Journal of Power Sources, volume 382, pages 128-134
Enhanced performance of P(VDF-HFP)-based composite polymer electrolytes doped with organic-inorganic hybrid particles PMMA-ZrO2 for lithium ion batteries
Publication type: Journal Article
Publication date: 2018-04-01
Journal:
Journal of Power Sources
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 9.2
ISSN: 03787753
Physical and Theoretical Chemistry
Electrical and Electronic Engineering
Energy Engineering and Power Technology
Renewable Energy, Sustainability and the Environment
Abstract
To improve the ionic conductivity as well as enhance the mechanical strength of the gel polymer electrolyte, poly(vinylidene fluoride-hexafluoroprolene) (P(VDF-HFP))-based composite polymer electrolyte (CPE) membranes doped with the organic-inorganic hybrid particles poly(methyl methacrylate) -ZrO2 (PMMA-ZrO2) are prepared by phase inversion method, in which PMMA is successfully grafted onto the surface of the homemade nano-ZrO2 particles via in situ polymerization confirmed by FT-IR. XRD and DSC patterns show adding PMMA-ZrO2 particles into P(VDF-HFP) can significantly decrease the crystallinity of the CPE membrane. The CPE membrane doped with 5 wt % PMMA-ZrO2 particles can not only present a homogeneous surface with abundant interconnected micro-pores, but maintain its initial shape after thermal exposure at 160 °C for 1 h, in which the ionic conductivity and lithium ion transference number at room temperature can reach to 3.59 × 10−3 S cm−1 and 0.41, respectively. The fitting results of the EIS plots indicate the doped PMMA-ZrO2 particles can significantly lower the interface resistance and promote lithium ions diffusion rate. The Li/CPE-sPZ/LiCoO2 and Li/CPE-sPZ/Graphite coin cells can deliver excellent rate and cycling performance. Those results suggest the P(VDF-HFP)-based CPE doped with 5 wt % PMMA-ZrO2 particles can become an exciting potential candidate as polymer electrolyte for the lithium ion battery.
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Xiao W. et al. Enhanced performance of P(VDF-HFP)-based composite polymer electrolytes doped with organic-inorganic hybrid particles PMMA-ZrO2 for lithium ion batteries // Journal of Power Sources. 2018. Vol. 382. pp. 128-134.
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Xiao W., WANG Z., Zhang Y., Fang R., Yuan Z., Miao C., Suchanek G., Jiang Yu. Enhanced performance of P(VDF-HFP)-based composite polymer electrolytes doped with organic-inorganic hybrid particles PMMA-ZrO2 for lithium ion batteries // Journal of Power Sources. 2018. Vol. 382. pp. 128-134.
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TY - JOUR
DO - 10.1016/j.jpowsour.2018.02.012
UR - https://linkinghub.elsevier.com/retrieve/pii/S0378775318301162
TI - Enhanced performance of P(VDF-HFP)-based composite polymer electrolytes doped with organic-inorganic hybrid particles PMMA-ZrO2 for lithium ion batteries
T2 - Journal of Power Sources
AU - Xiao, Wei
AU - WANG, ZHIYAN
AU - Zhang, Yan
AU - Fang, Rui
AU - Yuan, Zun
AU - Miao, Chang
AU - Suchanek, Gerry
AU - Jiang, Yu
PY - 2018
DA - 2018/04/01 00:00:00
PB - Elsevier
SP - 128-134
VL - 382
SN - 0378-7753
ER -
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@article{2018_Xiao,
author = {Wei Xiao and ZHIYAN WANG and Yan Zhang and Rui Fang and Zun Yuan and Chang Miao and Gerry Suchanek and Yu Jiang},
title = {Enhanced performance of P(VDF-HFP)-based composite polymer electrolytes doped with organic-inorganic hybrid particles PMMA-ZrO2 for lithium ion batteries},
journal = {Journal of Power Sources},
year = {2018},
volume = {382},
publisher = {Elsevier},
month = {apr},
url = {https://linkinghub.elsevier.com/retrieve/pii/S0378775318301162},
pages = {128--134},
doi = {10.1016/j.jpowsour.2018.02.012}
}