Journal of Power Sources, volume 240, pages 8-13

Efficient electron injection in non-toxic silver sulfide (Ag2S) sensitized solar cells

Heping Shen ¹

Xingjian Jiao ¹

D. Oron ²

Jianbao Li ³

Hong Lin ¹

Hide authors affiliations Show authors affiliations: 3 affiliations

State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science & Engineering, Tsinghua University, Beijing 100084, PR China |

Dept. of Physics of Complex Systems, Weizmann Inst. Of Science, Rehovot 76100 ISRAEL |

College of Materials Science and Chemical Engineering, Hainan University, Haikou 570228, PR China |

Publication type: Journal Article

Publication date: 2013-10-01

Elsevier

Journal: Journal of Power Sources

Quartile SCImago

Quartile WOS

Impact factor: 9.2

ISSN: 03787753

DOI: 10.1016/j.jpowsour.2013.03.168

Copy DOI

Physical and Theoretical Chemistry

Electrical and Electronic Engineering

Energy Engineering and Power Technology

Renewable Energy, Sustainability and the Environment

Abstract

α-Ag 2 S, with a direct forbidden bandgap of about 1.0 eV, is a non-toxic low bandgap semiconductor which can readily be deposited in the form of a thin film by chemical bath deposition. In a solar cell configuration, it can potentially provide a high short-circuit current due to the infrared absorption, and is compatible with the polysulfide electrolyte. Its practical use in a solar cell depends, however, critically on band alignment between the Ag 2 S, the oxide anode and the electrolyte redox potential. Here we examine the conduction band (CB) offsets in the nanostructured α-Ag 2 S sensitized TiO 2 and SnO 2 electrodes by X-ray Photoelectron Spectroscopy, and show that they can significantly differ from the extrapolated bulk values. The much higher CB offset for SnO 2 /Ag 2 S interface (∼0.6 eV) compared with that of ∼0.2 eV for TiO 2 /Ag 2 S, supplied a sufficient injection driving force and was favorable for the electron separation at the heterojunction. When fabricated into solar cells, a dramatically higher current density under AM 1.5 illumination for the SnO 2 /Ag 2 S heterojunction was obtained, which was contributed by the efficient electron injection.

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Citations by journals

	1 2 3
Electrochimica Acta	Electrochimica Acta, 3, 5.08% Electrochimica Acta 3 publications, 5.08%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 2, 3.39% Journal of Materials Science: Materials in Electronics 2 publications, 3.39%
Scientific Reports	Scientific Reports, 2, 3.39% Scientific Reports 2 publications, 3.39%
Journal of Power Sources	Journal of Power Sources, 2, 3.39% Journal of Power Sources 2 publications, 3.39%
Solar Energy Materials and Solar Cells	Solar Energy Materials and Solar Cells, 2, 3.39% Solar Energy Materials and Solar Cells 2 publications, 3.39%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 2, 3.39% Journal of Alloys and Compounds 2 publications, 3.39%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 2, 3.39% Physical Chemistry Chemical Physics 2 publications, 3.39%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 2, 3.39% Journal of Materials Chemistry A 2 publications, 3.39%
RSC Advances	RSC Advances, 2, 3.39% RSC Advances 2 publications, 3.39%
Chemistry of Materials	Chemistry of Materials, 1, 1.69% Chemistry of Materials 1 publication, 1.69%
Journal of Applied Physics	Journal of Applied Physics, 1, 1.69% Journal of Applied Physics 1 publication, 1.69%
AIP Advances	AIP Advances, 1, 1.69% AIP Advances 1 publication, 1.69%
Royal Society Open Science	Royal Society Open Science, 1, 1.69% Royal Society Open Science 1 publication, 1.69%
Modern Physics Letters B	Modern Physics Letters B, 1, 1.69% Modern Physics Letters B 1 publication, 1.69%
Materials	Materials, 1, 1.69% Materials 1 publication, 1.69%
Micromachines	Micromachines, 1, 1.69% Micromachines 1 publication, 1.69%
Applied Sciences (Switzerland)	Applied Sciences (Switzerland), 1, 1.69% Applied Sciences (Switzerland) 1 publication, 1.69%
Analytical and Bioanalytical Chemistry	Analytical and Bioanalytical Chemistry, 1, 1.69% Analytical and Bioanalytical Chemistry 1 publication, 1.69%
Theoretical Chemistry Accounts	Theoretical Chemistry Accounts, 1, 1.69% Theoretical Chemistry Accounts 1 publication, 1.69%
Journal of Solid State Electrochemistry	Journal of Solid State Electrochemistry, 1, 1.69% Journal of Solid State Electrochemistry 1 publication, 1.69%
Chinese Science Bulletin	Chinese Science Bulletin, 1, 1.69% Chinese Science Bulletin 1 publication, 1.69%
Nanoscale Research Letters	Nanoscale Research Letters, 1, 1.69% Nanoscale Research Letters 1 publication, 1.69%
Materials Today: Proceedings	Materials Today: Proceedings, 1, 1.69% Materials Today: Proceedings 1 publication, 1.69%
Nanotechnology	Nanotechnology, 1, 1.69% Nanotechnology 1 publication, 1.69%
Materials Science in Semiconductor Processing	Materials Science in Semiconductor Processing, 1, 1.69% Materials Science in Semiconductor Processing 1 publication, 1.69%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 1, 1.69% Coordination Chemistry Reviews 1 publication, 1.69%
Applied Surface Science	Applied Surface Science, 1, 1.69% Applied Surface Science 1 publication, 1.69%
Solar Energy	Solar Energy, 1, 1.69% Solar Energy 1 publication, 1.69%
Advances in Colloid and Interface Science	Advances in Colloid and Interface Science, 1, 1.69% Advances in Colloid and Interface Science 1 publication, 1.69%
Results in Physics	Results in Physics, 1, 1.69% Results in Physics 1 publication, 1.69%
	1 2 3

