Palladium(II) complexes of (pyridyl)imine ligands as catalysts for the methoxycarbonylation of olefins
Publication type: Journal Article
Publication date: 2020-02-01
scimago Q3
wos Q2
SJR: 0.393
CiteScore: 5.5
Impact factor: 3.2
ISSN: 00201693, 18733255
Materials Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Reactions of 2-methoxy-N-((pyridin-2-yl)methylene)ethanamine (L1), 2-((pyridin-2-yl)methyleneamino)ethanol (L2) and 3-methoxy-N-((pyridin-2-yl)methylene)propan-1-amine (L3) ligands with either [PdCl2(COD)] or [PdCl(Me)(COD)] produced the corresponding monometallic complexes [PdCl2(L1)] (1), [PdClMe(L1)] (2), [PdCl2(L2)] (3) and [PdCl2(L3)] (4). The solid state structure of complex 1 confirmed the bidentate coordination mode of L1, giving a distorted square planar geometry. All the complexes (1–4) formed active catalysts for the methoxycarbonylation of higher olefins to give linear and branched esters. The catalytic behavior of complexes 1–4 were influenced by both the complex structure and olefin chain length.
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11
Total citations:
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Citations from 2025:
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(18.18%)
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Zulu Z. et al. Palladium(II) complexes of (pyridyl)imine ligands as catalysts for the methoxycarbonylation of olefins // Inorganica Chimica Acta. 2020. Vol. 501. p. 119270.
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Zulu Z., Nyamato G. S., Tshabalala T. A., Ojwach S. O. Palladium(II) complexes of (pyridyl)imine ligands as catalysts for the methoxycarbonylation of olefins // Inorganica Chimica Acta. 2020. Vol. 501. p. 119270.
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TY - JOUR
DO - 10.1016/j.ica.2019.119270
UR - https://doi.org/10.1016/j.ica.2019.119270
TI - Palladium(II) complexes of (pyridyl)imine ligands as catalysts for the methoxycarbonylation of olefins
T2 - Inorganica Chimica Acta
AU - Zulu, Zethu
AU - Nyamato, George S.
AU - Tshabalala, Thandeka A
AU - Ojwach, Stephen O.
PY - 2020
DA - 2020/02/01
PB - Elsevier
SP - 119270
VL - 501
SN - 0020-1693
SN - 1873-3255
ER -
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@article{2020_Zulu,
author = {Zethu Zulu and George S. Nyamato and Thandeka A Tshabalala and Stephen O. Ojwach},
title = {Palladium(II) complexes of (pyridyl)imine ligands as catalysts for the methoxycarbonylation of olefins},
journal = {Inorganica Chimica Acta},
year = {2020},
volume = {501},
publisher = {Elsevier},
month = {feb},
url = {https://doi.org/10.1016/j.ica.2019.119270},
pages = {119270},
doi = {10.1016/j.ica.2019.119270}
}