Sustainable synthesis of N-heterocycles in water using alcohols following the double dehydrogenation strategy
Publication type: Journal Article
Publication date: 2019-05-01
scimago Q1
wos Q1
SJR: 1.558
CiteScore: 10.9
Impact factor: 6.5
ISSN: 00219517, 10902694
Catalysis
Physical and Theoretical Chemistry
Abstract
The present study describes the first example of synthesis of pharmaceutically relevant N-heterocycles like substituted quinolines, acridines and 1,8-naphthyridines in water under air using alcohols in presence of a new water soluble Ir-complex. The viability and efficiency of this approach was demonstrated by the efficient synthesis of biologically active natural product (±)-galipinine and gram scale synthesis of various N-heteroaromatics. Several kinetic experiments and DFT calculations were carried out to support the plausible reaction mechanism which disclosed that this system followed a concerted outer sphere mechanism for the dehydrogenation of alcohols.
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98
Total citations:
98
Citations from 2024:
36
(36.74%)
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GOST
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Maji M. et al. Sustainable synthesis of N-heterocycles in water using alcohols following the double dehydrogenation strategy // Journal of Catalysis. 2019. Vol. 373. pp. 93-102.
GOST all authors (up to 50)
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Maji M., Chakrabarti K., Panja D., Kundu S. Sustainable synthesis of N-heterocycles in water using alcohols following the double dehydrogenation strategy // Journal of Catalysis. 2019. Vol. 373. pp. 93-102.
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TY - JOUR
DO - 10.1016/j.jcat.2019.03.028
UR - https://doi.org/10.1016/j.jcat.2019.03.028
TI - Sustainable synthesis of N-heterocycles in water using alcohols following the double dehydrogenation strategy
T2 - Journal of Catalysis
AU - Maji, Milan
AU - Chakrabarti, Kaushik
AU - Panja, Dibyajyoti
AU - Kundu, Sabuj
PY - 2019
DA - 2019/05/01
PB - Elsevier
SP - 93-102
VL - 373
SN - 0021-9517
SN - 1090-2694
ER -
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BibTex (up to 50 authors)
Copy
@article{2019_Maji,
author = {Milan Maji and Kaushik Chakrabarti and Dibyajyoti Panja and Sabuj Kundu},
title = {Sustainable synthesis of N-heterocycles in water using alcohols following the double dehydrogenation strategy},
journal = {Journal of Catalysis},
year = {2019},
volume = {373},
publisher = {Elsevier},
month = {may},
url = {https://doi.org/10.1016/j.jcat.2019.03.028},
pages = {93--102},
doi = {10.1016/j.jcat.2019.03.028}
}