Suzuki polycondensation for the synthesis of polytriarylamines: A method to improve hole-transport material performance in perovskite solar cells
Publication type: Journal Article
Publication date: 2020-09-01
scimago Q3
wos Q3
SJR: 0.334
CiteScore: 3.2
Impact factor: 1.5
ISSN: 00404039, 18733581
Organic Chemistry
Drug Discovery
Biochemistry
Abstract
Polytriarylamines have attracted significant interest as hole transport materials for organic electronics. Herein we report the synthesis of a polytriarylamine (PTAA) using the Suzuki polycondensation reaction. The Pd-based catalytic system was optimized to obtain a polymer with a high molecular weight and low polydispersity. The synthesized PTAA polymer was evaluated as a hole transport material in perovskite solar cells with n-i-p configuration. The devices showed an improved power conversion efficiency of 17.6% and an open-circuit voltage of 1.06 V, whereas the referenced cells based on commercial PTAA delivered a lower efficiency of 16.7% and an open-circuit voltage of 1.02 V. Thus, the proposed synthetic approach yields high-quality PTAA with improved electrical properties.
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Total citations:
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Tepliakova M. M. et al. Suzuki polycondensation for the synthesis of polytriarylamines: A method to improve hole-transport material performance in perovskite solar cells // Tetrahedron Letters. 2020. Vol. 61. No. 38. p. 152317.
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Tepliakova M. M., Akkuratov A. V., Tsarev S., Troshin P. A. Suzuki polycondensation for the synthesis of polytriarylamines: A method to improve hole-transport material performance in perovskite solar cells // Tetrahedron Letters. 2020. Vol. 61. No. 38. p. 152317.
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RIS
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TY - JOUR
DO - 10.1016/j.tetlet.2020.152317
UR - https://linkinghub.elsevier.com/retrieve/pii/S0040403920307905
TI - Suzuki polycondensation for the synthesis of polytriarylamines: A method to improve hole-transport material performance in perovskite solar cells
T2 - Tetrahedron Letters
AU - Tepliakova, Marina M.
AU - Akkuratov, Alexander V.
AU - Tsarev, Sergey
AU - Troshin, Pavel A.
PY - 2020
DA - 2020/09/01
PB - Elsevier
SP - 152317
IS - 38
VL - 61
SN - 0040-4039
SN - 1873-3581
ER -
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BibTex (up to 50 authors)
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@article{2020_Tepliakova,
author = {Marina M. Tepliakova and Alexander V. Akkuratov and Sergey Tsarev and Pavel A. Troshin},
title = {Suzuki polycondensation for the synthesis of polytriarylamines: A method to improve hole-transport material performance in perovskite solar cells},
journal = {Tetrahedron Letters},
year = {2020},
volume = {61},
publisher = {Elsevier},
month = {sep},
url = {https://linkinghub.elsevier.com/retrieve/pii/S0040403920307905},
number = {38},
pages = {152317},
doi = {10.1016/j.tetlet.2020.152317}
}
Cite this
MLA
Copy
Tepliakova, Marina M., et al. “Suzuki polycondensation for the synthesis of polytriarylamines: A method to improve hole-transport material performance in perovskite solar cells.” Tetrahedron Letters, vol. 61, no. 38, Sep. 2020, p. 152317. https://linkinghub.elsevier.com/retrieve/pii/S0040403920307905.