Solid State Ionics, volume 253, pages 175-180
Water-stable lithium ion conducting solid electrolyte of the Li1.4Al0.4Ti1.6 − xGex(PO4)3 system (x = 0–1.0) with NASICON-type structure
Publication type: Journal Article
Publication date: 2013-12-01
General Chemistry
Condensed Matter Physics
General Materials Science
Abstract
Solid ionic conductors composed of Li 1.4 Al 0.4 Ti 1.6 − x Ge x (PO 4 ) 3 (x = 0–1.0) with the NASICON-type structure were synthesized with a precursor prepared using the sol–gel method. The electrical conductivity was examined as a function of x in Li 1.4 Al 0.4 Ti 1.6 − x Ge x (PO 4 ) 3 at various sintering temperatures and for various sintering periods. The highest electrical conductivity was obtained for Li 1.4 Al 0.4 Ti 1.4 Ge 0.2 (PO 4 ) 3 sintered at 900 °C for 11 h in air. The total and bulk conductivities of the sintered pellet were 1.29 × 10 − 3 and 2.35 × 10 − 3 S cm − 1 at 25 °C, respectively. The grain boundary resistance of Li 1.4 Al 0.4 Ti 1.4 Ge 0.2 (PO 4 ) 3 was significantly increased to 552 Ω cm 2 from 12.2 Ω cm 2 by immersion in distilled water at 50 °C for one week, whereas the bulk resistance was not increased. However, no significant increase of the bulk and grain boundary resistance was observed after immersion in a saturated aqueous solution of LiOH and LiCl.
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Zhang P. et al. Water-stable lithium ion conducting solid electrolyte of the Li1.4Al0.4Ti1.6 − xGex(PO4)3 system (x = 0–1.0) with NASICON-type structure // Solid State Ionics. 2013. Vol. 253. pp. 175-180.
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Zhang P., Matsui M., Hirano A., TAKEDA Y., Yamamoto O., Imanishi N. Water-stable lithium ion conducting solid electrolyte of the Li1.4Al0.4Ti1.6 − xGex(PO4)3 system (x = 0–1.0) with NASICON-type structure // Solid State Ionics. 2013. Vol. 253. pp. 175-180.
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TY - JOUR
DO - 10.1016/j.ssi.2013.09.022
UR - https://doi.org/10.1016/j.ssi.2013.09.022
TI - Water-stable lithium ion conducting solid electrolyte of the Li1.4Al0.4Ti1.6 − xGex(PO4)3 system (x = 0–1.0) with NASICON-type structure
T2 - Solid State Ionics
AU - Zhang, Peng
AU - Matsui, Masaki
AU - Hirano, Atsushi
AU - TAKEDA, Yasuo
AU - Yamamoto, Osamu
AU - Imanishi, Nobuyuki
PY - 2013
DA - 2013/12/01 00:00:00
PB - Elsevier
SP - 175-180
VL - 253
SN - 0167-2738
ER -
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@article{2013_Zhang,
author = {Peng Zhang and Masaki Matsui and Atsushi Hirano and Yasuo TAKEDA and Osamu Yamamoto and Nobuyuki Imanishi},
title = {Water-stable lithium ion conducting solid electrolyte of the Li1.4Al0.4Ti1.6 − xGex(PO4)3 system (x = 0–1.0) with NASICON-type structure},
journal = {Solid State Ionics},
year = {2013},
volume = {253},
publisher = {Elsevier},
month = {dec},
url = {https://doi.org/10.1016/j.ssi.2013.09.022},
pages = {175--180},
doi = {10.1016/j.ssi.2013.09.022}
}