Citations by publishers

	2 4 6 8 10 12 14 16 18
Elsevier	Elsevier, 17, 28.81% Elsevier 17 publications, 28.81%
Springer Nature	Springer Nature, 10, 16.95% Springer Nature 10 publications, 16.95%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 9, 15.25% Royal Society of Chemistry (RSC) 9 publications, 15.25%
American Chemical Society (ACS)	American Chemical Society (ACS), 8, 13.56% American Chemical Society (ACS) 8 publications, 13.56%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 5.08% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 5.08%
Wiley	Wiley, 3, 5.08% Wiley 3 publications, 5.08%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 3.39% American Institute of Physics (AIP) 2 publications, 3.39%
The Royal Society	The Royal Society, 1, 1.69% The Royal Society 1 publication, 1.69%
World Scientific	World Scientific, 1, 1.69% World Scientific 1 publication, 1.69%
IOP Publishing	IOP Publishing, 1, 1.69% IOP Publishing 1 publication, 1.69%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 1.69% Korean Society of Industrial Engineering Chemistry 1 publication, 1.69%
Trans Tech Publications	Trans Tech Publications, 1, 1.69% Trans Tech Publications 1 publication, 1.69%
Chinese Physical Society	Chinese Physical Society, 1, 1.69% Chinese Physical Society 1 publication, 1.69%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.69% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.69%
	2 4 6 8 10 12 14 16 18

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Shen H. et al. Efficient electron injection in non-toxic silver sulfide (Ag2S) sensitized solar cells // Journal of Power Sources. 2013. Vol. 240. pp. 8-13.

GOST all authors (up to 50) Copy

Shen H., Jiao X., Oron D., Li J., Lin H. Efficient electron injection in non-toxic silver sulfide (Ag2S) sensitized solar cells // Journal of Power Sources. 2013. Vol. 240. pp. 8-13.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.jpowsour.2013.03.168

UR - https://doi.org/10.1016/j.jpowsour.2013.03.168

TI - Efficient electron injection in non-toxic silver sulfide (Ag2S) sensitized solar cells

T2 - Journal of Power Sources

AU - Shen, Heping

AU - Jiao, Xingjian

AU - Oron, D.

AU - Li, Jianbao

AU - Lin, Hong

PY - 2013

DA - 2013/10/01 00:00:00

PB - Elsevier

SP - 8-13

VL - 240

SN - 0378-7753

ER -

BibTex

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BibTex Copy

@article{2013_Shen,

author = {Heping Shen and Xingjian Jiao and D. Oron and Jianbao Li and Hong Lin},

title = {Efficient electron injection in non-toxic silver sulfide (Ag2S) sensitized solar cells},

journal = {Journal of Power Sources},

year = {2013},

volume = {240},

publisher = {Elsevier},

month = {oct},

url = {https://doi.org/10.1016/j.jpowsour.2013.03.168},

pages = {8--13},

doi = {10.1016/j.jpowsour.2013.03.168}

}

Found error?

Publisher

Elsevier

Journal

Journal of Power Sources

Quartile SCImago

Quartile WOS

Impact factor

9.2

ISSN

03787753 (Print)