Joule, volume 3, issue 7, pages 1689-1702

Designer Anion Enabling Solid-State Lithium-Sulfur Batteries

Heng Zhang

Heng Zhang ¹

Uxue Oteo ¹

Xabier Judez

Xabier Judez ¹

Gebrekidan Gebresilassie Eshetu

Gebrekidan Gebresilassie Eshetu ^{2, 3}

María Martínez Ibañez

María Martinez-Ibañez ¹

Javier Carrasco

Javier Carrasco ¹

Chunmei Li

Chunmei Li ¹

Michel Armand

Michel Armand ¹

Hide authors affiliations Show authors affiliations: 3 affiliations

Electrical Energy Storage Department, CIC Energigune, Parque Tecnológico de Álava, Albert Einstein 48, 01510 Miñano, Álava, Spain |

Department of Chemistry, College of Natural and Computational Sciences, Mekelle University, P.O. Box 231, Mekelle, Ethiopia |

Institute for Power Electronics and Electrical Drives (ISEA), RWTH Aachen University, Jägerstraße 17/19, 52066 Aachen, Germany |

Publication type: Journal Article

Publication date: 2019-07-01

Elsevier

Journal: Joule

Quartile SCImago

Quartile WOS

Impact factor: 39.8

ISSN: 25424351, 25424351

DOI: 10.1016/j.joule.2019.05.003

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General Energy

Abstract

Summary With an extremely high theoretical energy density, solid-state lithium-sulfur (Li-S) batteries (SSLSBs) are emerging as one of the most feasible chemistries; however, their energy efficiency and long-term cyclability are severely hampered by the lithium metal (Li°) dendrite formation during repeated discharge/charge cycles and the shuttling of aggressive polysulfide intermediates between two electrodes. Herein, we report (difluoromethanesulfonyl) (trifluoromethanesulfonyl)imide anion [N(SO2CF2H)(SO2CF3)]−, hereafter DFTFSI−, as a designer anion for high-performance polymer-based SSLSBs. In contrast to the widely used bis(trifluoromethanesulfonyl)imide anion [N(SO2CF3)2]− (TFSI−), DFTFSI-based SSLSBs provide superior interfacial stability against Li°, extremely high discharge and areal capacities, very high Coulombic efficiency, and long-term cyclability, surpassing the reported literature values, in terms of gravimetric energy density. This work opens a new door for accelerating the practical deployment of SSLSBs in the future.

By date By citations

Top-30

Citations by journals

	1 2 3 4 5 6 7 8 9
Advanced Functional Materials	Advanced Functional Materials, 9, 7.2% Advanced Functional Materials 9 publications, 7.2%
Advanced Materials	Advanced Materials, 6, 4.8% Advanced Materials 6 publications, 4.8%
Small	Small, 5, 4% Small 5 publications, 4%
Advanced Energy Materials	Advanced Energy Materials, 5, 4% Advanced Energy Materials 5 publications, 4%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 5, 4% Journal of the Electrochemical Society 5 publications, 4%
Energy Storage Materials	Energy Storage Materials, 5, 4% Energy Storage Materials 5 publications, 4%
Journal of Energy Chemistry	Journal of Energy Chemistry, 4, 3.2% Journal of Energy Chemistry 4 publications, 3.2%
Batteries & Supercaps	Batteries & Supercaps, 4, 3.2% Batteries & Supercaps 4 publications, 3.2%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 4, 3.2% Journal of Materials Chemistry A 4 publications, 3.2%
Journal of Power Sources	Journal of Power Sources, 3, 2.4% Journal of Power Sources 3 publications, 2.4%
Energy & Fuels	Energy & Fuels, 3, 2.4% Energy & Fuels 3 publications, 2.4%
Journal of the American Chemical Society	Journal of the American Chemical Society, 3, 2.4% Journal of the American Chemical Society 3 publications, 2.4%
ACS Applied Energy Materials	ACS Applied Energy Materials, 3, 2.4% ACS Applied Energy Materials 3 publications, 2.4%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 2, 1.6% Journal of Physical Chemistry C 2 publications, 1.6%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 1.6% Chemical Engineering Journal 2 publications, 1.6%
Materials Today Energy	Materials Today Energy, 2, 1.6% Materials Today Energy 2 publications, 1.6%
Joule	Joule, 2, 1.6% Joule 2 publications, 1.6%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 2, 1.6% Angewandte Chemie - International Edition 2 publications, 1.6%
Angewandte Chemie	Angewandte Chemie, 2, 1.6% Angewandte Chemie 2 publications, 1.6%
Energy and Environmental Science	Energy and Environmental Science, 2, 1.6% Energy and Environmental Science 2 publications, 1.6%
Chemical Society Reviews	Chemical Society Reviews, 2, 1.6% Chemical Society Reviews 2 publications, 1.6%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 2, 1.6% Journal of Colloid and Interface Science 2 publications, 1.6%
Sustainability	Sustainability, 1, 0.8% Sustainability 1 publication, 0.8%
Nano-Micro Letters	Nano-Micro Letters, 1, 0.8% Nano-Micro Letters 1 publication, 0.8%
Composites Part B: Engineering	Composites Part B: Engineering, 1, 0.8% Composites Part B: Engineering 1 publication, 0.8%
Interdisciplinary Materials	Interdisciplinary Materials, 1, 0.8% Interdisciplinary Materials 1 publication, 0.8%
Nanomaterials	Nanomaterials, 1, 0.8% Nanomaterials 1 publication, 0.8%
Molecules	Molecules, 1, 0.8% Molecules 1 publication, 0.8%
Inorganics	Inorganics, 1, 0.8% Inorganics 1 publication, 0.8%
Batteries	Batteries, 1, 0.8% Batteries 1 publication, 0.8%
	1 2 3 4 5 6 7 8 9

