Nano Energy, volume 62, pages 55-63
Entrapping lithium deposition in lithiophilic reservoir constructed by vertically aligned ZnO nanosheets for dendrite-free Li metal anodes
Publication type: Journal Article
Publication date: 2019-08-01
General Materials Science
Electrical and Electronic Engineering
Renewable Energy, Sustainability and the Environment
Abstract
The safety issue and poor stability induced by dendrite growth and volume change present major barriers to the practical application of lithium-metal anode for next-generation high-energy-density batteries. Herein, we propose vertically aligned ZnO nanosheets derived from zinc-based MOF grown on Ni foam (LZNF) as a lithiophilic porous scaffold to mitigate these problems. The interspace between the cross-linked ZnO nanosheets as the lithiophilic reservoir enables homogenous plating/stripping of Li at a high deposition capacity of 15 mAh cm-2, which is difficult to realize on Ni foam substrate decorated with normal ZnO particles. The integration of vertically aligned ZnO nanosheets and 3D conductive Ni foam can not only induce dendrite-free lithium deposition with reduced current density but also alleviate the volume fluctuations of lithium. Consequently, a high Coulombic efficiency in LZNF/Li half-cell (98.5% for 150 cycles at 1 mA cm-2) and enhanced cycling stability of a symmetric LZNF@Li/LZNF@Li cell (5 mA cm-2 for 250 cycles) with a small voltage hysteresis (45 mV) can be achieved. Our investigation shows that LZNF can serve as a promising multi-functional 3D host for dendrite-free Li metal anodes.
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- We do not take into account publications without a DOI.
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- Statistics recalculated weekly.
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Zhao F. et al. Entrapping lithium deposition in lithiophilic reservoir constructed by vertically aligned ZnO nanosheets for dendrite-free Li metal anodes // Nano Energy. 2019. Vol. 62. pp. 55-63.
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Zhao F., Zhou X., Deng W., Liu Z. Entrapping lithium deposition in lithiophilic reservoir constructed by vertically aligned ZnO nanosheets for dendrite-free Li metal anodes // Nano Energy. 2019. Vol. 62. pp. 55-63.
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TY - JOUR
DO - 10.1016/j.nanoen.2019.04.087
UR - https://doi.org/10.1016/j.nanoen.2019.04.087
TI - Entrapping lithium deposition in lithiophilic reservoir constructed by vertically aligned ZnO nanosheets for dendrite-free Li metal anodes
T2 - Nano Energy
AU - Zhao, Fei
AU - Zhou, Xu-Feng
AU - Deng, Wei
AU - Liu, Zhaoping
PY - 2019
DA - 2019/08/01 00:00:00
PB - Elsevier
SP - 55-63
VL - 62
SN - 2211-2855
ER -
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@article{2019_Zhao,
author = {Fei Zhao and Xu-Feng Zhou and Wei Deng and Zhaoping Liu},
title = {Entrapping lithium deposition in lithiophilic reservoir constructed by vertically aligned ZnO nanosheets for dendrite-free Li metal anodes},
journal = {Nano Energy},
year = {2019},
volume = {62},
publisher = {Elsevier},
month = {aug},
url = {https://doi.org/10.1016/j.nanoen.2019.04.087},
pages = {55--63},
doi = {10.1016/j.nanoen.2019.04.087}
}