Reduced coke formation during the gas phase oxidative dehydration of glycerol over ferrierite zeolites synthesized in fluoride medium
Publication type: Journal Article
Publication date: 2016-03-01
scimago Q1
wos Q2
SJR: 1.003
CiteScore: 11.0
Impact factor: 4.7
ISSN: 13871811, 18733093
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanics of Materials
Abstract
Ferrierite zeolites were synthesized in fluoride medium with SiO 2 /Al 2 O 3 molar ratios 18, 22 and 37, using n-butylamine and pyridine as structure directing agents. The use of fluoride medium as mineralizing agent resulted in the formation of large crystals with morphology quite different from those obtained in hydroxide medium. These materials were characterized and evaluated in the gas-phase catalytic oxidative dehydration of glycerol at 300 °C, using air as carrier gas. Despite a low density of acid sites, the catalysts synthesized in fluoride medium led to high glycerol conversions and acrolein selectivities. Furthermore, coke formation was lower than that observed over the ferrierite synthesized in hydroxide medium.
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Total citations:
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Citations from 2025:
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Dos Santos M. B., Andrade H. M. C., Mascarenhas A. Reduced coke formation during the gas phase oxidative dehydration of glycerol over ferrierite zeolites synthesized in fluoride medium // Microporous and Mesoporous Materials. 2016. Vol. 223. pp. 105-113.
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Dos Santos M. B., Andrade H. M. C., Mascarenhas A. Reduced coke formation during the gas phase oxidative dehydration of glycerol over ferrierite zeolites synthesized in fluoride medium // Microporous and Mesoporous Materials. 2016. Vol. 223. pp. 105-113.
Cite this
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TY - JOUR
DO - 10.1016/j.micromeso.2015.10.040
UR - https://doi.org/10.1016/j.micromeso.2015.10.040
TI - Reduced coke formation during the gas phase oxidative dehydration of glycerol over ferrierite zeolites synthesized in fluoride medium
T2 - Microporous and Mesoporous Materials
AU - Dos Santos, Maurício B
AU - Andrade, Heloysa M C
AU - Mascarenhas, Artur
PY - 2016
DA - 2016/03/01
PB - Elsevier
SP - 105-113
VL - 223
SN - 1387-1811
SN - 1873-3093
ER -
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@article{2016_Dos Santos,
author = {Maurício B Dos Santos and Heloysa M C Andrade and Artur Mascarenhas},
title = {Reduced coke formation during the gas phase oxidative dehydration of glycerol over ferrierite zeolites synthesized in fluoride medium},
journal = {Microporous and Mesoporous Materials},
year = {2016},
volume = {223},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016/j.micromeso.2015.10.040},
pages = {105--113},
doi = {10.1016/j.micromeso.2015.10.040}
}