Materials Today Energy, volume 23, pages 100904

Layered g-C3N4/TiO2 nanocomposites for efficient photocatalytic water splitting and CO2 reduction: a review

Publication typeJournal Article
Publication date2022-01-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor9.3
ISSN24686069, 24686069
Materials Science (miscellaneous)
Energy Engineering and Power Technology
Fuel Technology
Nuclear Energy and Engineering
Renewable Energy, Sustainability and the Environment
Abstract
Solar-driven photocatalysts for water splitting and CO 2 reduction have been widely studied for dealing with environmental pollution and energy sustainability issues. Among the most promising semiconductor photocatalysts, graphitic carbon nitride (g-C 3 N 4 ) and TiO 2 (anatase) with band gaps of ∼2.7 and ∼3.2 eV, respectively, are investigated extensively. However, the high photogenerated carrier recombination efficiency of g-C 3 N 4 and the relatively wide band gap of TiO 2 (responsive to ultraviolet light only) are the factors that can lower the photocatalytic activities of the materials. Thus, one of the prevalent strategies is to construct g-C 3 N 4 /TiO 2 nanocomposites to promote charge carrier separation and to improve photoabsorption in the visible region for attaining efficient utilization of solar energy in photocatalytic water splitting, CO 2 reduction, and organic pollutant photodegradation. Here, a comprehensive overview is made on the exploitation of g-C 3 N 4 /TiO 2 nanocomposites for photocatalytic applications, emphasizing layered heterostructures, for solar-driven H 2 generation and CO 2 reduction. Challenges in resolving various issues such as low efficiency, low stability, and noble metal cocatalyst dependency, as well as band gap narrowing accompanied reduction in redox ability of the g-C 3 N 4 /TiO 2 nanocomposites, are discussed. • Layered g-C 3 N 4 /TiO 2 nanocomposites for photocatalytic water splitting and CO 2 reduction are reviewed. • g-C 3 N 4 /TiO 2 heterostructure-based catalysts with various dimensions are extensively explored. • Kinetics and mechanism of photocatalysis of g-C 3 N 4 /TiO 2 nanocomposites are described. • Challenging issues associated with high efficiency and durability of the system are discussed.

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Zhang X., Jiang S. P. Layered g-C3N4/TiO2 nanocomposites for efficient photocatalytic water splitting and CO2 reduction: a review // Materials Today Energy. 2022. Vol. 23. p. 100904.
GOST all authors (up to 50) Copy
Zhang X., Jiang S. P. Layered g-C3N4/TiO2 nanocomposites for efficient photocatalytic water splitting and CO2 reduction: a review // Materials Today Energy. 2022. Vol. 23. p. 100904.
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RIS Copy
TY - JOUR
DO - 10.1016/j.mtener.2021.100904
UR - https://doi.org/10.1016/j.mtener.2021.100904
TI - Layered g-C3N4/TiO2 nanocomposites for efficient photocatalytic water splitting and CO2 reduction: a review
T2 - Materials Today Energy
AU - Zhang, Xiao
AU - Jiang, San Ping
PY - 2022
DA - 2022/01/01 00:00:00
PB - Elsevier
SP - 100904
VL - 23
SN - 2468-6069
SN - 2468-6069
ER -
BibTex
Cite this
BibTex Copy
@article{2022_Zhang,
author = {Xiao Zhang and San Ping Jiang},
title = {Layered g-C3N4/TiO2 nanocomposites for efficient photocatalytic water splitting and CO2 reduction: a review},
journal = {Materials Today Energy},
year = {2022},
volume = {23},
publisher = {Elsevier},
month = {jan},
url = {https://doi.org/10.1016/j.mtener.2021.100904},
pages = {100904},
doi = {10.1016/j.mtener.2021.100904}
}
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