Journal of Power Sources, volume 301, pages 47-53

A new solid polymer electrolyte incorporating Li10GeP2S12 into a polyethylene oxide matrix for all-solid-state lithium batteries

Yanran Zhao ^{1, 2}

Chuan Wu ^{3, 4, 5, 6}

Gang Peng ⁷

Xiaotian Chen ⁷

Xiayin Yao ⁷

Ying Bai ^{3, 4, 5, 6}

Feng Wu ^{3, 4, 5, 6}

Shaojie Chen ⁷

Xiaoxiong Xu ⁷

Hide authors affiliations Show authors affiliations: 7 affiliations

Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, 315201, China |

Beijing Key Laboratory of Environmental Science and Engineering, School of Material Science and Engineering, Beijing Institute of Technology, Beijing, 100081, China |

Beijing Key Laboratory of Environmental Science and Engineering |

⁴

School of Material Science and Engineering

⁵

BeiJing Institute of Technology |

⁶

Beijing 100081 China |

⁷

Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China |

Publication type: Journal Article

Publication date: 2016-01-01

Elsevier

Journal: Journal of Power Sources

Quartile SCImago

Quartile WOS

Impact factor: 9.2

ISSN: 03787753

DOI: 10.1016/j.jpowsour.2015.09.111

Copy DOI

Physical and Theoretical Chemistry

Electrical and Electronic Engineering

Energy Engineering and Power Technology

Renewable Energy, Sustainability and the Environment

Abstract

Li10GeP2S12 (LGPS) is incorporated into polyethylene oxide (PEO) matrix to fabricate composite solid polymer electrolyte (SPE) membranes. The lithium ion conductivities of as-prepared composite membranes are evaluated, and the optimal composite membrane exhibits a maximum ionic conductivity of 1.21 × 10−3 S cm−1 at 80 °C and an electrochemical window of 0–5.7 V. The phase transition behaviors for electrolytes are characterized by DSC, and the possible reasons for their enhanced ionic conductivities are discussed. The LGPS microparticles, acting as active fillers incorporation into the PEO matrix, have a positive effect on the ionic conductivity, lithium ion transference number and electrochemical stabilities. In addition, two kinds of all-solid-state lithium batteries (LiFeO4/SPE/Li and LiCoO2/SPE/Li) are fabricated to demonstrate the good compatibility between this new SPE membrane and different electrodes. And the LiFePO4/Li battery exhibits fascinating electrochemical performance with high capacity retention (92.5% after 50 cycles at 60 °C) and attractive capacities of 158, 148, 138 and 99 mAh g−1 at current rates of 0.1 C, 0.2 C, 0.5 C and 1 C at 60 °C, respectively. It is demonstrated that this new composite SPE should be a promising electrolyte applied in solid state batteries based on lithium metal electrode.

By date By citations

Top-30

Citations by journals

	5 10 15 20 25
Journal of Power Sources	Journal of Power Sources, 23, 6.15% Journal of Power Sources 23 publications, 6.15%
Energy Storage Materials	Energy Storage Materials, 18, 4.81% Energy Storage Materials 18 publications, 4.81%
ACS applied materials & interfaces	ACS applied materials & interfaces, 16, 4.28% ACS applied materials & interfaces 16 publications, 4.28%
Electrochimica Acta	Electrochimica Acta, 15, 4.01% Electrochimica Acta 15 publications, 4.01%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 13, 3.48% Journal of Materials Chemistry A 13 publications, 3.48%
Solid State Ionics	Solid State Ionics, 12, 3.21% Solid State Ionics 12 publications, 3.21%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 9, 2.41% Journal of the Electrochemical Society 9 publications, 2.41%
Advanced Materials	Advanced Materials, 9, 2.41% Advanced Materials 9 publications, 2.41%
ACS Applied Energy Materials	ACS Applied Energy Materials, 9, 2.41% ACS Applied Energy Materials 9 publications, 2.41%
Journal of Energy Storage	Journal of Energy Storage, 7, 1.87% Journal of Energy Storage 7 publications, 1.87%
Nano Energy	Nano Energy, 7, 1.87% Nano Energy 7 publications, 1.87%
RSC Advances	RSC Advances, 7, 1.87% RSC Advances 7 publications, 1.87%
Ionics	Ionics, 6, 1.6% Ionics 6 publications, 1.6%
Journal of Energy Chemistry	Journal of Energy Chemistry, 6, 1.6% Journal of Energy Chemistry 6 publications, 1.6%
Advanced Functional Materials	Advanced Functional Materials, 6, 1.6% Advanced Functional Materials 6 publications, 1.6%
Advanced Energy Materials	Advanced Energy Materials, 6, 1.6% Advanced Energy Materials 6 publications, 1.6%
Chemical Engineering Journal	Chemical Engineering Journal, 5, 1.34% Chemical Engineering Journal 5 publications, 1.34%
Polymers	Polymers, 4, 1.07% Polymers 4 publications, 1.07%
Molecules	Molecules, 4, 1.07% Molecules 4 publications, 1.07%
Electrochemical Energy Reviews	Electrochemical Energy Reviews, 4, 1.07% Electrochemical Energy Reviews 4 publications, 1.07%
Journal of Membrane Science	Journal of Membrane Science, 4, 1.07% Journal of Membrane Science 4 publications, 1.07%
Batteries & Supercaps	Batteries & Supercaps, 4, 1.07% Batteries & Supercaps 4 publications, 1.07%
Energy and Environmental Science	Energy and Environmental Science, 4, 1.07% Energy and Environmental Science 4 publications, 1.07%
Advanced Science	Advanced Science, 3, 0.8% Advanced Science 3 publications, 0.8%
Functional Materials Letters	Functional Materials Letters, 3, 0.8% Functional Materials Letters 3 publications, 0.8%
Frontiers in Energy Research	Frontiers in Energy Research, 3, 0.8% Frontiers in Energy Research 3 publications, 0.8%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 3, 0.8% Journal of Materials Science: Materials in Electronics 3 publications, 0.8%
Applied Surface Science	Applied Surface Science, 3, 0.8% Applied Surface Science 3 publications, 0.8%
Materials Today Nano	Materials Today Nano, 3, 0.8% Materials Today Nano 3 publications, 0.8%
	5 10 15 20 25

