Open Access

Materials and Design

, volume 99 , pages 574-580

Nanosized Sn-MFI zeolite for selective detection of exhaust gases

Siddulu N. Talapaneni ¹

Julien Grand ¹

Sébastien Thomas ¹

Hacan Ali Ahmad ¹

S. Mintova ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Laboratoire Catalyse et Spectrochimie (LCS), ENSICAEN, Université de Caen, CNRS, 6 boulevard du Marechal Juin, 14050 Caen, France |

Publication type: Journal Article

Publication date: 2016-06-01

Elsevier

Materials and Design

scimago Q1

wos Q1

SJR: 1.727

CiteScore: 14.9

Impact factor: 7.9

ISSN: 02641275, 18734197

DOI: 10.1016/j.matdes.2016.03.035

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General Materials Science

Mechanical Engineering

Mechanics of Materials

Abstract

The properties of tin containing MFI type zeolite nanocrystals (Sn-MFI) synthesized under hydrothermal conditions from colloidal suspensions, and further application for selective detection of automotive exhaust gases (CO, CO 2 , NO x ) are reported. The properties of the Sn-MFI nanosized zeolite are compared with the pure silicalite-1 nanocrystals (Si-MFI) synthesized under identical conditions, and used as a reference. Additionally, both samples (Si-MFI and Sn-MFI) with high crystallinity and high porosity were stabilized in coating suspensions and deposited in films by spin-coating approach. The Si-MFI and Sn-MFI samples as self-supported pellets and thin films were exposed to different concentrations of exhaust gases in the presence of 100 ppm of water. The sorption behavior of the Sn-MFI and the Si-MFI towards CO, CO 2 , NO and NO 2 gases was followed by in situ IR spectroscopy. The influence of the tin concentration in the zeolite nanocrystals and the type of assembly (self-supported pellets and films) on the gas detection was studied. The fast detection of NO 2 with the Sn-MFI sample in comparison to the other gases implies that the tin containing zeolite could be considered for further use a selective material for detection of low concentrations of NO 2 (0–20 ppm).

Found

1 citation

Maslakov Konstantin

PhD in Physics and Mathematics

348 publications, 5 688 citations, 35 reviews

h-index: 35

Lomonosov Moscow State University

National Research Centre "Kurchatov Institute"

1 citation

Loktev Alexey

DSc in Chemistry, professor

100 publications, 879 citations, 55 reviews

h-index: 14

Kurnakov Institute of General and Inorganic Chemistry of the Russian Academy of Sciences

A.V. Topchiev Institute of Petrochemical Synthesis RAS

National University of Oil and Gas «Gubkin University»

Lomonosov Moscow State University

1 citation

Cherednichenko Kirill

🥼 🤝

PhD in Chemistry

82 publications, 871 citations, 6 reviews

h-index: 16

National University of Oil and Gas «Gubkin University»

Lomonosov Moscow State University

Hierarchically porous materials

Nanocomposites

Polymer composites

Refractory materials

Scanning electron microscopy

Synchrotron radiation

X-ray diffraction (XRD)

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GOST Copy

Talapaneni S. N. et al. Nanosized Sn-MFI zeolite for selective detection of exhaust gases // Materials and Design. 2016. Vol. 99. pp. 574-580.

GOST all authors (up to 50) Copy

Talapaneni S. N., Grand J., Thomas S., Ali Ahmad H., Mintova S. Nanosized Sn-MFI zeolite for selective detection of exhaust gases // Materials and Design. 2016. Vol. 99. pp. 574-580.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1016/j.matdes.2016.03.035

UR - https://doi.org/10.1016/j.matdes.2016.03.035

TI - Nanosized Sn-MFI zeolite for selective detection of exhaust gases

T2 - Materials and Design

AU - Talapaneni, Siddulu N.

AU - Grand, Julien

AU - Thomas, Sébastien

AU - Ali Ahmad, Hacan

AU - Mintova, S.

PY - 2016

DA - 2016/06/01

PB - Elsevier

SP - 574-580

VL - 99

SN - 0264-1275

SN - 1873-4197

ER -

BibTex

Cite this

BibTex (up to 50 authors) Copy

@article{2016_Talapaneni,

author = {Siddulu N. Talapaneni and Julien Grand and Sébastien Thomas and Hacan Ali Ahmad and S. Mintova},

title = {Nanosized Sn-MFI zeolite for selective detection of exhaust gases},

journal = {Materials and Design},

year = {2016},

volume = {99},

publisher = {Elsevier},

month = {jun},

url = {https://doi.org/10.1016/j.matdes.2016.03.035},

pages = {574--580},

doi = {10.1016/j.matdes.2016.03.035}

}

Publisher

Elsevier

Journal

Materials and Design

scimago Q1

wos Q1

SJR

1.727

CiteScore

14.9

Impact factor

7.9

ISSN

02641275 (Print)

18734197 (Electronic)