Effect of Co–Ni ratio on the activity and stability of Co–Ni bimetallic aerogel catalyst for methane Oxy-CO2 reforming
Тип публикации: Journal Article
Дата публикации: 2011-02-01
scimago Q1
wos Q1
БС1
SJR: 1.685
CiteScore: 13.3
Impact factor: 8.3
ISSN: 03603199, 18793487
Condensed Matter Physics
Energy Engineering and Power Technology
Fuel Technology
Renewable Energy, Sustainability and the Environment
Краткое описание
Co-Ni bimetallic aerogel catalysts with various Co/Ni ratios were synthesized by the sol gel method followed by the supercritical drying process. The catalysts were characterized by XRD, H-2-TPR, HRTEM, BET, TG and FESEM. It showed that the Co/Ni ratio influenced the micro-structure of the Co-Ni bimetallic aerogel catalysts. The formation of homogeneous metal alloy on the bimetallic catalysts was observed after the reduction. In addition, catalysts with higher Co/Ni ratios showed smaller active metal particle sizes. The activities of the aerogel catalysts in terms of CH4 conversion were found to be in the order of 5Co5Ni approximate to 3Co7Ni > 7Co3Ni > 10Ni >> 10Co. 5Co5Ni exhibited the highest CH4 conversion in methane Oxy-CO2 reforming, which is 16% and 55% greater than those of 10Ni and 10Co, respectively. The difference between the catalytic performances could mainly be attributed to the combined effect of the kinetics, the geometric and the SMSI effects. (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
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Chen L., Zhu Q., Wu R. Effect of Co–Ni ratio on the activity and stability of Co–Ni bimetallic aerogel catalyst for methane Oxy-CO2 reforming // International Journal of Hydrogen Energy. 2011. Vol. 36. No. 3. pp. 2128-2136.
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Chen L., Zhu Q., Wu R. Effect of Co–Ni ratio on the activity and stability of Co–Ni bimetallic aerogel catalyst for methane Oxy-CO2 reforming // International Journal of Hydrogen Energy. 2011. Vol. 36. No. 3. pp. 2128-2136.
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TY - JOUR
DO - 10.1016/j.ijhydene.2010.11.042
UR - https://doi.org/10.1016/j.ijhydene.2010.11.042
TI - Effect of Co–Ni ratio on the activity and stability of Co–Ni bimetallic aerogel catalyst for methane Oxy-CO2 reforming
T2 - International Journal of Hydrogen Energy
AU - Chen, Leah
AU - Zhu, Qingshan
AU - Wu, Rongfang
PY - 2011
DA - 2011/02/01
PB - Elsevier
SP - 2128-2136
IS - 3
VL - 36
SN - 0360-3199
SN - 1879-3487
ER -
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@article{2011_Chen,
author = {Leah Chen and Qingshan Zhu and Rongfang Wu},
title = {Effect of Co–Ni ratio on the activity and stability of Co–Ni bimetallic aerogel catalyst for methane Oxy-CO2 reforming},
journal = {International Journal of Hydrogen Energy},
year = {2011},
volume = {36},
publisher = {Elsevier},
month = {feb},
url = {https://doi.org/10.1016/j.ijhydene.2010.11.042},
number = {3},
pages = {2128--2136},
doi = {10.1016/j.ijhydene.2010.11.042}
}
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Chen, Leah, et al. “Effect of Co–Ni ratio on the activity and stability of Co–Ni bimetallic aerogel catalyst for methane Oxy-CO2 reforming.” International Journal of Hydrogen Energy, vol. 36, no. 3, Feb. 2011, pp. 2128-2136. https://doi.org/10.1016/j.ijhydene.2010.11.042.