volume 210 pages 366-373

Long-term cell degradation mechanism in high-temperature proton exchange membrane fuel cells

Yuka Oono 1
Atsuo SOUNAI 2
Michio Hori 1
1
 
Fuel Cell Research Center, Daido University, 10-3 Takiharu-cho, Minami-ku, Nagoya, Aichi 457-8530, Japan
2
 
Dept. of Materials Science & Engineering, Suzuka National College of Technology, Shirako-cho, Suzuka, Mie 510-0294, Japan
Publication typeJournal Article
Publication date2012-07-01
scimago Q1
wos Q1
SJR1.784
CiteScore14.9
Impact factor7.9
ISSN03787753, 18732755
Physical and Theoretical Chemistry
Electrical and Electronic Engineering
Energy Engineering and Power Technology
Renewable Energy, Sustainability and the Environment
Abstract
The mechanism underlying the decline in cell voltage over time was investigated for high-temperature proton exchange membrane fuel cells. Five identical cells were prepared and long-term power generation tests were conducted at an operation temperature of 150 °C and a current density of 0.2 A cm −2 for periods of up to 17,860 h. Each of the cells was then analyzed using transmission electron microscopy and electron probe micro-analysis (EPMA). The results indicated that growth of the Pt catalyst particles occurred during operation, in addition to oxidation of the carbon support. Degradation of the catalyst layers was investigated by EPMA of cross sections of the membrane electrode assemblies, allowing the mechanism of cell performance reduction to be clarified.
Found 
Found 

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GOST Copy
Oono Y., SOUNAI A., Hori M. Long-term cell degradation mechanism in high-temperature proton exchange membrane fuel cells // Journal of Power Sources. 2012. Vol. 210. pp. 366-373.
GOST all authors (up to 50) Copy
Oono Y., SOUNAI A., Hori M. Long-term cell degradation mechanism in high-temperature proton exchange membrane fuel cells // Journal of Power Sources. 2012. Vol. 210. pp. 366-373.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1016/j.jpowsour.2012.02.098
UR - https://doi.org/10.1016/j.jpowsour.2012.02.098
TI - Long-term cell degradation mechanism in high-temperature proton exchange membrane fuel cells
T2 - Journal of Power Sources
AU - Oono, Yuka
AU - SOUNAI, Atsuo
AU - Hori, Michio
PY - 2012
DA - 2012/07/01
PB - Elsevier
SP - 366-373
VL - 210
SN - 0378-7753
SN - 1873-2755
ER -
BibTex
Cite this
BibTex (up to 50 authors) Copy
@article{2012_Oono,
author = {Yuka Oono and Atsuo SOUNAI and Michio Hori},
title = {Long-term cell degradation mechanism in high-temperature proton exchange membrane fuel cells},
journal = {Journal of Power Sources},
year = {2012},
volume = {210},
publisher = {Elsevier},
month = {jul},
url = {https://doi.org/10.1016/j.jpowsour.2012.02.098},
pages = {366--373},
doi = {10.1016/j.jpowsour.2012.02.098}
}