Effect of CeO2 addition on Ni/Al2O3 catalysts for methanation of carbon dioxide with hydrogen
Тип публикации: Journal Article
Дата публикации: 2012-11-01
Organic Chemistry
General Chemical Engineering
Energy Engineering and Power Technology
Краткое описание
The Ni-CeO2/Al2O3 catalysts with a nickel content of 15 wt% prepared via impregnating boehmite were found to be highly active and stable for methanation of carbon dioxide with hydrogen at a H2/CO2 molar ratio of 4. The effects of CeO2 content and reaction temperature on the performance of the Ni-CeO2/Al2O3 catalysts were studied in detail. The results showed that the catalytic performance was strongly dependent on the CeO2 content in Ni-CeO2/Al2O3 catalysts and that the catalysts with 2 wt% CeO2 had the highest catalytic activity among the tested ones at 350 °C. The XRD and H2-TPR characterizations revealed that the addition of CeO2 decreased the reduction temperature by altering the interaction between Ni and Al2O3, and improved the reducibility of the catalyst. Preliminary stability test of 120 h on stream over the Ni-2CeO2/Al2O3 catalyst at 350 °C revealed that the catalyst was much better than the unpromoted one.
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Liu H. et al. Effect of CeO2 addition on Ni/Al2O3 catalysts for methanation of carbon dioxide with hydrogen // Journal of Natural Gas Chemistry. 2012. Vol. 21. No. 6. pp. 703-707.
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Liu H., Zou X., Wang X., Lu X., Ding W. Effect of CeO2 addition on Ni/Al2O3 catalysts for methanation of carbon dioxide with hydrogen // Journal of Natural Gas Chemistry. 2012. Vol. 21. No. 6. pp. 703-707.
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TY - JOUR
DO - 10.1016/s1003-9953(11)60422-2
UR - https://doi.org/10.1016/s1003-9953(11)60422-2
TI - Effect of CeO2 addition on Ni/Al2O3 catalysts for methanation of carbon dioxide with hydrogen
T2 - Journal of Natural Gas Chemistry
AU - Liu, Hezhi
AU - Zou, Xingli
AU - Wang, Xuguang
AU - Lu, Xionggang
AU - Ding, Weizhong
PY - 2012
DA - 2012/11/01
PB - Elsevier
SP - 703-707
IS - 6
VL - 21
SN - 1003-9953
ER -
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@article{2012_Liu,
author = {Hezhi Liu and Xingli Zou and Xuguang Wang and Xionggang Lu and Weizhong Ding},
title = {Effect of CeO2 addition on Ni/Al2O3 catalysts for methanation of carbon dioxide with hydrogen},
journal = {Journal of Natural Gas Chemistry},
year = {2012},
volume = {21},
publisher = {Elsevier},
month = {nov},
url = {https://doi.org/10.1016/s1003-9953(11)60422-2},
number = {6},
pages = {703--707},
doi = {10.1016/s1003-9953(11)60422-2}
}
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MLA
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Liu, Hezhi, et al. “Effect of CeO2 addition on Ni/Al2O3 catalysts for methanation of carbon dioxide with hydrogen.” Journal of Natural Gas Chemistry, vol. 21, no. 6, Nov. 2012, pp. 703-707. https://doi.org/10.1016/s1003-9953(11)60422-2.