Citations by publishers

	20 40 60 80 100 120 140 160
Elsevier	Elsevier, 145, 38.77% Elsevier 145 publications, 38.77%
Wiley	Wiley, 64, 17.11% Wiley 64 publications, 17.11%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 43, 11.5% Royal Society of Chemistry (RSC) 43 publications, 11.5%
American Chemical Society (ACS)	American Chemical Society (ACS), 39, 10.43% American Chemical Society (ACS) 39 publications, 10.43%
Springer Nature	Springer Nature, 23, 6.15% Springer Nature 23 publications, 6.15%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 13, 3.48% Multidisciplinary Digital Publishing Institute (MDPI) 13 publications, 3.48%
The Electrochemical Society	The Electrochemical Society, 9, 2.41% The Electrochemical Society 9 publications, 2.41%
IOP Publishing	IOP Publishing, 6, 1.6% IOP Publishing 6 publications, 1.6%
Frontiers Media S.A.	Frontiers Media S.A., 5, 1.34% Frontiers Media S.A. 5 publications, 1.34%
World Scientific	World Scientific, 3, 0.8% World Scientific 3 publications, 0.8%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 0.53% American Institute of Physics (AIP) 2 publications, 0.53%
Taylor & Francis	Taylor & Francis, 2, 0.53% Taylor & Francis 2 publications, 0.53%
OAE Publishing Inc.	OAE Publishing Inc., 2, 0.53% OAE Publishing Inc. 2 publications, 0.53%
SAGE	SAGE, 1, 0.27% SAGE 1 publication, 0.27%
Polymer Society of Korea	Polymer Society of Korea, 1, 0.27% Polymer Society of Korea 1 publication, 0.27%
Chemical Industry Press	Chemical Industry Press, 1, 0.27% Chemical Industry Press 1 publication, 0.27%
Scientific Publishers	Scientific Publishers, 1, 0.27% Scientific Publishers 1 publication, 0.27%
Chinese Ceramic Society	Chinese Ceramic Society, 1, 0.27% Chinese Ceramic Society 1 publication, 0.27%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 0.27% Korean Society of Industrial Engineering Chemistry 1 publication, 0.27%
Pleiades Publishing	Pleiades Publishing, 1, 0.27% Pleiades Publishing 1 publication, 0.27%
Walter de Gruyter	Walter de Gruyter, 1, 0.27% Walter de Gruyter 1 publication, 0.27%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.27% American Association for the Advancement of Science (AAAS) 1 publication, 0.27%
Tsinghua University Press	Tsinghua University Press, 1, 0.27% Tsinghua University Press 1 publication, 0.27%
Trans Tech Publications	Trans Tech Publications, 1, 0.27% Trans Tech Publications 1 publication, 0.27%
Saratov State University	Saratov State University, 1, 0.27% Saratov State University 1 publication, 0.27%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.27% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.27%
	20 40 60 80 100 120 140 160

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Zhao Y. et al. A new solid polymer electrolyte incorporating Li10GeP2S12 into a polyethylene oxide matrix for all-solid-state lithium batteries // Journal of Power Sources. 2016. Vol. 301. pp. 47-53.

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Zhao Y., Wu C., Peng G., Chen X., Yao X., Bai Y., Wu F., Chen S., Xu X. A new solid polymer electrolyte incorporating Li10GeP2S12 into a polyethylene oxide matrix for all-solid-state lithium batteries // Journal of Power Sources. 2016. Vol. 301. pp. 47-53.

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RIS Copy

TY - JOUR

DO - 10.1016/j.jpowsour.2015.09.111

UR - https://linkinghub.elsevier.com/retrieve/pii/S0378775315303712

TI - A new solid polymer electrolyte incorporating Li10GeP2S12 into a polyethylene oxide matrix for all-solid-state lithium batteries

T2 - Journal of Power Sources

AU - Zhao, Yanran

AU - Wu, Chuan

AU - Peng, Gang

AU - Chen, Xiaotian

AU - Yao, Xiayin

AU - Bai, Ying

AU - Wu, Feng

AU - Chen, Shaojie

AU - Xu, Xiaoxiong

PY - 2016

DA - 2016/01/01 00:00:00

PB - Elsevier

SP - 47-53

VL - 301

SN - 0378-7753

ER -

BibTex

Cite this

BibTex Copy

@article{2016_Zhao,

author = {Yanran Zhao and Chuan Wu and Gang Peng and Xiaotian Chen and Xiayin Yao and Ying Bai and Feng Wu and Shaojie Chen and Xiaoxiong Xu},

title = {A new solid polymer electrolyte incorporating Li10GeP2S12 into a polyethylene oxide matrix for all-solid-state lithium batteries},

journal = {Journal of Power Sources},

year = {2016},

volume = {301},

publisher = {Elsevier},

month = {jan},

url = {https://linkinghub.elsevier.com/retrieve/pii/S0378775315303712},

pages = {47--53},

doi = {10.1016/j.jpowsour.2015.09.111}

}

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Publisher

Elsevier

Journal

Journal of Power Sources

Quartile SCImago

Quartile WOS

Impact factor

9.2

ISSN

03787753 (Print)