Nano Energy, volume 46, pages 176-184

PEO/garnet composite electrolytes for solid-state lithium batteries: From “ceramic-in-polymer” to “polymer-in-ceramic”

Long Chen ¹

Yutao Li ²

Shuai Peng Li ¹

Li-Zhen Fan ^{3, 4}

Ce Wen Nan ⁵

John Goodenough ²

Hide authors affiliations Show authors affiliations: 5 affiliations

Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Advanced Materials and Technology, University of Science and Technology Beijing, Beijing 100083, China. |

Materials Science & Engineering Program and Texas Materials Institute, The University of Texas at Austin, Austin, TX 78712, United States |

Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Advanced Materials and Technology, University of Science and Technology Beijing, Beijing 100083, China |

⁴

Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin, TX 78712, United States |

⁵

School of Materials Science and Engineering, Tsinghua University,Beijing 100084,China |

Publication type: Journal Article

Publication date: 2018-04-01

Elsevier

Journal: Nano Energy

Quartile SCImago

Quartile WOS

Impact factor: 17.6

ISSN: 22112855

DOI: 10.1016/j.nanoen.2017.12.037

Copy DOI

General Materials Science

Electrical and Electronic Engineering

Renewable Energy, Sustainability and the Environment

Abstract

Composite polyethylene-oxide/garnet electrolytes containing LiTFSI as the lithium salt have a Li+ conductivity σLi > 10−4 S cm−1 at 55 °C and a low plating/stripping impedance of a dendrite-free Li-metal anode; they have been developed for a safe solid-state Li-metal rechargeable battery. Composites consisting of “ceramic-in-polymer” to “polymer-in-ceramic” that are flexible and mechanically robust are fabricated by hot-pressing. Safe pouch cells with a remarkable flexibility have been fabricated. Solid-state LiFePO4|Li batteries with electrolytes of “ceramic-in-polymer” and “polymer-in-ceramic” deliver excellent cycling stability with high discharge capacities (139.1 mAh g–1 with capacity retention of 93.6% after 100 cycles) and high capacity retention (103.6% with coulombic efficiency of 100% after 50 cycles) at 0.2 C and 55 °C. Both kinds of electrolytes can be applied to solid-state lithium batteries.

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Citations by journals

	10 20 30 40 50 60 70
Energy Storage Materials	Energy Storage Materials, 65, 6.06% Energy Storage Materials 65 publications, 6.06%
ACS applied materials & interfaces	ACS applied materials & interfaces, 61, 5.68% ACS applied materials & interfaces 61 publications, 5.68%
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Advanced Energy Materials	Advanced Energy Materials, 39, 3.63% Advanced Energy Materials 39 publications, 3.63%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 38, 3.54% Journal of Materials Chemistry A 38 publications, 3.54%
Chemical Engineering Journal	Chemical Engineering Journal, 35, 3.26% Chemical Engineering Journal 35 publications, 3.26%
ACS Applied Energy Materials	ACS Applied Energy Materials, 31, 2.89% ACS Applied Energy Materials 31 publications, 2.89%
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Advanced Functional Materials	Advanced Functional Materials, 23, 2.14% Advanced Functional Materials 23 publications, 2.14%
Small	Small, 22, 2.05% Small 22 publications, 2.05%
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Journal of Energy Storage	Journal of Energy Storage, 19, 1.77% Journal of Energy Storage 19 publications, 1.77%
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Journal of the Electrochemical Society	Journal of the Electrochemical Society, 18, 1.68% Journal of the Electrochemical Society 18 publications, 1.68%
Advanced Materials	Advanced Materials, 16, 1.49% Advanced Materials 16 publications, 1.49%
Advanced Science	Advanced Science, 15, 1.4% Advanced Science 15 publications, 1.4%
Journal of Membrane Science	Journal of Membrane Science, 15, 1.4% Journal of Membrane Science 15 publications, 1.4%
ACS Energy Letters	ACS Energy Letters, 14, 1.3% ACS Energy Letters 14 publications, 1.3%
Ionics	Ionics, 13, 1.21% Ionics 13 publications, 1.21%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 12, 1.12% Journal of Alloys and Compounds 12 publications, 1.12%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 11, 1.03% Journal of Colloid and Interface Science 11 publications, 1.03%
Angewandte Chemie	Angewandte Chemie, 11, 1.03% Angewandte Chemie 11 publications, 1.03%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 11, 1.03% Angewandte Chemie - International Edition 11 publications, 1.03%
Energy and Environmental Science	Energy and Environmental Science, 11, 1.03% Energy and Environmental Science 11 publications, 1.03%
Batteries	Batteries, 10, 0.93% Batteries 10 publications, 0.93%
Nano Research	Nano Research, 9, 0.84% Nano Research 9 publications, 0.84%
ACS Sustainable Chemistry and Engineering	ACS Sustainable Chemistry and Engineering, 9, 0.84% ACS Sustainable Chemistry and Engineering 9 publications, 0.84%
Materials Chemistry Frontiers	Materials Chemistry Frontiers, 9, 0.84% Materials Chemistry Frontiers 9 publications, 0.84%
	10 20 30 40 50 60 70

