Solid State Ionics, volume 221, pages 1-5
Mechanochemical synthesis of Li-argyrodite Li6PS5X (X=Cl, Br, I) as sulfur-based solid electrolytes for all solid state batteries application
Publication type: Journal Article
Publication date: 2012-08-01
General Chemistry
Condensed Matter Physics
General Materials Science
Abstract
article i nfo Highly ion-conductive Li6PS5X (X = Cl, Br, I) Li-argyrodites were prepared through a high-energy ball milling. Electrical and electrochemical properties were investigated. Ball-milled compounds exhibit a high conductiv- ity between 2 and 7 × 10 − 4 S/cm with an activation energy of 0.3-0.4 eV for conduction. These attractive proper- ties were attributed to the spontaneous formation of crystallized Li-argyrodite during ball-milling. An optimization of milling time led to a conductivity of 1.33×10 −3 S/cm for the Li6PS5Cl phase with an electrochemical stability up to 7 V vs. lithium. An all solid state LiCoO2/Elec./In lithium ion battery using ball-milled Li6PS5Cl as electrolyte was suc- cessfully assembled, and its room temperature performance is reported.
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- We do not take into account publications without a DOI.
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Boulineau S. et al. Mechanochemical synthesis of Li-argyrodite Li6PS5X (X=Cl, Br, I) as sulfur-based solid electrolytes for all solid state batteries application // Solid State Ionics. 2012. Vol. 221. pp. 1-5.
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Boulineau S., Courty M., Tarascon J., Viallet V. Mechanochemical synthesis of Li-argyrodite Li6PS5X (X=Cl, Br, I) as sulfur-based solid electrolytes for all solid state batteries application // Solid State Ionics. 2012. Vol. 221. pp. 1-5.
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TY - JOUR
DO - 10.1016/j.ssi.2012.06.008
UR - https://doi.org/10.1016/j.ssi.2012.06.008
TI - Mechanochemical synthesis of Li-argyrodite Li6PS5X (X=Cl, Br, I) as sulfur-based solid electrolytes for all solid state batteries application
T2 - Solid State Ionics
AU - Boulineau, Sylvain
AU - Courty, Matthieu
AU - Tarascon, Jean-Marie
AU - Viallet, Virginie
PY - 2012
DA - 2012/08/01 00:00:00
PB - Elsevier
SP - 1-5
VL - 221
SN - 0167-2738
ER -
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@article{2012_Boulineau,
author = {Sylvain Boulineau and Matthieu Courty and Jean-Marie Tarascon and Virginie Viallet},
title = {Mechanochemical synthesis of Li-argyrodite Li6PS5X (X=Cl, Br, I) as sulfur-based solid electrolytes for all solid state batteries application},
journal = {Solid State Ionics},
year = {2012},
volume = {221},
publisher = {Elsevier},
month = {aug},
url = {https://doi.org/10.1016/j.ssi.2012.06.008},
pages = {1--5},
doi = {10.1016/j.ssi.2012.06.008}
}