Journal of Alloys and Compounds, volume 764, pages 446-451

High-sensitivity broadband colloidal quantum dot heterojunction photodetector for night-sky radiation

Publication typeJournal Article
Publication date2018-10-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor6.2
ISSN09258388
Materials Chemistry
Metals and Alloys
Mechanical Engineering
Mechanics of Materials
Abstract
Being with excellent photosensibility, bandgap tunability and solution processibility, lead sulfide (PbS) colloidal quantum dot (CQD) gets one of the most attracting nanomaterials for photodetectors and light-harvesting devices. Usually short ligands are used to passivate the surface of CQDs to enhance the carrier mobility in QD films, and different types of ligands show distinct influence on the physical/electrical properties on the passivated CQD films. In this paper, a high-sensitivity broadband photodetector based on PbS-EDT/PbS-TBAl heterojunction by band-alignment engineering was presented. After optimizing the thickness of PbS CQD films, we found that the maximum specific detectivity of the photodiode ITO/ZnO(40 nm)/PbS-TBAl(160 nm)/PbS-EDT(40 nm)/Au reached to 3.93 × 1013 Jones and 5.52 × 1013 Jones under 2.0 μW/cm2 910 nm and 1.9 μW/cm2 500 nm illuminations, respectively, showing excellent stability in air and high sensitivity to weak signal (i.e. night-sky radiation). Further, the device performance of photodiode ITO/ZnO/PbS-TBAl/PbS-EDT/Au is compared with that of the control device ITO/ZnO/PbS-TBAI/Au, and the underneath mechanism for the enhanced performance is discussed.

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GOST Copy
Xu J. et al. High-sensitivity broadband colloidal quantum dot heterojunction photodetector for night-sky radiation // Journal of Alloys and Compounds. 2018. Vol. 764. pp. 446-451.
GOST all authors (up to 50) Copy
Xu J., Wang H., Yang S., Ni G., Liu R. High-sensitivity broadband colloidal quantum dot heterojunction photodetector for night-sky radiation // Journal of Alloys and Compounds. 2018. Vol. 764. pp. 446-451.
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RIS Copy
TY - JOUR
DO - 10.1016/j.jallcom.2018.06.105
UR - https://doi.org/10.1016/j.jallcom.2018.06.105
TI - High-sensitivity broadband colloidal quantum dot heterojunction photodetector for night-sky radiation
T2 - Journal of Alloys and Compounds
AU - Xu, Junfeng
AU - Wang, Haowei
AU - Yang, Sheng-Yi
AU - Ni, Guoqiang
AU - Liu, Rui-Bin
PY - 2018
DA - 2018/10/01 00:00:00
PB - Elsevier
SP - 446-451
VL - 764
SN - 0925-8388
ER -
BibTex
Cite this
BibTex Copy
@article{2018_Xu,
author = {Junfeng Xu and Haowei Wang and Sheng-Yi Yang and Guoqiang Ni and Rui-Bin Liu},
title = {High-sensitivity broadband colloidal quantum dot heterojunction photodetector for night-sky radiation},
journal = {Journal of Alloys and Compounds},
year = {2018},
volume = {764},
publisher = {Elsevier},
month = {oct},
url = {https://doi.org/10.1016/j.jallcom.2018.06.105},
pages = {446--451},
doi = {10.1016/j.jallcom.2018.06.105}
}
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