Matter, volume 1, issue 1, pages 250-265

Epitaxial Dimers and Auger-Assisted Detrapping in PbS Quantum Dot Solids

Rachel H. Gilmore ¹

Yun Liu ²

Wenbi Shcherbakov Wu ³

Nabeel S Dahod ¹

Elizabeth M Y Lee ¹

Mark C. Weidman ¹

Hua-Shan Li ²

J. Jean ⁴

Vladimir Bulović ⁴

Adam P. Willard ³

Jeffrey A. Grossman ²

WILLIAM A. TISDALE ¹

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Department of Chemical Engineering Massachusetts Institute of Technology Cambridge MA 02139 USA |

Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, MA, 02139 (USA) |

Department of Chemistry, Massachusetts Institute of Technology , Cambridge, MA, 02139, USA |

⁴

Department of Electrical Engineering and Computer Science, Massachusetts Institute of Technology, Cambridge, MA 02139 (USA) |

Publication type: Journal Article

Publication date: 2019-07-10

Elsevier

Journal: Matter

Quartile SCImago

Quartile WOS

Impact factor: 18.9

ISSN: 25902393, 25902385, 25902385

DOI: 10.1016/j.matt.2019.05.015

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General Materials Science

Abstract

Summary We explore the dynamic interaction of charge carriers between band-edge states and sub-band trap states in PbS quantum dot (QD) solids using time-resolved spectroscopy. In monodisperse arrays of 4- to 5-nm diameter PbS QDs, we observe an optically active trap state ∼100–200 meV below the band edge that occurs at a frequency of 1 in ∼2,500 QDs. Uncoupled QD solids with oleic acid ligands show trap-to-ground-state recombination that resembles Auger recombination. In electronically coupled QD solids, we observe entropically driven uphill thermalization of trapped charge carriers from the trap state to the band edge via two distinct mechanisms: Auger-assisted charge transfer (∼35 ps) and thermally activated hopping (∼500 ps). Photophysical characterization combined with atomistic simulations and high-resolution electron microscopy suggest that these states arise from epitaxially fused pairs of QDs rather than electron or hole traps at the QD surface, offering new strategies for improving the optoelectronic performance of QD materials.

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ACS applied materials & interfaces	ACS applied materials & interfaces, 5, 8.2% ACS applied materials & interfaces 5 publications, 8.2%
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Nature Communications	Nature Communications, 3, 4.92% Nature Communications 3 publications, 4.92%
Advanced Materials	Advanced Materials, 3, 4.92% Advanced Materials 3 publications, 4.92%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 3, 4.92% Journal of Physical Chemistry Letters 3 publications, 4.92%
ACS Applied Electronic Materials	ACS Applied Electronic Materials, 3, 4.92% ACS Applied Electronic Materials 3 publications, 4.92%
Chemistry of Materials	Chemistry of Materials, 2, 3.28% Chemistry of Materials 2 publications, 3.28%
ACS Nano	ACS Nano, 2, 3.28% ACS Nano 2 publications, 3.28%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 2, 3.28% Journal of Physical Chemistry C 2 publications, 3.28%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 2, 3.28% Journal of Materials Chemistry A 2 publications, 3.28%
Journal of Chemical Physics	Journal of Chemical Physics, 1, 1.64% Journal of Chemical Physics 1 publication, 1.64%
Applied Physics Reviews	Applied Physics Reviews, 1, 1.64% Applied Physics Reviews 1 publication, 1.64%
Optical and Quantum Electronics	Optical and Quantum Electronics, 1, 1.64% Optical and Quantum Electronics 1 publication, 1.64%
Nature Photonics	Nature Photonics, 1, 1.64% Nature Photonics 1 publication, 1.64%
Matter	Matter, 1, 1.64% Matter 1 publication, 1.64%
Nano Research	Nano Research, 1, 1.64% Nano Research 1 publication, 1.64%
Chem	Chem, 1, 1.64% Chem 1 publication, 1.64%
Joule	Joule, 1, 1.64% Joule 1 publication, 1.64%
Advanced Functional Materials	Advanced Functional Materials, 1, 1.64% Advanced Functional Materials 1 publication, 1.64%
Chemistry - An Asian Journal	Chemistry - An Asian Journal, 1, 1.64% Chemistry - An Asian Journal 1 publication, 1.64%
Advanced Science	Advanced Science, 1, 1.64% Advanced Science 1 publication, 1.64%
ACS Applied Energy Materials	ACS Applied Energy Materials, 1, 1.64% ACS Applied Energy Materials 1 publication, 1.64%
Accounts of Chemical Research	Accounts of Chemical Research, 1, 1.64% Accounts of Chemical Research 1 publication, 1.64%
ACS Energy Letters	ACS Energy Letters, 1, 1.64% ACS Energy Letters 1 publication, 1.64%
Physical Review Applied	Physical Review Applied, 1, 1.64% Physical Review Applied 1 publication, 1.64%
Chemical Science	Chemical Science, 1, 1.64% Chemical Science 1 publication, 1.64%
Energy and Environmental Science	Energy and Environmental Science, 1, 1.64% Energy and Environmental Science 1 publication, 1.64%
Nanoscale Horizons	Nanoscale Horizons, 1, 1.64% Nanoscale Horizons 1 publication, 1.64%
Chemical Society Reviews	Chemical Society Reviews, 1, 1.64% Chemical Society Reviews 1 publication, 1.64%
Science	Science, 1, 1.64% Science 1 publication, 1.64%
	1 2 3 4 5

