Reactions of excess electrons with "bridged" amidoesters in low-temperature matrices
Publication type: Journal Article
Publication date: 2013-04-01
scimago Q2
wos Q1
SJR: 0.543
CiteScore: 5.6
Impact factor: 3.3
ISSN: 0969806X, 18790895
Radiation
Abstract
Abstract Structure of radical anions of “bridged” amidoesters MeOOC(CH2)nCONMe2 (n=0–3) generated by X-ray irradiation was investigated by EPR, optical absorption spectroscopy and quantum-chemical calculations. Amidoester-0 (n=0) has positive calculated electron affinity and the corresponding delocalized radical anion is stabilized independent of matrix polarity. Meanwhile, for amidoesters with n=1–3 groups possessing apparently negative intrinsic electron affinity the role of matrix in stabilization of the corresponding radical anions becomes crucial. Two types of the localized radical anions were observed in the latter case.
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Saenko E. V. et al. Reactions of excess electrons with "bridged" amidoesters in low-temperature matrices // Radiation Physics and Chemistry. 2013. Vol. 85. pp. 147-151.
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Saenko E. V., Laikov D., Feldman V. I. Reactions of excess electrons with "bridged" amidoesters in low-temperature matrices // Radiation Physics and Chemistry. 2013. Vol. 85. pp. 147-151.
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TY - JOUR
DO - 10.1016/j.radphyschem.2012.12.003
UR - https://linkinghub.elsevier.com/retrieve/pii/S0969806X12004999
TI - Reactions of excess electrons with "bridged" amidoesters in low-temperature matrices
T2 - Radiation Physics and Chemistry
AU - Saenko, Elizaveta V
AU - Laikov, Dimitri
AU - Feldman, Vladimir I.
PY - 2013
DA - 2013/04/01
PB - Elsevier
SP - 147-151
VL - 85
SN - 0969-806X
SN - 1879-0895
ER -
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@article{2013_Saenko,
author = {Elizaveta V Saenko and Dimitri Laikov and Vladimir I. Feldman},
title = {Reactions of excess electrons with "bridged" amidoesters in low-temperature matrices},
journal = {Radiation Physics and Chemistry},
year = {2013},
volume = {85},
publisher = {Elsevier},
month = {apr},
url = {https://linkinghub.elsevier.com/retrieve/pii/S0969806X12004999},
pages = {147--151},
doi = {10.1016/j.radphyschem.2012.12.003}
}