Scripta Materialia, volume 229, pages 115352
Uniform lithium deposition guided by Au nanoparticles in vertical-graphene/carbon-cloth skeleton for dendrite-free and stable lithium metal anode
Tingting Xu
1
,
Lijuan Hou
1
,
Congcong Yan
1
,
Jingrui Hou
1
,
Bofang Tian
1
,
Huiyu Yuan
2, 3
,
Dejin Kong
1
,
Hui Wang
1
,
Xinjian Li
1
,
Ye Wang
1
,
GUOPENG ZHANG
1
2
Key Laboratory of Henan Province for High Temperature Functional Materials, Zhengzhou, PR China
|
Publication type: Journal Article
Publication date: 2023-05-01
Metals and Alloys
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Mechanics of Materials
Abstract
Owing to the high electrochemical reactivity and infinite volume expansion of lithium metal anode, the uncontrollable lithium dendrite growth drags the lithium metal anode out of the real application for a long time. Herein, a heterogeneous seed layer of Au nanoparticles (NPs) is uniformly deposited on the 3D porous vertical graphene nanosheets on carbon cloth (Au-VG/CC) to construct a lithiophilic surface, achieving a smooth and dendrite-free morphology. As a result, Au-VG/CC electrode delivers a small voltage hysteresis of 67.2 mV and a long cycling life of more than 500 h at a high current density of 5 mA cm−2 with 5 mAh cm−2. Results of XRD and in-situ transmission electron microscopy indicate that the formed lithiophilic layer is Li3Au which can guide the lithium deposition. Moreover, a full battery assembled with [email protected]/CC as the anode and LiFePO4 as the cathode delivers 77.3 mAh g−1 at 100 mA g−1 after 200 cycles.
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Citations by publishers
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2 publications, 18.18%
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Wiley
2 publications, 18.18%
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1 publication, 9.09%
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1 publication, 9.09%
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1 publication, 9.09%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Xu T. et al. Uniform lithium deposition guided by Au nanoparticles in vertical-graphene/carbon-cloth skeleton for dendrite-free and stable lithium metal anode // Scripta Materialia. 2023. Vol. 229. p. 115352.
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Xu T., Hou L., Yan C., Hou J., Tian B., Yuan H., Kong D., Wang H., Li X., Wang Y., ZHANG G. Uniform lithium deposition guided by Au nanoparticles in vertical-graphene/carbon-cloth skeleton for dendrite-free and stable lithium metal anode // Scripta Materialia. 2023. Vol. 229. p. 115352.
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TY - JOUR
DO - 10.1016/j.scriptamat.2023.115352
UR - https://doi.org/10.1016/j.scriptamat.2023.115352
TI - Uniform lithium deposition guided by Au nanoparticles in vertical-graphene/carbon-cloth skeleton for dendrite-free and stable lithium metal anode
T2 - Scripta Materialia
AU - Xu, Tingting
AU - Hou, Lijuan
AU - Yan, Congcong
AU - Hou, Jingrui
AU - Tian, Bofang
AU - Yuan, Huiyu
AU - Kong, Dejin
AU - Wang, Hui
AU - Li, Xinjian
AU - Wang, Ye
AU - ZHANG, GUOPENG
PY - 2023
DA - 2023/05/01 00:00:00
PB - Elsevier
SP - 115352
VL - 229
SN - 1359-6462
ER -
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@article{2023_Xu,
author = {Tingting Xu and Lijuan Hou and Congcong Yan and Jingrui Hou and Bofang Tian and Huiyu Yuan and Dejin Kong and Hui Wang and Xinjian Li and Ye Wang and GUOPENG ZHANG},
title = {Uniform lithium deposition guided by Au nanoparticles in vertical-graphene/carbon-cloth skeleton for dendrite-free and stable lithium metal anode},
journal = {Scripta Materialia},
year = {2023},
volume = {229},
publisher = {Elsevier},
month = {may},
url = {https://doi.org/10.1016/j.scriptamat.2023.115352},
pages = {115352},
doi = {10.1016/j.scriptamat.2023.115352}
}