Highly nanodispersed Gd-doped Ni/ZSM-5 catalyst for enhanced carbon-resistant dry reforming of methane
Publication type: Journal Article
Publication date: 2016-12-01
SJR: —
CiteScore: —
Impact factor: —
ISSN: 13811169
Catalysis
Physical and Theoretical Chemistry
Process Chemistry and Technology
Abstract
Gd-promoted mesoporous Ni/ZSM-5 (GdNi/ZSM-5) catalysts was prepared and evaluated in the dry reforming of methane. Addition of Gd forms GdNi5 alloy on the ZSM-5 support; the particle size of GdNi5 species supported on mesoporous ZSM-5 was found to be in the range of 2–10 nm. The addition of Gd enables superior mass transfer of reactants and products while preventing the agglomeration of the Ni nanoparticles. The presence of Gd supplies the oxygen atom to neighbouring Ni site, which oxidize the accumulated coke on Ni sites. Gd promoted Ni/ZSM-5 catalyst can work till 100 h without any deactivation. Ni/ZSM-5 catalyst (without promoter) shows severe deactivation due to the sintering of Ni nanoparticles during reforming reaction.
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45
Total citations:
45
Citations from 2025:
4
(8.89%)
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GOST
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Sarkar B. et al. Highly nanodispersed Gd-doped Ni/ZSM-5 catalyst for enhanced carbon-resistant dry reforming of methane // Journal of Molecular Catalysis A Chemical. 2016. Vol. 424. pp. 17-26.
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Sarkar B., Goyal R., Pendem C., Sasaki T., Bal R. Highly nanodispersed Gd-doped Ni/ZSM-5 catalyst for enhanced carbon-resistant dry reforming of methane // Journal of Molecular Catalysis A Chemical. 2016. Vol. 424. pp. 17-26.
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TY - JOUR
DO - 10.1016/j.molcata.2016.08.006
UR - https://linkinghub.elsevier.com/retrieve/pii/S1381116916303284
TI - Highly nanodispersed Gd-doped Ni/ZSM-5 catalyst for enhanced carbon-resistant dry reforming of methane
T2 - Journal of Molecular Catalysis A Chemical
AU - Sarkar, Bipul
AU - Goyal, Reena
AU - Pendem, Chandrashekar
AU - Sasaki, Takehiko
AU - Bal, Rajaram
PY - 2016
DA - 2016/12/01
PB - Elsevier
SP - 17-26
VL - 424
SN - 1381-1169
ER -
Cite this
BibTex (up to 50 authors)
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@article{2016_Sarkar,
author = {Bipul Sarkar and Reena Goyal and Chandrashekar Pendem and Takehiko Sasaki and Rajaram Bal},
title = {Highly nanodispersed Gd-doped Ni/ZSM-5 catalyst for enhanced carbon-resistant dry reforming of methane},
journal = {Journal of Molecular Catalysis A Chemical},
year = {2016},
volume = {424},
publisher = {Elsevier},
month = {dec},
url = {https://linkinghub.elsevier.com/retrieve/pii/S1381116916303284},
pages = {17--26},
doi = {10.1016/j.molcata.2016.08.006}
}