Journal of Power Sources, volume 391, pages 73-79
All-solid-state batteries with slurry coated LiNi0.8Co0.1Mn0.1O2 composite cathode and Li6PS5Cl electrolyte: Effect of binder content
J Zhang
1
,
Jun Zhang
,
Haoyue Zhong
1
,
Chao Zheng
1
,
Chao Zheng
,
Yang Xia
1
,
Liang Chu
,
Chu Liang
1
,
Hui Huang
,
Hui Huang
1
,
Yongping Gan
,
Yongping Gan
1
,
Xinyong Tao
,
Xinyong Tao
1
,
Wenkui Zhang
,
Wenkui Zhang
1
Publication type: Journal Article
Publication date: 2018-07-01
Journal:
Journal of Power Sources
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 9.2
ISSN: 03787753
Physical and Theoretical Chemistry
Electrical and Electronic Engineering
Energy Engineering and Power Technology
Renewable Energy, Sustainability and the Environment
Abstract
The synthesis of solid electrolytes with high ionic conductivity and the design of electrode interface with preferable compatibility are critical to realize the bulk-type application of all-solid-state batteries. In order to realize the superior electrochemical performance, argyrodite Li6PS5Cl is a promising solid electrolyte in all-solid-state batteries due to high ionic conductivity and electrochemical stability. Meanwhile, the solution reprecipitation is a valid process providing intimate ionic contact between electrodes and electrolytes to mitigate the interface incompatibility. Here, a wet-slurry process by dispersing active material (LiNi0.8Co0.1Mn0.1O2), solid electrolyte (Li6PS5Cl), binder (ethyl cellulose) and conductive additives (carbon black) in anhydrous ethanol is developed to fabricate cathode. The effect of different contents of the binder in the composite cathodes on the electrochemical performance is investigated. The all-solid-state battery with a composite cathode containing 1 wt% of ethyl cellulose shows a reversible discharge capacity of 111.7 mAh g−1 at 30 °C and its capacity retention is approximately 89.7% after 100 cycles. This work demonstrates that the fast ion migration and stable interface between active particles and solid electrolyte enabled by optimum content of chemically compatible binder are critical to the electrochemical performance of all-solid-state lithium-ion batteries.
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Citations by publishers
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1 publication, 0.57%
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1 publication, 0.57%
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1 publication, 0.57%
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10
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Zhang J. et al. All-solid-state batteries with slurry coated LiNi0.8Co0.1Mn0.1O2 composite cathode and Li6PS5Cl electrolyte: Effect of binder content // Journal of Power Sources. 2018. Vol. 391. pp. 73-79.
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Zhang J., Zhang J., Zhong H., Zheng C., Zheng C., Xia Y., Chu L., Liang C., Huang H., Huang H., Gan Y., Gan Y., Tao X., Tao X., Zhang W., Zhang W. All-solid-state batteries with slurry coated LiNi0.8Co0.1Mn0.1O2 composite cathode and Li6PS5Cl electrolyte: Effect of binder content // Journal of Power Sources. 2018. Vol. 391. pp. 73-79.
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TY - JOUR
DO - 10.1016/j.jpowsour.2018.04.069
UR - https://doi.org/10.1016/j.jpowsour.2018.04.069
TI - All-solid-state batteries with slurry coated LiNi0.8Co0.1Mn0.1O2 composite cathode and Li6PS5Cl electrolyte: Effect of binder content
T2 - Journal of Power Sources
AU - Zhang, Jun
AU - Zhong, Haoyue
AU - Zheng, Chao
AU - Xia, Yang
AU - Chu, Liang
AU - Huang, Hui
AU - Gan, Yongping
AU - Tao, Xinyong
AU - Zhang, Wenkui
AU - Zhang, J
AU - Zheng, Chao
AU - Liang, Chu
AU - Huang, Hui
AU - Gan, Yongping
AU - Tao, Xinyong
AU - Zhang, Wenkui
PY - 2018
DA - 2018/07/01 00:00:00
PB - Elsevier
SP - 73-79
VL - 391
SN - 0378-7753
ER -
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@article{2018_Zhang,
author = {Jun Zhang and Haoyue Zhong and Chao Zheng and Yang Xia and Liang Chu and Hui Huang and Yongping Gan and Xinyong Tao and Wenkui Zhang and J Zhang and Chao Zheng and Chu Liang and Hui Huang and Yongping Gan and Xinyong Tao and Wenkui Zhang},
title = {All-solid-state batteries with slurry coated LiNi0.8Co0.1Mn0.1O2 composite cathode and Li6PS5Cl electrolyte: Effect of binder content},
journal = {Journal of Power Sources},
year = {2018},
volume = {391},
publisher = {Elsevier},
month = {jul},
url = {https://doi.org/10.1016/j.jpowsour.2018.04.069},
pages = {73--79},
doi = {10.1016/j.jpowsour.2018.04.069}
}