Solid State Ionics, volume 284, pages 61-70

Structural and electrolyte properties of Li4P2S6

Miaofang Chi ^{1, 2, 3}

Cameron Kates ⁴

Melanie Kirkham ⁵

Shiba Prasad Adhikari ⁶

Chengdu Liang ^{1, 2, 3}

Natalie Holzwarth ⁴

Hide authors affiliations Show authors affiliations: 6 affiliations

Center for Nanophase Materials Sciences

Oak Ridge National laboratory |

Oak Ridge TN 37831 USA |

⁴

Department of Physics, Wake Forest University, Winston-Salem, NC 27109-7507, USA |

⁵

Spallation Neutron Source , Oak Ridge National Laboratory , Oak Ridge, TN, 37831, USA |

⁶

Department of Chemistry, Wake Forest University, Winston-Salem, NC 27109-7486, USA. |

Publication type: Journal Article

Publication date: 2016-01-01

Elsevier

Journal: Solid State Ionics

Quartile SCImago

Quartile WOS

Impact factor: 3.2

ISSN: 01672738

DOI: 10.1016/j.ssi.2015.10.015

Copy DOI

General Chemistry

Condensed Matter Physics

General Materials Science

Abstract

Experiment and simulations are used to investigate the structural and electrolyte properties of Li4P2S6. Compared with other thiophosphate materials, Li4P2S6 is quite stable, maintaining its crystal structure up to temperatures as high as 950 °C in vacuum and up to 280 °C in air. While its ionic conductivity is small, 2.38 × 10− 7 S/cm at 25 °C and 2.33 × 10− 6 S/cm at 100 °C, its Arrhenius activation energy of 0.29 eV is similar to technologically viable electrolytes. Computer simulations provide insight into the causes and effects of disorder in this material and also indicate that the mechanism of the ion conduction is dominated by interstitial sites.

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Citations by publishers

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Elsevier	Elsevier, 12, 19.67% Elsevier 12 publications, 19.67%
American Chemical Society (ACS)	American Chemical Society (ACS), 11, 18.03% American Chemical Society (ACS) 11 publications, 18.03%
Wiley	Wiley, 11, 18.03% Wiley 11 publications, 18.03%
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American Physical Society (APS)	American Physical Society (APS), 5, 8.2% American Physical Society (APS) 5 publications, 8.2%
Springer Nature	Springer Nature, 5, 8.2% Springer Nature 5 publications, 8.2%
The Electrochemical Society	The Electrochemical Society, 3, 4.92% The Electrochemical Society 3 publications, 4.92%
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Ceramic Society of Japan	Ceramic Society of Japan, 1, 1.64% Ceramic Society of Japan 1 publication, 1.64%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 1.64% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 1.64%
IOP Publishing	IOP Publishing, 1, 1.64% IOP Publishing 1 publication, 1.64%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.64% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.64%
	2 4 6 8 10 12

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Chi M. et al. Structural and electrolyte properties of Li4P2S6 // Solid State Ionics. 2016. Vol. 284. pp. 61-70.

GOST all authors (up to 50) Copy

Chi M., Kates C., Kirkham M., Adhikari S. P., Liang C., Holzwarth N. Structural and electrolyte properties of Li4P2S6 // Solid State Ionics. 2016. Vol. 284. pp. 61-70.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1016/j.ssi.2015.10.015

UR - https://doi.org/10.1016/j.ssi.2015.10.015

TI - Structural and electrolyte properties of Li4P2S6

T2 - Solid State Ionics

AU - Chi, Miaofang

AU - Kates, Cameron

AU - Kirkham, Melanie

AU - Adhikari, Shiba Prasad

AU - Liang, Chengdu

AU - Holzwarth, Natalie

PY - 2016

DA - 2016/01/01 00:00:00

PB - Elsevier

SP - 61-70

VL - 284

SN - 0167-2738

ER -

BibTex

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BibTex Copy

@article{2016_Chi,

author = {Miaofang Chi and Cameron Kates and Melanie Kirkham and Shiba Prasad Adhikari and Chengdu Liang and Natalie Holzwarth},

title = {Structural and electrolyte properties of Li4P2S6},

journal = {Solid State Ionics},

year = {2016},

volume = {284},

publisher = {Elsevier},

month = {jan},

url = {https://doi.org/10.1016/j.ssi.2015.10.015},

pages = {61--70},

doi = {10.1016/j.ssi.2015.10.015}

}

Found error?

Publisher

Elsevier

Journal

Solid State Ionics

Quartile SCImago

Quartile WOS

Impact factor

3.2

ISSN

01672738 (Print)