Enhanced hydrogenation of dimethyl oxalate to ethylene glycol over indium promoted Cu/SiO2
Publication type: Journal Article
Publication date: 2019-12-01
scimago Q1
wos Q1
SJR: 1.558
CiteScore: 10.9
Impact factor: 6.5
ISSN: 00219517, 10902694
Catalysis
Physical and Theoretical Chemistry
Abstract
Hydrogenation of dimethyl oxalate (DMO) on Cu/SiO2 catalysts is the final reaction step in a growing industrial syngas to ethylene glycol (StEG) process. In the present work, indium species are found to dramatically enhance the performance of a Cu/SiO2 catalyst prepared by urea-assisted gelation for the conversion of DMO to EG. Characterization reveals that indium species have negligible effect on the content of Cu+ species on the surface. Rather, the promotional effect likely originates from interactions between reduced indium species and Cu0 species though enhanced ability of the latter to activate H2.
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56
Total citations:
56
Citations from 2025:
15
(26.79%)
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GOST
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Yu X. et al. Enhanced hydrogenation of dimethyl oxalate to ethylene glycol over indium promoted Cu/SiO2 // Journal of Catalysis. 2019. Vol. 380. pp. 289-296.
GOST all authors (up to 50)
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Yu X., Vest T. A., Gleason Boure N., Karakalos S., Tate G. L., Burkholder M., Monnier J., Williams C. Enhanced hydrogenation of dimethyl oxalate to ethylene glycol over indium promoted Cu/SiO2 // Journal of Catalysis. 2019. Vol. 380. pp. 289-296.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1016/j.jcat.2019.10.001
UR - https://doi.org/10.1016/j.jcat.2019.10.001
TI - Enhanced hydrogenation of dimethyl oxalate to ethylene glycol over indium promoted Cu/SiO2
T2 - Journal of Catalysis
AU - Yu, Xinbin
AU - Vest, Trey A
AU - Gleason Boure, Nicolas
AU - Karakalos, Stavros
AU - Tate, Gregory L.
AU - Burkholder, Michael
AU - Monnier, John
AU - Williams, C
PY - 2019
DA - 2019/12/01
PB - Elsevier
SP - 289-296
VL - 380
SN - 0021-9517
SN - 1090-2694
ER -
Cite this
BibTex (up to 50 authors)
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@article{2019_Yu,
author = {Xinbin Yu and Trey A Vest and Nicolas Gleason Boure and Stavros Karakalos and Gregory L. Tate and Michael Burkholder and John Monnier and C Williams},
title = {Enhanced hydrogenation of dimethyl oxalate to ethylene glycol over indium promoted Cu/SiO2},
journal = {Journal of Catalysis},
year = {2019},
volume = {380},
publisher = {Elsevier},
month = {dec},
url = {https://doi.org/10.1016/j.jcat.2019.10.001},
pages = {289--296},
doi = {10.1016/j.jcat.2019.10.001}
}