Effects arising from the replacement of aprotic dipolar solvents with ionic liquids in the nickel-catalyzed reduction of aryl chlorides
Publication type: Journal Article
Publication date: 2018-12-01
scimago Q1
wos Q2
SJR: 0.878
CiteScore: 7.2
Impact factor: 4.9
ISSN: 24688231
Catalysis
Physical and Theoretical Chemistry
Process Chemistry and Technology
Abstract
In the work on the example of liquid-phase catalytic processes of the aromatic C Cl bonds activation occurring in the presence of nickel complexes under reducing conditions the main effects arising from the replacement of aprotic dipolar solvents with ionic liquids are analyzed. The features of the nickel-catalyzed reaction of aryl chlorides, related to the nature of the anion and cation of the ionic liquid, were observed. It was shown that a high concentration of cations and anions in the ionic liquid affects the process of reduction of the nickel complex to the catalytically active state. In addition, the presence of a reactive hydrogen atom in the imidazolium cation of ionic liquid causes the process of hydrodechlorination of aryl chlorides.
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Prikhodko S. A. et al. Effects arising from the replacement of aprotic dipolar solvents with ionic liquids in the nickel-catalyzed reduction of aryl chlorides // Molecular Catalysis. 2018. Vol. 461. pp. 19-25.
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Prikhodko S. A., Popov A., Adonin N. Effects arising from the replacement of aprotic dipolar solvents with ionic liquids in the nickel-catalyzed reduction of aryl chlorides // Molecular Catalysis. 2018. Vol. 461. pp. 19-25.
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TY - JOUR
DO - 10.1016/j.mcat.2018.09.022
UR - https://doi.org/10.1016/j.mcat.2018.09.022
TI - Effects arising from the replacement of aprotic dipolar solvents with ionic liquids in the nickel-catalyzed reduction of aryl chlorides
T2 - Molecular Catalysis
AU - Prikhodko, Sergey A
AU - Popov, A.G.
AU - Adonin, N.Yu.
PY - 2018
DA - 2018/12/01
PB - Elsevier
SP - 19-25
VL - 461
SN - 2468-8231
ER -
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@article{2018_Prikhodko,
author = {Sergey A Prikhodko and A.G. Popov and N.Yu. Adonin},
title = {Effects arising from the replacement of aprotic dipolar solvents with ionic liquids in the nickel-catalyzed reduction of aryl chlorides},
journal = {Molecular Catalysis},
year = {2018},
volume = {461},
publisher = {Elsevier},
month = {dec},
url = {https://doi.org/10.1016/j.mcat.2018.09.022},
pages = {19--25},
doi = {10.1016/j.mcat.2018.09.022}
}