Materials Today Nano, volume 8, pages 100048

Liquid-involved synthesis and processing of sulfide-based solid electrolytes, electrodes, and all-solid-state batteries

Jianbin Xu ¹

L. Liu ²

N. Yao ³

F. Wu ⁴

Hui Li ⁴

Lixin Chen ⁴

Hide authors affiliations Show authors affiliations: 4 affiliations

Key Laboratory for Renewable Energy, Beijing Key Laboratory for New Energy Materials and Devices, Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China. |

Tianmu Lake Institute of Advanced Energy Storage Technologies, Liyang, 213300, China |

Princeton Institute for the Science and Technology of Materials (PRISM), Princeton University, 70 Prospect Avenue, Princeton, NJ 08540, USA |

⁴

Publication type: Journal Article

Publication date: 2019-12-01

Elsevier

Journal: Materials Today Nano

Quartile SCImago

Quartile WOS

Impact factor: 10.3

ISSN: 25888420, 25888420

DOI: 10.1016/j.mtnano.2019.100048

Copy DOI

Materials Chemistry

Electronic, Optical and Magnetic Materials

Condensed Matter Physics

Biomaterials

Abstract

Solid-state battery has been widely accepted as the next-generation energy-storage technology because of its better safety and potentially higher energy density. Solid electrolyte plays the most critical role in its performance, among which sulfides show the highest lithium-ion conductivities. To realize the mass production and practical application of sulfide-based electrolytes and all-solid-state batteries, one of the most promising methods is by in-situ solidification of sulfide–electrolyte solution/slurries with liquid-involved processing that can be performed in controlled atmosphere with low temperature. This enables wet coating process for electrolyte/electrode layer formation and thus opens up the possibility of mass production of sulfide solid-state batteries. In this review, liquid-involved process is carefully classified into liquid-phase synthesis, solution, and slurry process with clear definition to avoid any confusion among these different processes. The liquid-involved processes of sulfide solid electrolytes themselves on material level, sulfide-based composite electrolytes/electrodes on component level, and sulfide-based all-solid-state batteries on device level are summarized and discussed in details. Strategies to design and prepare solid sulfide-based electrolytes/electrode layers and batteries with liquid-involved process are also suggested.

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Elsevier	Elsevier, 20, 32.26% Elsevier 20 publications, 32.26%
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Xu J. et al. Liquid-involved synthesis and processing of sulfide-based solid electrolytes, electrodes, and all-solid-state batteries // Materials Today Nano. 2019. Vol. 8. p. 100048.

GOST all authors (up to 50) Copy

Xu J., Liu L., Yao N., Wu F., Li H., Chen L. Liquid-involved synthesis and processing of sulfide-based solid electrolytes, electrodes, and all-solid-state batteries // Materials Today Nano. 2019. Vol. 8. p. 100048.

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RIS Copy

TY - JOUR

DO - 10.1016/j.mtnano.2019.100048

UR - https://doi.org/10.1016/j.mtnano.2019.100048

TI - Liquid-involved synthesis and processing of sulfide-based solid electrolytes, electrodes, and all-solid-state batteries

T2 - Materials Today Nano

AU - Xu, Jianbin

AU - Liu, L.

AU - Yao, N.

AU - Wu, F.

AU - Li, Hui

AU - Chen, Lixin

PY - 2019

DA - 2019/12/01 00:00:00

PB - Elsevier

SP - 100048

VL - 8

SN - 2588-8420

ER -

BibTex

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BibTex Copy

@article{2019_Xu,

author = {Jianbin Xu and L. Liu and N. Yao and F. Wu and Hui Li and Lixin Chen},

title = {Liquid-involved synthesis and processing of sulfide-based solid electrolytes, electrodes, and all-solid-state batteries},

journal = {Materials Today Nano},

year = {2019},

volume = {8},

publisher = {Elsevier},

month = {dec},

url = {https://doi.org/10.1016/j.mtnano.2019.100048},

pages = {100048},

doi = {10.1016/j.mtnano.2019.100048}

}

Found error?

Publisher

Elsevier

Journal

Materials Today Nano

Quartile SCImago

Quartile WOS

Impact factor

10.3

ISSN

25888420 (Electronic)
25888420 (Print)