Journal of Energy Chemistry, volume 59, pages 108-125

Emerging material engineering strategies for amplifying photothermal heterogeneous CO2 catalysis

Publication typeJournal Article
Publication date2021-08-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor13.1
ISSN20954956
Electrochemistry
Energy Engineering and Power Technology
Fuel Technology
Energy (miscellaneous)
Abstract
A fundamental understanding of basic driving forces and the role of light in photothermal CO 2 catalysis is covered. The progress of the catalyst development and corresponding material engineering strategies are summarized. Closing the carbon loop, through CO 2 capture and utilization, is a promising route to mitigate climate change. Solar energy is a sustainable energy source which can be exploited to drive catalytic reactions for utilizing CO 2 , including converting the CO 2 into useful products. Solar energy can be harnessed through a range of different pathways to valorize CO 2 . Whilst using solar energy to drive CO 2 reduction has vast potential to promote catalytic CO 2 conversions, the progress is limited due to the lack of understanding of property-performance relations as well as feasible material engineering approaches. Herein, we outline the various driving forces involved in photothermal CO 2 catalysis. The heat from solar energy can be utilized to induce CO 2 catalytic reduction reactions via the photothermal effect. Further, solar energy can act to modify reaction pathways through light-matter interactions. Light-induced chemical functions have demonstrated the ability to regulate intermediary reaction steps, and thus control the reaction selectivity. Photothermal catalyst structures and specific catalyst design strategies are discussed in this context. This review provides a comprehensive understanding of the heat-light synergy and guidance for rational photothermal catalyst design for CO 2 utilization.

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GOST Copy
Xie B. et al. Emerging material engineering strategies for amplifying photothermal heterogeneous CO2 catalysis // Journal of Energy Chemistry. 2021. Vol. 59. pp. 108-125.
GOST all authors (up to 50) Copy
Xie B., Lu X., Tan T., Jantarang S., Yu M., Scott J. A., Amal R. Emerging material engineering strategies for amplifying photothermal heterogeneous CO2 catalysis // Journal of Energy Chemistry. 2021. Vol. 59. pp. 108-125.
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RIS Copy
TY - JOUR
DO - 10.1016/j.jechem.2020.11.005
UR - https://doi.org/10.1016/j.jechem.2020.11.005
TI - Emerging material engineering strategies for amplifying photothermal heterogeneous CO2 catalysis
T2 - Journal of Energy Chemistry
AU - Xie, Bingqiao
AU - Lu, Xunyu
AU - Tan, Tze-Woei
AU - Jantarang, Salina
AU - Yu, Mengying
AU - Scott, Jason A.
AU - Amal, Rose
PY - 2021
DA - 2021/08/01 00:00:00
PB - Elsevier
SP - 108-125
VL - 59
SN - 2095-4956
ER -
BibTex
Cite this
BibTex Copy
@article{2021_Xie,
author = {Bingqiao Xie and Xunyu Lu and Tze-Woei Tan and Salina Jantarang and Mengying Yu and Jason A. Scott and Rose Amal},
title = {Emerging material engineering strategies for amplifying photothermal heterogeneous CO2 catalysis},
journal = {Journal of Energy Chemistry},
year = {2021},
volume = {59},
publisher = {Elsevier},
month = {aug},
url = {https://doi.org/10.1016/j.jechem.2020.11.005},
pages = {108--125},
doi = {10.1016/j.jechem.2020.11.005}
}
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