Materials Research Bulletin, volume 140, pages 111298

Near-infrared two-photon absorption upconversion of PbS/CdS quantum dots prepared by cation exchange method

Publication typeJournal Article
Publication date2021-08-01
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor5.4
ISSN00255408
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Mechanics of Materials
Abstract
Schematic diagram about the energy band arrangement of the core/shell structures at different stages of the cation exchange reaction. • PbS/CdS QDs with the band alignment changeing from type-I to quasi-type II are prepared via the cation exchange method. • Nonlinear two-photon absorption upconversion luminescence is obtained in quantum dots excited by 1064 nm femtosecond laser. • The long fluorescence lifetime inherited from the PbS core endows PbS/CdS QD a decay lifetime of hundreds of nanoseconds. Taking advantage of multi-photon absorption, the semiconductor quantum dots show great potential in the field of bio-logical fluorescence imaging. In this paper, PbS/CdS core-shell quantum dots with the band alignment adjustable from type-I to quasi-type II are prepared through the cation exchange method. The core-shell quantum dots exhibit bright broad-band visible/near-infrared upconversion emission upon the excitation of 1064 nm pulse laser, and the core-shell QDs hold a decay lifetime of hundreds of nanoseconds. These characteristics enable the present PbS/CdS core-shell quantum dots to be a promising candidate for biomedical fluorescence imaging.

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Cheng L. et al. Near-infrared two-photon absorption upconversion of PbS/CdS quantum dots prepared by cation exchange method // Materials Research Bulletin. 2021. Vol. 140. p. 111298.
GOST all authors (up to 50) Copy
Cheng L., Cheng Y., Xu J. F., Lin H., Wang Y. Near-infrared two-photon absorption upconversion of PbS/CdS quantum dots prepared by cation exchange method // Materials Research Bulletin. 2021. Vol. 140. p. 111298.
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RIS Copy
TY - JOUR
DO - 10.1016/j.materresbull.2021.111298
UR - https://doi.org/10.1016/j.materresbull.2021.111298
TI - Near-infrared two-photon absorption upconversion of PbS/CdS quantum dots prepared by cation exchange method
T2 - Materials Research Bulletin
AU - Cheng, L
AU - Cheng, Yao
AU - Xu, Ju Feng
AU - Lin, Hang
AU - Wang, Yuansheng
PY - 2021
DA - 2021/08/01 00:00:00
PB - Elsevier
SP - 111298
VL - 140
SN - 0025-5408
ER -
BibTex
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BibTex Copy
@article{2021_Cheng,
author = {L Cheng and Yao Cheng and Ju Feng Xu and Hang Lin and Yuansheng Wang},
title = {Near-infrared two-photon absorption upconversion of PbS/CdS quantum dots prepared by cation exchange method},
journal = {Materials Research Bulletin},
year = {2021},
volume = {140},
publisher = {Elsevier},
month = {aug},
url = {https://doi.org/10.1016/j.materresbull.2021.111298},
pages = {111298},
doi = {10.1016/j.materresbull.2021.111298}
}
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