Materials Letters, volume 231, pages 43-46

High lithium ionic conductivity of garnet-type oxide Li7+xLa3Zr2-xSmxO12 (x = 0–0.1) ceramics

Xishu Wang ¹

Jie Liu ¹

Rui Yin ¹

Yichen Xu ¹

Yonghua Cui ¹

Liang Zhao ¹

Xibin Yu ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Education Ministry Key Lab of Resource Chemistry and Shanghai Key Laboratory of Rare Earth Functional Materials Department of Chemistry Shanghai Normal University Shanghai 200234 China |

Publication type: Journal Article

Publication date: 2018-11-01

Elsevier

Journal: Materials Letters

Quartile SCImago

Quartile WOS

Impact factor: 3

ISSN: 0167577X

DOI: 10.1016/j.matlet.2018.08.006

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Condensed Matter Physics

General Materials Science

Mechanical Engineering

Mechanics of Materials

Abstract

Li7La3Zr2O12 (LLZO) garnet is one of the most promising Lithium-ion solid electrolytes in all-solid-state Lithium-ion batteries, due to its higher chemical stability to Li metal and relatively higher lithium-ion conductivity. To further increase the electrical conductivity of LLZO, Sm3+ is doped into the Zr4+ site of LLZO so that excess Li occupies the position of the octahedral. Thereby lithium ion transport and increasing ionic conductivity are promoted. The optimal addition of Sm3+ is 0.06. Li7+xLa3Zr2-xSmxO12 (LLZSO, x = 0.06) electrolyte with cubic phase is obtained with sintering at 1200 °C for only 3 h. It has higher relative density and better ionic conductivity than the pristine LLZO. Its bulk and total ionic conductivity are ∼6.4 × 10−4 S·cm−1 and 2.46 × 10−4 S·cm−1 at 20 °C, respectively.

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American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 3.45% American Institute of Physics (AIP) 1 publication, 3.45%
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Wang X. et al. High lithium ionic conductivity of garnet-type oxide Li7+xLa3Zr2-xSmxO12 (x = 0–0.1) ceramics // Materials Letters. 2018. Vol. 231. pp. 43-46.

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Wang X., Liu J., Yin R., Xu Y., Cui Y., Zhao L., Yu X. High lithium ionic conductivity of garnet-type oxide Li7+xLa3Zr2-xSmxO12 (x = 0–0.1) ceramics // Materials Letters. 2018. Vol. 231. pp. 43-46.

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RIS Copy

TY - JOUR

DO - 10.1016/j.matlet.2018.08.006

UR - https://doi.org/10.1016/j.matlet.2018.08.006

TI - High lithium ionic conductivity of garnet-type oxide Li7+xLa3Zr2-xSmxO12 (x = 0–0.1) ceramics

T2 - Materials Letters

AU - Wang, Xishu

AU - Liu, Jie

AU - Yin, Rui

AU - Xu, Yichen

AU - Cui, Yonghua

AU - Zhao, Liang

AU - Yu, Xibin

PY - 2018

DA - 2018/11/01 00:00:00

PB - Elsevier

SP - 43-46

VL - 231

SN - 0167-577X

ER -

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BibTex Copy

@article{2018_Wang,

author = {Xishu Wang and Jie Liu and Rui Yin and Yichen Xu and Yonghua Cui and Liang Zhao and Xibin Yu},

title = {High lithium ionic conductivity of garnet-type oxide Li7+xLa3Zr2-xSmxO12 (x = 0–0.1) ceramics},

journal = {Materials Letters},

year = {2018},

volume = {231},

publisher = {Elsevier},

month = {nov},

url = {https://doi.org/10.1016/j.matlet.2018.08.006},

pages = {43--46},

doi = {10.1016/j.matlet.2018.08.006}

}

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Elsevier

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Materials Letters

Quartile SCImago

Quartile WOS

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0167577X (Print)