Journal of Photochemistry and Photobiology C: Photochemistry Reviews, volume 18, pages 71-90

Genesis of rare molecules using light-induced reactions of matrix-isolated tetrazoles

Luı́s M.T Frija ¹

Maria L. S. Cristiano ²

Andrea Gómez-Zavaglia ^{3, 4}

Igor Reva ⁴

Rui Fausto ⁴

Hide authors affiliations Show authors affiliations: 4 affiliations

Research Institute for Medicines and Pharmaceutical Sciences (iMed.UL), Faculty of Pharmacy, University of Lisbon. Av. Prof. Gama Pinto, 1649-003 Lisbon, Portugal |

CCMAR and Department of Chemistry and Pharmacy, F.C.T, University of Algarve, Campus de Gambelas, 8005-039 Faro, Portugal |

Centro de Investigación y Desarrollo en Criotecnología de Alimentos (Conicet La Plata, UNLP), RA-1900, Argentina |

⁴

Department of Chemistry, University of Coimbra, 3004-535, Portugal |

Publication type: Journal Article

Publication date: 2014-03-01

Elsevier

Journal: Journal of Photochemistry and Photobiology C: Photochemistry Reviews

Quartile SCImago

Quartile WOS

Impact factor: 13.6

ISSN: 13895567

DOI: 10.1016/j.jphotochemrev.2013.09.001

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Catalysis

Organic Chemistry

Physical and Theoretical Chemistry

Abstract

Tetrazoles exhibit a very rich photochemistry, strongly influenced by the nature of substituents in the tetrazolic ring. Photolysis of representative tetrazoles trapped in a rigid environment of solidified noble gases at cryogenic temperatures (usually argon at 10–15 K) results in photofragmentation of the monomeric species with a wide range of exit channels. Since the obtained fragments are generally confined to the matrix cage where they are formed, no subsequent cross-reactions involving species resulting from photolysis can occur, strongly reducing the number of possible photoproducts in comparison with gas phase or solution studies. These conditions introduce a useful simplification for the interpretation of the reaction mechanisms and enable spectroscopic characterization of novel and/or highly reactive molecules. In this review, we provide an updated report on the photolysis of matrix-isolated tetrazoles, focusing on the scope and usefulness of this methodology for generation of rare molecules and investigation of photocleavage pathways. Special emphasis is placed on mechanistic interpretations and characterization of rare molecules and on the relevance of conformation and tautomerism on the photochemistry of the studied compounds.

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Frija L. M. et al. Genesis of rare molecules using light-induced reactions of matrix-isolated tetrazoles // Journal of Photochemistry and Photobiology C: Photochemistry Reviews. 2014. Vol. 18. pp. 71-90.

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Frija L. M., Cristiano M. L. S., Gómez-Zavaglia A., Reva I., Fausto R. Genesis of rare molecules using light-induced reactions of matrix-isolated tetrazoles // Journal of Photochemistry and Photobiology C: Photochemistry Reviews. 2014. Vol. 18. pp. 71-90.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.jphotochemrev.2013.09.001

UR - https://doi.org/10.1016/j.jphotochemrev.2013.09.001

TI - Genesis of rare molecules using light-induced reactions of matrix-isolated tetrazoles

T2 - Journal of Photochemistry and Photobiology C: Photochemistry Reviews

AU - Frija, Luı́s M.T

AU - Cristiano, Maria L. S.

AU - Gómez-Zavaglia, Andrea

AU - Reva, Igor

AU - Fausto, Rui

PY - 2014

DA - 2014/03/01 00:00:00

PB - Elsevier

SP - 71-90

VL - 18

SN - 1389-5567

ER -

BibTex

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BibTex Copy

@article{2014_Frija,

author = {Luı́s M.T Frija and Maria L. S. Cristiano and Andrea Gómez-Zavaglia and Igor Reva and Rui Fausto},

title = {Genesis of rare molecules using light-induced reactions of matrix-isolated tetrazoles},

journal = {Journal of Photochemistry and Photobiology C: Photochemistry Reviews},

year = {2014},

volume = {18},

publisher = {Elsevier},

month = {mar},

url = {https://doi.org/10.1016/j.jphotochemrev.2013.09.001},

pages = {71--90},

doi = {10.1016/j.jphotochemrev.2013.09.001}

}

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Publisher

Elsevier

Journal

Journal of Photochemistry and Photobiology C: Photochemistry Reviews

Quartile SCImago

Quartile WOS

Impact factor

13.6

ISSN

13895567 (Print)