Citations by publishers

	5 10 15 20 25
American Chemical Society (ACS)	American Chemical Society (ACS), 25, 40.98% American Chemical Society (ACS) 25 publications, 40.98%
Wiley	Wiley, 8, 13.11% Wiley 8 publications, 13.11%
Elsevier	Elsevier, 7, 11.48% Elsevier 7 publications, 11.48%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 7, 11.48% Royal Society of Chemistry (RSC) 7 publications, 11.48%
Springer Nature	Springer Nature, 6, 9.84% Springer Nature 6 publications, 9.84%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 3.28% American Institute of Physics (AIP) 2 publications, 3.28%
American Physical Society (APS)	American Physical Society (APS), 1, 1.64% American Physical Society (APS) 1 publication, 1.64%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 1.64% American Association for the Advancement of Science (AAAS) 1 publication, 1.64%
Pleiades Publishing	Pleiades Publishing, 1, 1.64% Pleiades Publishing 1 publication, 1.64%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.64% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.64%
IOP Publishing	IOP Publishing, 1, 1.64% IOP Publishing 1 publication, 1.64%
	5 10 15 20 25

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Gilmore R. H. et al. Epitaxial Dimers and Auger-Assisted Detrapping in PbS Quantum Dot Solids // Matter. 2019. Vol. 1. No. 1. pp. 250-265.

GOST all authors (up to 50) Copy

Gilmore R. H., Liu Y., Shcherbakov Wu W., Dahod N. S., Lee E. M. Y., Weidman M. C., Li H., Jean J., Bulović V., Willard A. P., Grossman J. A., TISDALE W. A. Epitaxial Dimers and Auger-Assisted Detrapping in PbS Quantum Dot Solids // Matter. 2019. Vol. 1. No. 1. pp. 250-265.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.matt.2019.05.015

UR - https://doi.org/10.1016/j.matt.2019.05.015

TI - Epitaxial Dimers and Auger-Assisted Detrapping in PbS Quantum Dot Solids

T2 - Matter

AU - Gilmore, Rachel H.

AU - Liu, Yun

AU - Shcherbakov Wu, Wenbi

AU - Dahod, Nabeel S

AU - Lee, Elizabeth M Y

AU - Weidman, Mark C.

AU - Li, Hua-Shan

AU - Jean, J.

AU - Bulović, Vladimir

AU - Willard, Adam P.

AU - Grossman, Jeffrey A.

AU - TISDALE, WILLIAM A.

PY - 2019

DA - 2019/07/10 00:00:00

PB - Elsevier

SP - 250-265

IS - 1

VL - 1

SN - 2590-2393

SN - 2590-2385

ER -

BibTex |

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BibTex Copy

@article{2019_Gilmore,

author = {Rachel H. Gilmore and Yun Liu and Wenbi Shcherbakov Wu and Nabeel S Dahod and Elizabeth M Y Lee and Mark C. Weidman and Hua-Shan Li and J. Jean and Vladimir Bulović and Adam P. Willard and Jeffrey A. Grossman and WILLIAM A. TISDALE},

title = {Epitaxial Dimers and Auger-Assisted Detrapping in PbS Quantum Dot Solids},

journal = {Matter},

year = {2019},

volume = {1},

publisher = {Elsevier},

month = {jul},

url = {https://doi.org/10.1016/j.matt.2019.05.015},

number = {1},

pages = {250--265},

doi = {10.1016/j.matt.2019.05.015}

}

MLA

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MLA Copy

Gilmore, Rachel H., et al. “Epitaxial Dimers and Auger-Assisted Detrapping in PbS Quantum Dot Solids.” Matter, vol. 1, no. 1, Jul. 2019, pp. 250-265. https://doi.org/10.1016/j.matt.2019.05.015.

Found error?

Publisher

Elsevier

Journal

Matter

Quartile SCImago

Quartile WOS

Impact factor

18.9

ISSN

25902393 (Print)
25902385 (Electronic)
25902385 (Print)