies towards the interface between lithium anode and Li10GeP2S12 electrolyte in all-solid-state lithium metal batteries // Energy Storage Materials. 2023. Vol. 63. p. 103038.
GOST all authors (up to 50) Copy
Zheng Q., Song Y., Huang W., Yang J., Li T., Xu Y. Challenges and strategies towards the interface between lithium anode and Li10GeP2S12 electrolyte in all-solid-state lithium metal batteries // Energy Storage Materials. 2023. Vol. 63. p. 103038.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1016/j.ensm.2023.103038
UR - https://doi.org/10.1016/j.ensm.2023.103038
TI - Challenges and strategies towards the interface between lithium anode and Li10GeP2S12 electrolyte in all-solid-state lithium metal batteries
T2 - Energy Storage Materials
AU - Zheng, Quan
AU - Song, Yi
AU - Huang, Weixing
AU - Yang, Jie
AU - Li, Tao
AU - Xu, Ying
PY - 2023
DA - 2023/11/01 00:00:00
PB - Elsevier
SP - 103038
VL - 63
SN - 2405-8297
SN - 2405-8297
ER -
BibTex
Cite this
BibTex Copy
@article{2023_Zheng,
author = {Quan Zheng and Yi Song and Weixing Huang and Jie Yang and Tao Li and Ying Xu},
title = {Challenges and strategies towards the interface between lithium anode and Li10GeP2S12 electrolyte in all-solid-state lithium metal batteries},
journal = {Energy Storage Materials},
year = {2023},
volume = {63},
publisher = {Elsevier},
month = {nov},
url = {https://doi.org/10.1016/j.ensm.2023.103038},
pages = {103038},
doi = {10.1016/j.ensm.2023.103038}
}
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