Palladium-catalyzed propargylative and allenylative dearomatization of 2-(chloromethyl)thiophenes: remarkable effect of solvents
Publication type: Journal Article
Publication date: 2016-01-01
scimago Q3
wos Q2
SJR: 0.426
CiteScore: 4.1
Impact factor: 2.2
ISSN: 00404020, 14645416
Organic Chemistry
Drug Discovery
Biochemistry
Abstract
Palladium-catalyzed a solvent-dependent product distribution in the propargylative and allenylative dearomatization reaction of 2-(chloromethyl)thiophenes with allenyltributylstannane under mild conditions is reported in this study. In the coordinating solvent acetonitrile, the propargylative dearomatization reaction selectively occurred to produce only the propargylic compounds with satisfactory to good yield. In the uncoordinating solvent dichloromethane, allenic compounds were obtained as major products with a small amount of propargylic compounds.
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GOST
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Ullah A. et al. Palladium-catalyzed propargylative and allenylative dearomatization of 2-(chloromethyl)thiophenes: remarkable effect of solvents // Tetrahedron. 2016. Vol. 72. No. 1. pp. 170-175.
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Ullah A., Zhang S., Bao M., Yamamoto Y., Almansour A. I., Arumugam N., Kumar R. S. Palladium-catalyzed propargylative and allenylative dearomatization of 2-(chloromethyl)thiophenes: remarkable effect of solvents // Tetrahedron. 2016. Vol. 72. No. 1. pp. 170-175.
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TY - JOUR
DO - 10.1016/j.tet.2015.11.020
UR - https://doi.org/10.1016/j.tet.2015.11.020
TI - Palladium-catalyzed propargylative and allenylative dearomatization of 2-(chloromethyl)thiophenes: remarkable effect of solvents
T2 - Tetrahedron
AU - Ullah, Aziz
AU - Zhang, Sheng
AU - Bao, Ming
AU - Yamamoto, Yoshinori
AU - Almansour, Abdulrahman I.
AU - Arumugam, Natarajan
AU - Kumar, Raju Suresh
PY - 2016
DA - 2016/01/01
PB - Elsevier
SP - 170-175
IS - 1
VL - 72
SN - 0040-4020
SN - 1464-5416
ER -
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BibTex (up to 50 authors)
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@article{2016_Ullah,
author = {Aziz Ullah and Sheng Zhang and Ming Bao and Yoshinori Yamamoto and Abdulrahman I. Almansour and Natarajan Arumugam and Raju Suresh Kumar},
title = {Palladium-catalyzed propargylative and allenylative dearomatization of 2-(chloromethyl)thiophenes: remarkable effect of solvents},
journal = {Tetrahedron},
year = {2016},
volume = {72},
publisher = {Elsevier},
month = {jan},
url = {https://doi.org/10.1016/j.tet.2015.11.020},
number = {1},
pages = {170--175},
doi = {10.1016/j.tet.2015.11.020}
}
Cite this
MLA
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Ullah, Aziz, et al. “Palladium-catalyzed propargylative and allenylative dearomatization of 2-(chloromethyl)thiophenes: remarkable effect of solvents.” Tetrahedron, vol. 72, no. 1, Jan. 2016, pp. 170-175. https://doi.org/10.1016/j.tet.2015.11.020.