Citations by publishers

	5 10 15 20 25 30 35 40
Wiley	Wiley, 40, 32% Wiley 40 publications, 32%
Elsevier	Elsevier, 33, 26.4% Elsevier 33 publications, 26.4%
American Chemical Society (ACS)	American Chemical Society (ACS), 16, 12.8% American Chemical Society (ACS) 16 publications, 12.8%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 10, 8% Royal Society of Chemistry (RSC) 10 publications, 8%
Springer Nature	Springer Nature, 8, 6.4% Springer Nature 8 publications, 6.4%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 5, 4% Multidisciplinary Digital Publishing Institute (MDPI) 5 publications, 4%
The Electrochemical Society	The Electrochemical Society, 5, 4% The Electrochemical Society 5 publications, 4%
Taylor & Francis	Taylor & Francis, 1, 0.8% Taylor & Francis 1 publication, 0.8%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 0.8% Korean Society of Industrial Engineering Chemistry 1 publication, 0.8%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.8% Nonferrous Metals Society of China 1 publication, 0.8%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.8% American Association for the Advancement of Science (AAAS) 1 publication, 0.8%
Hans Publishers	Hans Publishers, 1, 0.8% Hans Publishers 1 publication, 0.8%
OAE Publishing Inc.	OAE Publishing Inc., 1, 0.8% OAE Publishing Inc. 1 publication, 0.8%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 0.8% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 0.8%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.8% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.8%
	5 10 15 20 25 30 35 40

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Zhang H. et al. Designer Anion Enabling Solid-State Lithium-Sulfur Batteries // Joule. 2019. Vol. 3. No. 7. pp. 1689-1702.

GOST all authors (up to 50) Copy

Zhang H., Zhang H., Oteo U., Judez X., Judez X., Eshetu G. G., Eshetu G. G., Martínez Ibañez M., Martinez-Ibañez M., Carrasco J., Carrasco J., Li C., Li C., Armand M., Armand M. Designer Anion Enabling Solid-State Lithium-Sulfur Batteries // Joule. 2019. Vol. 3. No. 7. pp. 1689-1702.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.joule.2019.05.003

UR - https://doi.org/10.1016/j.joule.2019.05.003

TI - Designer Anion Enabling Solid-State Lithium-Sulfur Batteries

T2 - Joule

AU - Zhang, Heng

AU - Oteo, Uxue

AU - Judez, Xabier

AU - Eshetu, Gebrekidan Gebresilassie

AU - Martínez Ibañez, María

AU - Carrasco, Javier

AU - Li, Chunmei

AU - Armand, Michel

AU - Zhang, Heng

AU - Judez, Xabier

AU - Eshetu, Gebrekidan Gebresilassie

AU - Martinez-Ibañez, María

AU - Carrasco, Javier

AU - Li, Chunmei

AU - Armand, Michel

PY - 2019

DA - 2019/07/01 00:00:00

PB - Elsevier

SP - 1689-1702

IS - 7

VL - 3

SN - 2542-4351

ER -

BibTex |

Cite this

BibTex Copy

@article{2019_Zhang,

author = {Heng Zhang and Uxue Oteo and Xabier Judez and Gebrekidan Gebresilassie Eshetu and María Martínez Ibañez and Javier Carrasco and Chunmei Li and Michel Armand and Heng Zhang and Xabier Judez and Gebrekidan Gebresilassie Eshetu and María Martinez-Ibañez and Javier Carrasco and Chunmei Li and Michel Armand},

title = {Designer Anion Enabling Solid-State Lithium-Sulfur Batteries},

journal = {Joule},

year = {2019},

volume = {3},

publisher = {Elsevier},

month = {jul},

url = {https://doi.org/10.1016/j.joule.2019.05.003},

number = {7},

pages = {1689--1702},

doi = {10.1016/j.joule.2019.05.003}

}

MLA

Cite this

MLA Copy

Zhang, Heng, et al. “Designer Anion Enabling Solid-State Lithium-Sulfur Batteries.” Joule, vol. 3, no. 7, Jul. 2019, pp. 1689-1702. https://doi.org/10.1016/j.joule.2019.05.003.

Found error?

Publisher

Elsevier

Journal

Joule

Quartile SCImago

Quartile WOS

Impact factor

39.8

ISSN

25424351 (Electronic)
25424351 (Print)