Journal of Energy Chemistry, volume 79, pages 357-364
High-performance solid-state lithium metal batteries achieved by interface modification
Publication type: Journal Article
Publication date: 2023-04-01
Journal:
Journal of Energy Chemistry
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 13.1
ISSN: 20954956
Electrochemistry
Energy Engineering and Power Technology
Fuel Technology
Energy (miscellaneous)
Abstract
Garnet-structured ceramic electrolyte Li6.75La3Zr1.75Ta0.25O12 (LLZTO) attracts significant consideration in solid-state Li metal batteries due to its wide electrochemical window and favorable compatibility with Li metal. However, the deployment of LLZTO is severely hampered by poor contact between LLZTO and Li metal anode. In this paper, an ultra-thin Al-Si interface buffer layer (10 nm) is constructed on LLZTO by a magnetron sputtering method, which allows superior wetting of Li onto the LLZTO surface due to the alloying reaction between the Al-Si layer and Li metal. The resulting Li/Al-Si coated LLZTO (ASL)/Li symmetrical cell delivers an interfacial resistance of 15.0 Ω cm−2, which is much lower than that of 1140.3 Ω cm−2 for the bare LLZTO symmetrical cell. Moreover, the Li/ASL/Li symmetrical cells exhibit stable plating/striping performance (800 h) with small voltage hysteresis at 1.0 mA cm−2. Besides, the full cell with LiFePO4 cathode reveals a high capacity of 124.1 mA h g−1 after 600 cycles at 0.5C with a low-capacity decay of 0.032% per cycle. We believe this work will facilitate the development of solid-state rechargeable batteries.
Top-30
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Nanoscale Advances
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1 publication, 2.44%
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1 publication, 2.44%
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1 publication, 2.44%
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Surfaces and Interfaces
1 publication, 2.44%
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1 publication, 2.44%
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Journal of Materials Chemistry A
1 publication, 2.44%
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Energy and Environmental Science
1 publication, 2.44%
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1 publication, 2.44%
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Materials Chemistry Frontiers
1 publication, 2.44%
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Materials Today Sustainability
1 publication, 2.44%
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ACS applied materials & interfaces
1 publication, 2.44%
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Chemical Science
1 publication, 2.44%
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1 publication, 2.44%
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1 publication, 2.44%
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1 publication, 2.44%
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Citations by publishers
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5
10
15
20
25
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Elsevier
25 publications, 60.98%
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Wiley
5 publications, 12.2%
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Royal Society of Chemistry (RSC)
5 publications, 12.2%
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American Chemical Society (ACS)
4 publications, 9.76%
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 2.44%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 2.44%
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5
10
15
20
25
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Zhai L. et al. High-performance solid-state lithium metal batteries achieved by interface modification // Journal of Energy Chemistry. 2023. Vol. 79. pp. 357-364.
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Zhai L., Yang K., Jiang F., Liu W., Yan Z., Sun J. High-performance solid-state lithium metal batteries achieved by interface modification // Journal of Energy Chemistry. 2023. Vol. 79. pp. 357-364.
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TY - JOUR
DO - 10.1016/j.jechem.2023.01.022
UR - https://doi.org/10.1016/j.jechem.2023.01.022
TI - High-performance solid-state lithium metal batteries achieved by interface modification
T2 - Journal of Energy Chemistry
AU - Zhai, Lei
AU - Yang, K
AU - Jiang, F.Y.
AU - Liu, Wenbao
AU - Yan, Zhenhua
AU - Sun, Jian-Chao
PY - 2023
DA - 2023/04/01 00:00:00
PB - Elsevier
SP - 357-364
VL - 79
SN - 2095-4956
ER -
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@article{2023_Zhai,
author = {Lei Zhai and K Yang and F.Y. Jiang and Wenbao Liu and Zhenhua Yan and Jian-Chao Sun},
title = {High-performance solid-state lithium metal batteries achieved by interface modification},
journal = {Journal of Energy Chemistry},
year = {2023},
volume = {79},
publisher = {Elsevier},
month = {apr},
url = {https://doi.org/10.1016/j.jechem.2023.01.022},
pages = {357--364},
doi = {10.1016/j.jechem.2023.01.022}
}
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