Journal of Energy Chemistry, volume 81, pages 358-378
Solid polymer electrolytes in all-solid-state lithium metal batteries: from microstructures to properties
Publication type: Journal Article
Publication date: 2023-06-01
Journal:
Journal of Energy Chemistry
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 13.1
ISSN: 20954956
Electrochemistry
Energy Engineering and Power Technology
Fuel Technology
Energy (miscellaneous)
Abstract
All-solid-state lithium (Li) metal batteries (ASSLMBs) are considered one of the most promising secondary batteries due to their high theoretical capacity and high safety performance. However, low room-temperature ionic conductivity and poor interfacial stability are two key factors affecting the practical application of ASSLMBs, and our understanding of the mechanisms behind these key problems from microscopic perspective is still limited. In this review, the mechanisms and advanced characterization techniques of ASSLMBs are summarized to correlate the microstructures and properties. Firstly, we summarize the challenges faced by solid polymer electrolytes (SPEs) in ASSLMBs, such as the low room-temperature ionic conductivity and the poor interfacial stability. Secondly, several typical improvement methods of polymer ASSLMBs are discussed, including composite SPEs, ultra-thin SPEs, SPEs surface modification and Li anode surface modification. Finally, we conclude the characterizations for correlating the microstructures and the properties of SPEs, with emphasis on the use of emerging advanced techniques (e.g., cryo-transmission electron microscopy) for in-depth analyzing ASSLMBs. The influence of the microstructures on the properties is very important. Until now, it has been difficult for us to understand the microstructures of batteries. However, some recent studies have demonstrated that we have a better understanding of the microstructures of batteries. Then we suggest that in situ characterization, nondestructive characterization and sub-angstrom resolution are the key technologies to help us further understand the batteries’ microstructures and promote the development of batteries. And potential investigations to understand the microstructures evolution and the batteries behaviors are also prospected to expect further reasonable theoretical guidance for the design of ASSLMBs with ideal performance.
Top-30
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1 publication, 4%
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1 publication, 4%
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1 publication, 4%
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1 publication, 4%
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1 publication, 4%
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Citations by publishers
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Elsevier
10 publications, 40%
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Wiley
6 publications, 24%
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Royal Society of Chemistry (RSC)
5 publications, 20%
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American Chemical Society (ACS)
2 publications, 8%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 4%
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 4%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Lin Z. et al. Solid polymer electrolytes in all-solid-state lithium metal batteries: from microstructures to properties // Journal of Energy Chemistry. 2023. Vol. 81. pp. 358-378.
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Lin Z., Sheng O., Cai X., Duan D., Ke Y., Nai J., Wang Y., Liu T., Tao X., Liu Y. Solid polymer electrolytes in all-solid-state lithium metal batteries: from microstructures to properties // Journal of Energy Chemistry. 2023. Vol. 81. pp. 358-378.
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TY - JOUR
DO - 10.1016/j.jechem.2023.01.063
UR - https://doi.org/10.1016/j.jechem.2023.01.063
TI - Solid polymer electrolytes in all-solid-state lithium metal batteries: from microstructures to properties
T2 - Journal of Energy Chemistry
AU - Lin, Zongxi
AU - Sheng, Ouwei
AU - Cai, Xiaohan
AU - Duan, Dan
AU - Ke, Yue
AU - Nai, Jianwei
AU - Wang, Yao
AU - Liu, Tiefeng
AU - Tao, Xinyong
AU - Liu, Yujing
PY - 2023
DA - 2023/06/01 00:00:00
PB - Elsevier
SP - 358-378
VL - 81
SN - 2095-4956
ER -
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@article{2023_Lin,
author = {Zongxi Lin and Ouwei Sheng and Xiaohan Cai and Dan Duan and Yue Ke and Jianwei Nai and Yao Wang and Tiefeng Liu and Xinyong Tao and Yujing Liu},
title = {Solid polymer electrolytes in all-solid-state lithium metal batteries: from microstructures to properties},
journal = {Journal of Energy Chemistry},
year = {2023},
volume = {81},
publisher = {Elsevier},
month = {jun},
url = {https://doi.org/10.1016/j.jechem.2023.01.063},
pages = {358--378},
doi = {10.1016/j.jechem.2023.01.063}
}