Solid State Ionics, volume 289, pages 180-187

Effect of simultaneous addition of aluminum and chromium on the lithium ionic conductivity of LiGe2(PO4)3 NASICON-type glass–ceramics

Mohammad Illbeigi ¹

Alireza Fazlali ¹

Mahdi Kazazi ²

Amir Mohammadi ^{3, 4}

Hide authors affiliations Show authors affiliations: 4 affiliations

Department of Chemical Engineering, Faculty of Engineering , Arak University , Arak, Iran |

Department of Materials Engineering, Faculty of Engineering, Malayer University, Malayer, Iran |

Département de Génie des Mines, de la Métallurgie et des Matériaux, Faculté des Sciences et de Génie, Université Laval, Québec, (QC) G1V 0A6, Canada |

⁴

Thermodynamics Research Unit, School of Engineering, University of KwaZulu-Natal, Howard College Campus, King George V Avenue, Durban 4041, South Africa |

Publication type: Journal Article

Publication date: 2016-06-01

Elsevier

Journal: Solid State Ionics

Quartile SCImago

Quartile WOS

Impact factor: 3.2

ISSN: 01672738

DOI: 10.1016/j.ssi.2016.03.012

Copy DOI

General Chemistry

Condensed Matter Physics

General Materials Science

Abstract

New high lithium ion conductor glass–ceramics with NASICON-type structure (Li 1 + x + y Al x Cr y Ge 2 − x − y (PO 4 ) 3 , x + y = 0.5) were synthesized using melt-quenching method and converted to glass–ceramics through heat treatment. Influence of addition of different concentrations of aluminum and chromium in LiGe 2 (PO 4 ) 3 glass-ceramic was investigated. Substitution of Ge 4 + ions by Al 3 + and Cr 3 + ions induced more Li + ions in A 2 vacant sites and also changed the unit cell parameters and resulted in ionic conductivity improvement of glass–ceramics. The glass–ceramics were characterized by X-ray Diffraction (XRD), Field Emission Scanning Electron Microscopy (FESEM), Energy-Dispersive X-ray spectroscopy (EDX), Differential Scanning Calorimetry (DSC), Complex Impedance Spectroscopy (CIS) and cyclic voltammetry (CV). The highest lithium ion conductivity of 6.65 × 10 − 3 S/cm was obtained for x = 0.4 and y = 0.1 (Li 1.5 Al 0.4 Cr 0.1 Ge 1.5 (PO 4 ) 3 ) crystallized at 850 °C for 8 h with minimum activation energy of 0.292 eV.

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Elsevier	Elsevier, 18, 34.62% Elsevier 18 publications, 34.62%
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American Chemical Society (ACS)	American Chemical Society (ACS), 1, 1.92% American Chemical Society (ACS) 1 publication, 1.92%
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OAE Publishing Inc.	OAE Publishing Inc., 1, 1.92% OAE Publishing Inc. 1 publication, 1.92%
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Illbeigi M. et al. Effect of simultaneous addition of aluminum and chromium on the lithium ionic conductivity of LiGe2(PO4)3 NASICON-type glass–ceramics // Solid State Ionics. 2016. Vol. 289. pp. 180-187.

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Illbeigi M., Fazlali A., Kazazi M., Mohammadi A. Effect of simultaneous addition of aluminum and chromium on the lithium ionic conductivity of LiGe2(PO4)3 NASICON-type glass–ceramics // Solid State Ionics. 2016. Vol. 289. pp. 180-187.

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RIS Copy

TY - JOUR

DO - 10.1016/j.ssi.2016.03.012

UR - https://doi.org/10.1016/j.ssi.2016.03.012

TI - Effect of simultaneous addition of aluminum and chromium on the lithium ionic conductivity of LiGe2(PO4)3 NASICON-type glass–ceramics

T2 - Solid State Ionics

AU - Illbeigi, Mohammad

AU - Fazlali, Alireza

AU - Kazazi, Mahdi

AU - Mohammadi, Amir

PY - 2016

DA - 2016/06/01 00:00:00

PB - Elsevier

SP - 180-187

VL - 289

SN - 0167-2738

ER -

BibTex

Cite this

BibTex Copy

@article{2016_Illbeigi,

author = {Mohammad Illbeigi and Alireza Fazlali and Mahdi Kazazi and Amir Mohammadi},

title = {Effect of simultaneous addition of aluminum and chromium on the lithium ionic conductivity of LiGe2(PO4)3 NASICON-type glass–ceramics},

journal = {Solid State Ionics},

year = {2016},

volume = {289},

publisher = {Elsevier},

month = {jun},

url = {https://doi.org/10.1016/j.ssi.2016.03.012},

pages = {180--187},

doi = {10.1016/j.ssi.2016.03.012}

}

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Elsevier

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Solid State Ionics

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Quartile WOS

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01672738 (Print)