Citations by publishers

	50 100 150 200 250 300 350 400 450
Elsevier	Elsevier, 402, 37.47% Elsevier 402 publications, 37.47%
Wiley	Wiley, 220, 20.5% Wiley 220 publications, 20.5%
American Chemical Society (ACS)	American Chemical Society (ACS), 161, 15% American Chemical Society (ACS) 161 publications, 15%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 105, 9.79% Royal Society of Chemistry (RSC) 105 publications, 9.79%
Springer Nature	Springer Nature, 64, 5.96% Springer Nature 64 publications, 5.96%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 34, 3.17% Multidisciplinary Digital Publishing Institute (MDPI) 34 publications, 3.17%
The Electrochemical Society	The Electrochemical Society, 18, 1.68% The Electrochemical Society 18 publications, 1.68%
IOP Publishing	IOP Publishing, 10, 0.93% IOP Publishing 10 publications, 0.93%
Frontiers Media S.A.	Frontiers Media S.A., 7, 0.65% Frontiers Media S.A. 7 publications, 0.65%
OAE Publishing Inc.	OAE Publishing Inc., 5, 0.47% OAE Publishing Inc. 5 publications, 0.47%
World Scientific	World Scientific, 4, 0.37% World Scientific 4 publications, 0.37%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 4, 0.37% Nonferrous Metals Society of China 4 publications, 0.37%
Chinese Ceramic Society	Chinese Ceramic Society, 4, 0.37% Chinese Ceramic Society 4 publications, 0.37%
Chinese Physical Society	Chinese Physical Society, 3, 0.28% Chinese Physical Society 3 publications, 0.28%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 2, 0.19% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 2 publications, 0.19%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 0.19% American Institute of Physics (AIP) 2 publications, 0.19%
Bentham Science	Bentham Science, 2, 0.19% Bentham Science 2 publications, 0.19%
Tsinghua University Press	Tsinghua University Press, 2, 0.19% Tsinghua University Press 2 publications, 0.19%
University of Science and Technology Beijing	University of Science and Technology Beijing, 2, 0.19% University of Science and Technology Beijing 2 publications, 0.19%
Materials Research Society	Materials Research Society, 2, 0.19% Materials Research Society 2 publications, 0.19%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 2, 0.19% Korean Society of Industrial Engineering Chemistry 2 publications, 0.19%
Oxford University Press	Oxford University Press, 2, 0.19% Oxford University Press 2 publications, 0.19%
Chemical Industry Press	Chemical Industry Press, 1, 0.09% Chemical Industry Press 1 publication, 0.09%
Walter de Gruyter	Walter de Gruyter, 1, 0.09% Walter de Gruyter 1 publication, 0.09%
The Korean Electrochemical Society	The Korean Electrochemical Society, 1, 0.09% The Korean Electrochemical Society 1 publication, 0.09%
Shanghai Institute of Ceramics	Shanghai Institute of Ceramics, 1, 0.09% Shanghai Institute of Ceramics 1 publication, 0.09%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 0.09% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 0.09%
Oriental Scientific Publishing Company	Oriental Scientific Publishing Company, 1, 0.09% Oriental Scientific Publishing Company 1 publication, 0.09%
Hans Publishers	Hans Publishers, 1, 0.09% Hans Publishers 1 publication, 0.09%
	50 100 150 200 250 300 350 400 450

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Chen L. et al. PEO/garnet composite electrolytes for solid-state lithium batteries: From “ceramic-in-polymer” to “polymer-in-ceramic” // Nano Energy. 2018. Vol. 46. pp. 176-184.

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Chen L., Li Y., Li S. P., Fan L., Nan C. W., Goodenough J. PEO/garnet composite electrolytes for solid-state lithium batteries: From “ceramic-in-polymer” to “polymer-in-ceramic” // Nano Energy. 2018. Vol. 46. pp. 176-184.

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RIS Copy

TY - JOUR

DO - 10.1016/j.nanoen.2017.12.037

UR - https://linkinghub.elsevier.com/retrieve/pii/S2211285517308133

TI - PEO/garnet composite electrolytes for solid-state lithium batteries: From “ceramic-in-polymer” to “polymer-in-ceramic”

T2 - Nano Energy

AU - Chen, Long

AU - Li, Yutao

AU - Li, Shuai Peng

AU - Fan, Li-Zhen

AU - Nan, Ce Wen

AU - Goodenough, John

PY - 2018

DA - 2018/04/01 00:00:00

PB - Elsevier

SP - 176-184

VL - 46

SN - 2211-2855

ER -

BibTex

Cite this

BibTex Copy

@article{2018_Chen,

author = {Long Chen and Yutao Li and Shuai Peng Li and Li-Zhen Fan and Ce Wen Nan and John Goodenough},

title = {PEO/garnet composite electrolytes for solid-state lithium batteries: From “ceramic-in-polymer” to “polymer-in-ceramic”},

journal = {Nano Energy},

year = {2018},

volume = {46},

publisher = {Elsevier},

month = {apr},

url = {https://linkinghub.elsevier.com/retrieve/pii/S2211285517308133},

pages = {176--184},

doi = {10.1016/j.nanoen.2017.12.037}

}

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Publisher

Elsevier

Journal

Nano Energy

Quartile SCImago

Quartile WOS

Impact factor

17.6

ISSN

22112855 (Print)